Climate sensitivity to cloud optical properties

A radiative–convective model was developed to investigate the sensitivity of climate to cloud optical properties and the related feedback processes. This model demonstrates that the Earth's surface temperature increases with cloud optical depth when the clouds are very thin but decreases with cloud optical depth when the cloud shortwave (solar) radiative forcing is larger than the cloud longwave (terrestrial) radiative forcing. When clouds are included in the model, the magnitude of the greenhouse effect due to a doubling of the CO₂ concentration varies with the cloudoptical depth: the thicker the clouds, the weaker the greenhouse warming. In addition, a small variation in the cloud droplet size has a larger impact on the equilibrium state temperature in the lower atmosphere than the warming caused by a doubling of the CO₂ concentration: a 2% increase in the average cloud droplet size per degree increase in temperature doubles the warming caused by the doubling of the CO₂ concentration. These findings suggest that physically reliable correlations between the cloud droplet size and macrophysical meteorological variables such as temperature, wind and water vapor fields are needed on a global climate scale to assess the climate impact of increases in greenhouse gases.     

Direct Radiative Forcing of Anthropogenic Aerosols over Oceans from Satellite Observations

Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases.     

温室气体和硫酸盐气溶胶的辐射强迫作用

对GOALS4 .0海 陆 气耦合模式的相关部分进行了改进 ,主要改进包括温室气体的扩充和硫酸盐气溶胶“显式”方案的引入 ,并引入 2 0世纪温室气体的实际浓度变化以及硫循环模式模拟的硫酸盐气溶胶的三维全球浓度分布 ,模拟了温室气体和硫酸盐气溶胶造成的辐射强迫的空间分布和时间变化。全球平均的温室气体和硫酸盐气溶胶的辐射强迫分别为 2 .17W /m2 和 - 0 .2 9W /m2 ;温室气体造成的辐射强迫在空间上呈现明显的纬向结构 ,最大值 (大于 2 .5W/m2 )和最小值 (小于 1W /m2 )分别位于副热带和两极地区 ,在北半球主要工业区硫酸盐气溶胶的辐射强迫绝对值接近温室气体的辐射强迫值 (大于 - 2 .0W /m2 )。     

The dynamics of the Indian Ocean sea surface temperature forcing of Sahel drought

Given the pronounced warming in the Indian Ocean sea surface temperature (SST) during the second half of the twentieth century and the empirical relationship between the Indian Ocean SST and Sahel summer precipitation, we investigate the mechanisms underlying this relationship using the GFDL atmospheric model AM2.0 to simulate the equilibrium and transient response to the warming of the Indian Ocean. Equatorial wave dynamics, in particular the westward propagating equatorial Rossby waves, communicates the signal of tropospheric warming and stabilization from the Indian Ocean to the African continent. The stabilization associated with the Rossby wave front acts to suppress the convection. Feedbacks with local precipitation and depletion of moisture amplify the dynamically induced subsidence. While this stabilization mechanism is expected to operate in climate change response, the future prospects for the Sahelian climate under global warming are complicated by the intricate sensitivities to the SSTs from different ocean basins and to the direct radiative forcing of greenhouse gases.     

黑碳气溶胶辐射强迫全球分布的模拟研究

利用一个改进的辐射传输模式,结合全球气溶胶数据集（GADS）,计算晴空条件下冬夏两季黑碳气溶胶的直接辐射强迫在对流层顶和地面的全球分布。计算结果表明,与温室气体引起的整层大气都是正的辐射强迫不同,黑碳气溶胶的辐射强迫在对流层顶为正值,而在地面的辐射强迫却是负值。作者从理论上解释了造成这种结果的原因。对北半球冬季和夏季而言,在对流层顶黑碳气溶胶的全球辐射强迫的平均值分别为0.085W/m2和0.155 W/m2,在地面则分别为-0.37 W/m2和-0.63 W/m2。虽然气溶胶的辐射强迫主要依赖于其本身的光学性质和在大气中的浓度,太阳高度角和地表反照率对黑碳气溶胶的辐射强迫会产生很大的影响。研究指出:黑碳气溶胶在对流层顶正的辐射强迫和在地面负的辐射强迫的绝对值都随太阳天顶角的余弦和地表反照率的增加线性增大;地表反照率对黑碳气溶胶辐射强迫的强度和分布都有重要影响。黑碳气溶胶的辐射强迫分布具有明显的纬度变化特征,冬夏两季的大值区都位于30°N~90°N之间,表明人类活动是造成黑碳气溶胶辐射强迫的主要原因。     

人类活动对气候影响的研究Ⅱ.对东亚和中国气候变化的影响

系统总结和介绍了20世纪90年代以来作者所开展的有关人类活动对东亚和中国气候影响的一系列研究活动.其中包括温室气体辐射强迫及其气候效应,大气微量气体的全球增温潜能,对流层和平流层气溶胶的辐射气候效应,气候系统外部因子对中国气候影响的总体评估,人类活动对中国和东亚地区未来气候变化的影响,以及20世纪和21世纪东亚及中国的气候变化.同时给出了一系列研究成果,这些研究成果对于正确认识和准确预测东亚地区以及中国气候变化具有十分重要的意义.     

