Spatial distribution mapping and radiological hazard assessment of groundwater and soil gas radon in Ekiti State,Southwest Nigeria

Groundwater constitutes the major source of utility water in Ekiti State with the majority of the population depending on groundwater for drinking and other household uses. Soil in the area is commonly used as a component of building materials, which may produce radon in the indoor environment. Excessive concentrations of radon in water and soil can cause radiological health risks to human as witnessed by the increased cases of lung cancer among non-smokers in Nigeria, which may be traceable to the ingestion and inhalation ²²²Rn in drinking water and indoor air. In the present study, comparative in situ measurements of radon in groundwater and soil gas were carried out at one hundred selected locations across the Ekiti State in southwest Nigeria, using a RAD7 radon detector to generate a radon distribution map and to estimate radiation hazards due to radon. The concentrations of radon in groundwater ranged from 0.9 to 472 Bq L^?1 with a mean of 34.7?±?4.4 Bq L^?1, while those of soil gas ranged from 0.1 to 315 kBq L^?1 with a mean of 38.9?±?1.4 kBq L^?1. The total annual effective dose due to inhalation and ingestion of radon in groundwater amounted to 94.7 µSv year^?1, which is lower than the reference dose of 100 µSv year^?1 recommended by the World Health Organization (WHO). The radon map generated for groundwater and soil gas identified three distinct areas with radon levels ranging from low to high. The results of this study show that some locations (Emure, Gbonyin, Ijero and Ikole) show mean total annual effective doses which are higher than the recommended limit. It can then be inferred that the groundwater samples pose significant radiological hazards to the population and that the noticed increase in lung cancer cases may be attributed to the consumption of groundwater in the area.     

Radon distributions in the Hail Region of Northern Saudi Arabia

Indoor radon measurements were carried out in a total of 420 dwellings and 17 schools in Hail region of Saudi Arabia, using NTDs based radon dosimeters. The duration of the measurements was one year, from April 2008 to April 2009. The indoor radon concentrations varied from 4 to 513 Bq/m³ with an overall average of 45 Bq/m³ for all surveyed dwellings. These passive measurements were confirmed by the active measurements. The anomalous concentrations above 200 Bq/m³ were observed in 13 dwellings, representing 3.1 % of the total surveyed dwellings. In Inbowan village alone, it was found that 7.6 % of the dwellings have indoor radon concentration above 200 Bq/m³. The highest average indoor radon concentration of 64 Bq/m³ was found in Inbowan village while the lowest average of 24 Bq/m³ was found in Majasah village. The city of Hail showed an average indoor radon concentration of 49 Bq/m³. The average indoor radon concentration in one area located at the edge of the Aja Mountain in Hail city was 111 Bq/m³. The elevated indoor radon concentrations in many dwellings in the Hail region, prompted us to measure outdoor ground radon in such locations using gas monitor. It was found that radon concentrations at a depth of 0.5 m varied significantly from place to place ranging from 1.2 to 177 kBq/m³. The outdoor radon concentrations are generally correlated with the indoor radon measurements. Radon exhalations from construction materials and soil samples from the Hail region were also measured. It was found that radon exhalations from soil samples are higher than that of construction materials by a factor of at least 3 and reaching up to 11. These results indicate that soil is the main source of indoor radon. Geological interpretations of the results are also given.     

Geochemistry and ground permeability as determinants of indoor radon concentrations in southernmost Sweden

A study of the indoor radon gas levels was performed in 935 homes in Scania, southernmost Sweden, located on geologically different ground with regard to uranium (U) content. In one of these two areas the bedrock consists of alum shale with U contents exceeding 200 ppm. In the other area there is no U-rich bedrock. Indoor radon levels are influenced by U content and permeability as shown below.For maam nancy for table, please place here. Thanx!The results show that the indoor radon levels were highest in homes located on bedrock with medium to high U content combined with a highly permeable drift covering the bedrock. The difference was statistically significant(P < 0.0001). Other results of the investigation are: 14 homes built from aerated concrete made from U-rich alum shale had higher levels than 767 homes with walls from other material (312 vs 106 Bq/m³;P = 0.0011); 242 homes with a cellar had lower radon levels than 563 without (62 vs 138 Bq/m³;P <0.0001); further, 418 homes with private well had higher levels than 360 with public water supply (140 vs 82 Bq/m³;P <0.0001). The results of the investigation show a profound effect of a combination of high bedrock U content and high cover permeability. The effect of the uraniferous drift on the indoor radon levels is evident. Thus, the geological conditions should be carefully considered when screening for high-risk buildings, as well as when planning for new ones. Also, the construction of the building and its water supply have some influence.     