SF6气体的辐射强迫和全球增温潜能的研究

IPCC(2007)指出, 六氟化硫(SF6) 作为臭氧消耗物质 (ODSs) 的部分替代物质, 近年来排放量大大增加。它作为控制排放的人造长寿命温室气体之一已经被列入《京都议定书》。但是, 目前在臭氧消耗物质替代品中, 对SF6的辐射强迫和全球增温潜能的研究较少, 而且所用的谱吸收资料陈旧。本文采用最新的分子吸收数据库HITRAN2004中的SF6的吸收截面数据, 利用Shi(1981) 的吸收系数重排法, 建立了SF6的相关k分布的辐射计算方案, 在此基础上研究了SF6在晴空大气下的辐射效率和全球增温潜能, 并首次计算了SF6的全球温变潜能, 与其全球增温潜能进行了比较。本文的研究表明: SF6的辐射效率为0.512 W/m2, 经过大气寿命调整之后的辐射效率为0.506 W/m2, 二者差别不大; 根据IPCC (2007) 给出的排放情景, 到2100年, SF6在大气中的体积分数将达到35×10-12～70×10-12, 引起的相应辐射强迫将在0.004～0.028 W/m2之间变化; 相对于二氧化碳的100年全球增温潜能为2.33×104, 比IPCC(2007)的结果大2.2%; 100年的持续排放的全球增温潜能为2.26×104, 与其他长寿命人造温室气体一道, 其对全球变暖的长期影响不容忽视。     

Climate response to the physiological impact of carbon dioxide on plants in the Met Office Unified Model HadCM3

The concentration of carbon dioxide in the atmosphere acts to control the stomatal conductance of plants. There is observational and modelling evidence that an increase in the atmospheric concentration of CO₂ would suppress the evapotranspiration (ET) rate over land. This process is known as CO₂ physiological forcing and has been shown to induce changes in surface temperature and continental runoff. We analyse two transient climate simulations for the twenty-first century to isolate the climate response to the CO₂ physiological forcing. The land surface warming associated with the decreased ET rate is accompanied by an increase in the atmospheric lapse rate, an increase in specific humidity, but a decrease in relative humidity and stratiform cloud over land. We find that the water vapour feedback more than compensates for the decrease in latent heat flux over land as far as the budget of atmospheric water vapour is concerned. There is evidence that surface snow, water vapour and cloudiness respond to the CO₂ physiological forcing and all contribute to further warm the climate system. The climate response to the CO₂ physiological forcing has a quite different signature to that from the CO₂ radiative forcing, especially in terms of the changes in the temperature vertical profile and surface energy budget over land.     

Hydrological changes in the climate system from leaf responses to increasing CO2

Vegetation is a major component of the climate system because of its controls on the energy and water balance over land. This functioning changes because of the physiological response of leaves to increased CO₂. A climate model is used to compare these changes with the climate changes from radiative forcing by greenhouse gases. For this purpose, we use the Community Earth System Model coupled to a slab ocean. Ensemble integrations are done for current and doubled CO₂. The consequent reduction of transpiration and net increase of surface radiative heating from reduction in cloudiness increases the temperature over land by a significant fraction of that directly from the radiative warming by CO₂. Large-scale atmospheric circulation adjustments result. In particular, over the tropics, a low-level westerly wind anomaly develops associated with reduced geopotential height over land, enhancing moisture transport and convergence, and precipitation increases over the western Amazon, the Congo basin, South Africa, and Indonesia, while over mid-latitudes, land precipitation decreases from reduced evapotranspiration. On average, land precipitation is enhanced by 0.03 mm day^?1 (about 19 % of the CO₂ radiative forcing induced increase). This increase of land precipitation with decreased ET is an apparent negative feedback, i.e., less ET makes more precipitation. Global precipitation is slightly reduced. Runoff increases associated with both the increased land precipitation and reduced evapotranspiration. Examining the consistency of the variations among ensemble members shows that vegetation feedbacks on precipitation are more robust over the tropics and in mid to high latitudes than over the subtropics where vegetation is sparse and the internal climate variability has a larger influence.     

Stratospheric Temperature Changes and Ozone Recovery in the 21st Century

Increasing greenhouse gases and likely ozone recovery will be the two most important factors influencing changes in stratospheric temperatures in the 21st century. The radiative effect of increasing greenhouse gases will cause cooling in the stratosphere, while ozone recovery will lead to stratospheric warming. To investigate how stratospheric temperatures change under the two opposite forcings in the 21st century, we use observed ozone and reanalysis data as well as simulation results from four coupled oceanic and atmo- spheric general circulation models （GISS-ER, GFDL-CM20, NCAR-CCSM3, and UKMO-HadCM3） used in the IPCC （Intergovernment Panel for Climate Change） Fourth Assessment Report （AR4）. Observational analysis shows that total column ozone and lower stratospheric temperatures all show increasing in the past 10 years, while middle stratospheric temperatures demonstrate cooling. IPCC AR4 simulations show that greenhouse forcing alone will lead to stratospheric cooling. However, with forcing of both increasing greenhouse gases and ozone recovery, the middle stratosphere will be cooled, while the lower stratosphere will be warmed. Warming magnitudes vary from one model to another. UKMO-HadCM3 generates relatively strong warming for all three greenhouse scenarios, and warming extends to 40 hPa. GFDL-CM20 and NCAR-CCSM3 produce weak warming, and warming mainly exists at lower levels, below about 60 hPa. In addition, we also discuss the effect of temperature changes on ozone recovery.     

Future impact of anthropogenic sulfate aerosol on North Atlantic climate

We examine the simulated future change of the North Atlantic winter climate influenced by anthropogenic greenhouses gases and sulfate aerosol. Two simulations performed with the climate model ECHAM4/OPYC3 are investigated: a simulation forced by greenhouse gases and a simulation forced by greenhouse gases and sulfate aerosol. Only the direct aerosol effect on the clear-sky radiative fluxes is considered. The sulfate aerosol has a significant impact on temperature, radiative quantities, precipitation and atmospheric dynamics. Generally, we find a similar, but weaker future climate response if sulfate aerosol is considered additionally. Due to the induced negative top-of-the-atmosphere radiative forcing, the future warming is attenuated. We find no significant future trends in North Atlantic Oscillation (NAO) index in both simulations. However, the aerosol seems to have a balancing effect on the occurence of extreme NAO events. The simulated correlation patterns of the NAO index with temperature and precipitation, respectively, agree well with observations up to the present. The extent of the regions influenced by the NAO tends to be reduced under strong greenhouse gas forcing. If sulfate is included and the warming is smaller, this tendency is reversed. Also, the future decrease in baroclinicity is smaller due to the aerosols’ cooling effect and the poleward shift in track density is partly offset. Our findings imply that in simulations where aerosol cooling is neglected, the magnitude of the future warming over the North Atlantic region is overestimated, and correlation patterns differ from those based on the future simulation including aerosols.     

CFCs及其代用品的全球增温潜能

本文用一维辐射·对流模式系统地研究了现有含氯氟烃气体(CFCs)及其可能代用品的辐射强迫、比地面增温效应和全球增温潜能(GWP).结果发现:大多数提议的代用品的GWP值明显小于现有的CFCs.这主要归因于:(1)它们所产生的辐射强迫和比地面增温效应较小,一般只有CFCs的50％—60％;(2)其大气寿命比CFCs短得多.     

The Role Of Halocarbons In The Climate Change Of The Troposphere And Stratosphere

Releases of halocarbons into the atmosphere over the last 50 years are among the factors that have contributed to changes in the Earth’s climate since pre-industrial times. Their individual and collective potential to contribute directly to surface climate change is usually gauged through calculation of their radiative efficiency, radiative forcing, and/or Global Warming Potential (GWP). For those halocarbons that contain chlorine and bromine, indirect effects on temperature via ozone layer depletion represent another way in which these gases affect climate. Further, halocarbons can also affect the temperature in the stratosphere. In this paper, we use a narrow-band radiative transfer model together with a range of climate models to examine the role of these gases on atmospheric temperatures in the stratosphere and troposphere. We evaluate in detail the halocarbon contributions to temperature changes at the tropical tropopause, and find that they have contributed a significant warming of ~0.4 K over the last 50 years, dominating the effect of the other well-mixed greenhouse gases at these levels. The fact that observed tropical temperatures have not warmed strongly suggests that other mechanisms may be countering this effect. In a climate model this warming of the tropopause layer is found to lead to a 6% smaller climate sensitivity for halocarbons on a globally averaged basis, compared to that for carbon dioxide changes. Using recent observations together with scenarios we also assess their past and predicted future direct and indirect roles on the evolution of surface temperature. We find that the indirect effect of stratospheric ozone depletion could have offset up to approximately half of the predicted past increases in surface temperature that would otherwise have occurred as a result of the direct effect of halocarbons. However, as ozone will likely recover in the next few decades, a slightly faster rate of warming should be expected from the net effect of halocarbons, and we find that together halocarbons could bring forward next century’s expected warming by ~20 years if future emissions projections are realized. In both the troposphere and stratosphere CFC-12 contributes most to the past temperature changes and the emissions projection considered suggest that HFC-134a could contribute most of the warming over the coming century.     