Dependence of radon concentration in natural gas on the geological and physical parameters of the gas reservoir

Pressure of natural gas in its rock reservoir determines the final radon concentration in this gas after its decompression to normal conditions. In this investigation, radon contents of 62 natural gas samples were measured and a simple physical model of the gas reservoir was applied. The model takes into account an additional dependence of radon concentration on the natural gas pressure and on the porosity of the rock reservoir. The influence of the gas pressure on the value of the radon emanating power is discussed. The mean ²²⁶ Ra content in the source rock needed for generation of ²²² Rn concentrations observed in gas is also calculated. The calculations are made with the help of regression analysis.     

Geological and tectonic influence on water–soil–radon relationship in Mandi–Manali area,Himachal Himalaya

Radon measurements in soil and groundwater (springs, thermal springs and handpumps) were made in a variety of lithological units including major thrusts between Mandi and Manali in Himachal Himalaya. Analysis of radon data in light of lithological controls and influence of deep-seated thrusts has been made to elucidate the causative factors for anomalous emanation of radon. The lithological types include banded gneisses, schists, quartzite, granite, phyllites, volcanics and mylonites. The low-grade metasedimentries of Shali and Dharamsala generally show low and narrow range of radon concentration in water (5.6–13.4 Bq/l) as well as in soil (1.8–3.2 kBq/m³) except for the samples related to thrusts. On the other hand, sheared and deformed rocks of Chail and Jutogh show moderate radon content (average 5.03 kBq/m³, range 2.9–11.1 kBq/m³) in soil. However, the groundwater radon concentration shows wide variation in different types of sources (2.1–80.8 Bq/l). The quartzite and volcanic rocks of Rampur formation in this area present as a window separated by Chail thrust. Radon emanations on these rock types are relatively high (6.3–68.1 Bq/l in water and 5.5–15.9 kBq/m³ in soil) and are exceptionally high in samples that are related to uranium mineralization, deep-seated thrusts and hot springs (13.5–653.5 Bq/l). It is generally observed that anomalous high radon content is associated with mineralization, deeper source and tectonic discontinuities. Whereas it is obvious that subsurface radioactive mineralization would facilitate enhanced radon production, however, thrust plains provide easy pathways for escape of gases from the deeper sources. Shallow and deep sources of the groundwater have contrasting radon content particularly in the deformed and metamorphosed rocks of Jutogh and Chail. Shallow groundwater sources, mainly handpumps, have lower radon concentration due to limited superficial water circulation, whereas deeper sources, mainly perennial springs, show higher radon content because of larger opportunity for water–rock interaction.     

Determination of radon exhalation from granite, dolerite and marbles decorative stones of the Azad Kashmir area, Pakistan

Extensive export quality reserves of granite, dolerite and marbles which are used for interior decorations as wall facing, paving floors, kitchen counter tops, etc., are available in Azad Kashmir. Since these stones contain radium in trace amounts, therefore, its use as a building material may be a potential source of indoor radon. In order to assess health hazards due to the use of these stones as a building material, samples were collected from different mining sites. After processing, these samples were placed in plastic containers and box type radon detectors were installed in it at the height of 25 cm above the surface of the samples. The containers were then hermetically sealed. After 60 days of exposure to radon, CR-39 detectors were etched in 6 M NaOH at 70 °C for 9 h and measured track densities were related to radon concentration. Radon exhalation rate form the studied granites, marble and dolerite samples varied from 87 ± 26 to 353 ± 36 mBq m^?2h^?1, 79 ± 25 to 650 ± 42 mBq m^?2h^?1 and 90 ± 26 to 324 ± 36 mBq m^?2h^?1, respectively. These decorative stones are therefore used in buildings and for export purposes as the observed radon exhalation values are smaller than that of the EPA recommended-action level.     

Measurement of radon exhalation rate in various building materials and soil samples

Indoor radon is considered as one of the potential dangerous radioactive elements. Common building materials and soil are the major source of this radon gas in the indoor environment. In the present study, the measurement of radon exhalation rate in the soil and building material samples of Una and Hamirpur districts of Himachal Pradesh has been done with solid state alpha track detectors, LR-115 type-II plastic track detectors. The radon exhalation rate for the soil samples varies from 39.1 to 91.2 mBq kg^?1 h^?1 with a mean value 59.7 mBq kg^?1 h^?1. Also the radium concentration of the studied area is found and it varies from 30.6 to 51.9 Bq kg^?1 with a mean value 41.6 Bq kg^?1. The exhalation rate for the building material samples varies from 40.72 (sandstone) to 81.40 mBq kg^?1 h^?1 (granite) with a mean value of 59.94 mBq kg^?1 h^?1.     