Direct human influence of irrigation on atmospheric water vapour and climate

Human activity increases the atmospheric water vapour content in an indirect way through climate feedbacks. We conclude here that human activity also has a direct influence on the water vapour concentration through irrigation. In idealised simulations we estimate a global mean radiative forcing in the range of 0.03 to +0.1 Wm^–2 due to the increase in water vapour from irrigation. However, because the water cycle is embodied in the climate system, irrigation has a more complex influence on climate. We also simulate a change in the temperature vertical profile and a large surface cooling of up to 0.8 K over irrigated land areas. This is of opposite sign than expected from the radiative forcing alone, and this questions the applicability of the radiative forcing concept for such a climatic perturbation. Further, this study shows stronger links than previously recognised between climate change and freshwater scarcity which are environmental issues of paramount importance for the twenty first century.     

土地利用和土地覆盖变化对气候系统影响的研究进展

土地利用和土地覆盖变化（LUCC或LULCC）不仅对人类赖以生存的地球环境有重要影响,同时与人类福祉密切联系。人类活动对气候的强迫不仅包括温室气体排放导致的气候变暖,还通过直接改变地表物理性状以及间接改变其他生物地球物理过程和生物地球化学过程等对气候系统产生深刻影响。作者在此认识的基础上回顾了LUCC对气候系统影响的研究历史,结合新近的研究结果归纳了诸如森林砍伐、城市化、修坝等LUCC活动在区域和全球尺度的气候效应。LUCC具有高度的空间异质性,因此气候系统对它的反馈也具有明显的空间差异。由于全球平均后变化幅度相对区域上的小,LUCC对区域气候影响显著,而对全球气候影响不明显。它对区域气候的影响取决于反照率、蒸散发效率和地表粗糙率等变化的综合效应：在热带地区LUCC主要引起温度升高,在高纬度地区使温度下降。在全球尺度上LUCC导致气候的变暖主要通过减少蒸散发和潜热通量引起陆表水循环的改变,其次通过改变地表反照率导致辐射强迫改变。最后指出目前LUCC在气候变化学科中的研究所存在的问题。在此基础上提出了未来的研究首先需要评估的3个气候指标,并提倡多学科间的相互合作。     

Why Is the Climate Forcing of Sulfate Aerosols So Uncertain?

l. IntroductionAlthough the aerosol has been recognized as an important factor which has innuence onthe past, present and future climate for a long time, it still has much uncertainty in assessingits climate forcing. The direct radiative forcing of sulfate aerosols has been estimated rangingfrom --0.3 W/ m2 to --0.9 W/ m2 in recent publications (Charlson et al., l992, Kiehl andBriegleb l993; Taylor and Penner 1994, Boucher and Anderson l995, Kieh1 and Rodhe l995;Chuang et al., l997, Penne…     

Abatement of Greenhouse Gases: Does Location Matter?