Active and passive measurements of radon diffusion coefficient from building construction materials

The gaseous state and chemical inert behavior of radon make it important tracer for the radon transport study through the building materials. The radon resistant property of building construction materials is important parameter to control the indoor radon levels in living and workplaces. The materials with higher radium content can be made less severe by the use of some building materials of low diffusion coefficient and diffusion length. This makes the study of radon diffusion through building material more important along with the study of exhalation and radioactivity content. Keeping this in mind the radon diffusion study was carried out through different building construction materials used for wall and floor by active and passive techniques. The diffusion coefficient from these building materials measured by passive methods varied from (0.9 ± 0.5) × 10^?7 to (22.95 ± 13.19) × 10^?6 m²s^?1 and radon diffusion length varied from 0.21 to 3.31 m for cement, soil, sand, wall putty and plaster of Paris (POP) etc. The radon diffusion coefficient measured by active technique varied from 1.93 × 10^?10 to 1.36 × 10^?7 m²s^?1 for samples with definite geometry like paper, polyethylene, marble, granite etc. The radon diffusion coefficient and diffusion length depend upon the porosity and density of materials for powder samples.     

Measurement of soil-gas radon in some areas of northern Rajasthan,India

The health hazards of the radioactive gas radon on general public are well known. In order to understand the level and distribution of ²²²Rn concentrations in soil-gas in Sri Ganganagar district of Rajasthan, a ²²²Rn survey was carried out for the first time using RAD7, an electronic radon detector manufactured by Durridge Company (USA), at different locations covering a total area of 10,978 km ², having a population of approximately 20 lakh. The measurement of ²²²Rn concentration in soil-gas was carried out at four different depths (10, 40, 70, and 100 cm). The radon concentration in soil-gas for 10, 40, 70, and 100 cm depths ranged from 0.09–4.25, 0.15–6.30, 0.50–9.18, and 0.72–10.40 kBq m ^?3, respectively. The minimum value of radon concentration is observed in 33 GB village at 10 cm depth and maximum for Mohanpura village at 100 cm depth. As expected, our data show an increase of soil-gas radon concentration levels with depth. The present results are compared with the available radon data from other studies.     

Correlation of soil radon and uranium with indoor radon in the Albuquerque,New Mexico area

High indoor radon in approximately 30 percent of private dwellings in the Albuquerque, New Mexico area has been reported previously. The present study explains the areas of high indoor radon as a function of different soil and/or bedrock in the area. Soils were sampled during summer and winter periods using alpha track radon detectors. The values range from 40 to 890 pCi/I air at a depth of 38 cm. The gross mean average is 360 pCi/I for the area for summer readings and 200 pCi/I for winter readings; both values are well over the average U.S. soil radon values of approximately 100 pCi/I. Analyses of soil uranium show a range in values of 1–6 ppm, with a mean of 3.1 ppm. Thorium values range from 3.3 to 28.8 ppm, and Th/U ratios range from 2.9 to 4.6.These values for U, Th, and Th/U suggest that soil U and Th are close to the values reported for the Sandia granite, the source of most of the pediment on which Albuquerque is built. Soil infiltration rates range from ~6 × 10^–4 to 4.5 × 10^–3 cm/sec for the samples, and soil moisture content ranges from 1.4 to 7.2 percent. A fair correlation of summer soil radon with infiltration rate is noted. Correlation of soil radon with moisture content and/or with percent silt, silt + clay, clay size fraction material is not established by this study. Soil radon values do correlate with regions in the Albuquerque area where high indoor radon is common. A better correlation of high indoor radon values with soils developed immediately over bedrock is observed. Furthermore, all values of average soil and indoor radon increase significantly with proximity of the stations to the Sandia Mountains. Soil uranium also shows this trend. The data argue that regions of potentially high radon can thus be identified.     