Today's climate policy is based on the assumption that the location of emissions reductions has no impact on the overall climate effect. However, this may not be the case since reductions of greenhouse gases generally will lead to changes in emissions of short-lived gases and aerosols. Abatement measures may be primarily targeted at reducing CO₂, but may also simultaneously reduce emissions of NO_x, CO, CH₄ and SO₂ and aerosols. Emissions of these species may cause significant additional radiative forcing. We have used a global 3-D chemical transport model and a radiative transfer model to study the impact on climate in terms of radiative forcing for a realistic change in location of the emissions from large-scale sources. Based on an assumed 10% reduction in CO₂ emissions, reductions in the emissions of other species have been estimated. Climate impact for the SRES A1B scenario is compared to two reduction cases, with the main focus on a case with emission reductions between 2010 and 2030, but also a case with sustained emission reductions. The emission reductions are applied to four different regions (Europe, China, South Asia, and South America). In terms of integrated radiative forcing (over 100 yr), the total effect (including only the direct effect of aerosols) is always smaller than for CO₂ alone. Large variations between the regions are found (53–86% of the CO₂ effect). Inclusion of the indirect effects of sulphate aerosols reduces the net effect of measures towards zero. The global temperature responses, calculated with a simple energy balance model, show an initial additional warming of different magnitude between the regions followed by a more uniform reduction in the warming later. A major part of the regional differences can be attributed to differences related to aerosols, while ozone and changes in methane lifetime make relatively small contributions. Emission reductions in a different sector (e.g. transportation instead of large-scale sources) might change this conclusion since the NO_x to SO₂ ratio in the emissions is significantly higher for transportation than for large-scale sources. The total climate effect of abatement measures thus depends on (i) which gases and aerosols are affected by the measure, (ii) the lifetime of the measure implemented, (iii) time horizon over which the effects are considered, and (iv) the chemical, physical and meteorological conditions in the region. There are important policy implications of the results. Equal effects of a measure cannot be assumed if the measure is implemented in a different region and if several gases are affected. Thus, the design of emission reduction measures should be considered thoroughly before implementation.     

Warming of an elevated layer over Africa

This paper analyzes trends of temperatures over Africa and seeks to quantify the most significant processes. Observations of air temperature reveal significant warming trends in the 925–600 hPa layer over tropical west Africa and the east Atlantic. This is related to the influence of desert dust and biomass burning emissions on the atmospheric energy budget. We calculate a net radiative absorption of ～??20 W m^???2. The southern (northern) plume is rich in short-lived greenhouse gases (dust aerosols), and the atmospheric response, according to a simplified radiative transfer model, is a >3°C heating of the 2–4 km layer. The observed pattern of warming coincides with a mixture of dust, black carbon and short-lived greenhouse gases in space, time and height. Physical forcing provides a secondary source of regional warming, with sinking motions over the Sahel. The elevated warm layer stabilizes the lower atmosphere over and west of Africa, so drying trends may be anticipated.     

A probabilistic quantification of the anthropogenic component of twentieth century global warming

This paper examines in detail the statement in the 2007 IPCC Fourth Assessment Report that “Most of the observed increase in global average temperatures since the mid-twentieth century is very likely due to the observed increase in anthropogenic greenhouse gas concentrations”. We use a quantitative probabilistic analysis to evaluate this IPCC statement, and discuss the value of the statement in the policy context. For forcing by greenhouse gases (GHGs) only, we show that there is a greater than 90 % probability that the expected warming over 1950–2005 is larger than the total amount (not just “most”) of the observed warming. This is because, following current best estimates, negative aerosol forcing has substantially offset the GHG-induced warming. We also consider the expected warming from all anthropogenic forcings using the same probabilistic framework. This requires a re-assessment of the range of possible values for aerosol forcing. We provide evidence that the IPCC estimate for the upper bound of indirect aerosol forcing is almost certainly too high. Our results show that the expected warming due to all human influences since 1950 (including aerosol effects) is very similar to the observed warming. Including the effects of natural external forcing factors has a relatively small impact on our 1950–2005 results, but improves the correspondence between model and observations over 1900–2005. Over the longer period, however, externally forced changes are insufficient to explain the early twentieth century warming. We suggest that changes in the formation rate of North Atlantic Deep Water may have been a significant contributing factor.     

Simulation of the influence of solar radiation variations on the global climate with an ocean-atmosphere general circulation model

 Two simulations with a global coupled ocean-atmosphere circulation model have been carried out to study the potential impact of solar variability on climate. The Hoyt and Schatten estimate of solar variability from 1700 to 1992 has been used to force the model. Results indicate that the near-surface temperature simulated by the model is dominated by the long periodic solar fluctuations (Gleissberg cycle), with global mean temperatures varying by about 0.5 K. Further results indicate that solar variability and an increase in greenhouse gases both induce to a first approximation a comparable pattern of surface temperature change, i.e., an increase of the land-sea contrast. However, the solar-induced warming pattern in annual means and summer is more centered over the subtropics, compared to a more uniform warming associated with the increase in greenhouse gases. The observed temperature rise over the most recent 30 and 100 years is larger than the trend in the solar forcing simulation during the same period, indicating a strong likelihood that, if the model forcing and response is realistic, other factors have contributed to the observed warming. Since the pattern of the recent observed warming agrees better with the greenhouse warming pattern than with the solar variability response, it is likely that one of these factors is the increase of the atmospheric greenhouse gas concentration. Received: 14 October 1996 / Accepted: 9 May 1997