Collection of radon decay products — a uranium exploration technique

The spontaneous deposition of short-lived radon decay products onto solid surfaces (“collectors”) provides the basis for a simple and efficient way of prospecting for uranium. The alpha activity of two of the decay products, ²¹⁸Po and ²¹⁴Po, can be measured by conventional counting techniques following the exposure of a collector to a radon source. Laboratory studies have shown: (a) radon decay products can be collected on a wide variety of materials; (b) the number of radon decay products increases with the collector surface area; (c) a negative charge applied to the collectors enhances the number of decay products collected; (d) the shape of the collectors is relatively unimportant; and (e) reproducibility is about ± 5% of the measured value.Field tests on known uranium anomalies involved suspending collectors for an overnight exposure, in either covered holes or inverted containers buried in soil. Subsequent removal of the collectors was immediately followed by counting the alpha activity. Anomalies were readily detected at three different test sites. Replicate measurements at selected sites both on an hour-to-hour and on a day-to-day basis showed remarkably good agreement. Some anomalies were also outlined using activity measurements from collectors suspended above soil aliquots in sealed containers.Because the half-lives of two of the thoron (²²⁰Rn) decay products are much longer than those of the radon (²²²Rn) decay products, a thoron correction can be applied to the original activity measured from the collectors, thus discriminating against thoron in thorium-rich terrains.The counting of radon decay products deposited onto collectors is an effective method for delineating radon anomalies in uranium exploration. The field techniques are simple to apply, and results are available after very short exposure times (about 18 hours) and after short counting intervals (5 minutes).     

Study of the radon concentrations in drinking water from three main cities of Shaanxi Province,China

This paper presents the results of radon concentration measurements in the drinking water from the municipal water supply system and private wells of Xian, Xianyang and Baoji city of Shaanxi province of China. The measurements were carried out on 38 samples. Radon levels in drinking water in Xian, Xianyang and Baoji were found to be 5.78, 13.04 and 15.01 k Bq m^–3, respectively. The AM radon concentration of private well water from Xianyang and Baoji is 28.84 k Bq m^–3 and 38.85 k Bq m^–3, respectively, which is 2.56 times and 3.14 times as high as that of tap water radon, respectively. The radiation risk of radon in water would be due to degassing and not due to drinking water. The domestic use of showers, humidifiers, and cooking, washing up, laundering, etc. may lead to an additional increase of the radon concentration in the indoor air. The observed radon concentration in drinking water from three main cities of Shaanxi Province can contribute to a 4.86 to 32.63% increase in indoor radon concentration and can cause 0.068±0.016 mSv y^–1 to 0.177±0.045 mSv y^–1 extra annual effective dose to males, 0.060±0.014 mSv y^–1 to 0.155±0.039 mSv y^–1 to females. The mean annual effective dose equivalents to males and females of Xianyang and Baoji from well water account for 25.94 to 39.75% of environmental radon and radon daughters annual effective dose equivalents. The radon concentrations in the well water from Xianyang and Baoji will bring a definite additional risk to the population.     

Study of radon in soil gas,trace elements and climatic parameters around South Kordofan state,Sudan

This study was conducted primarily to measure and map radon activity concentration in soil gas and to understand the effect of geology and lithology and meteorology on radon concentration. Portable radon meter has been used for the measurement of soil gas radon at 30 different locations around Uro and Korn area in eastern Nuba Mountain South Kordofan State. The results indicate that the activity concentrations of ²²²Rn in soil gas fall within the range of 20–1,359 Bq/m³ with geometric mean of 102.80 Bq/cm³. The obtained data show that samples around Uro have anomaly of ²²²Rn concentrations than the sample around Korn. The reason could be attributed to differences in the geological structure, lithology and climate parameters. GIS predicative map has shown that the elevated levels of radon concentration were measured in North study area. Upon comparing the results with global data, it was found that the obtained values are far below the reported range of India, Slovenia, Portugal and Syria. However, the range of ²²²Rn concentrations in the soil observed in this study is significantly high relative to similar data reported from Libya. The regression analysis has shown that no correlation was noted between radon concentrations, climatic parameters and trace element.     

Radioactive elements in natural gas: a case study on distribution of gaseous 222radon and its origin mechanism

As natural gas becomes increasingly important in our daily life, studies have been carried out on trace elements such as mercury and arsenic within it. Other than those, the existence of radioactive gaseous radon from the combustion of natural gas indoors can cause severe diseases and damages to body organs, putting a hazardous impact on human health. At the same time, the radon can also corrode gas production and transportation equipment. A review of the literature on radon concentrations in natural gas produced from gas reservoirs in China and other countries have been studied. Radon is a decay product from ²³⁸U, which is closely related to the accumulation and migration of organic matter during diagenesis. Gas recovered from reservoirs with higher than average natural ²³⁸U contains higher than average levels of ²²²Rn. Massive fault systems and fracture zones appear to play a significant role in radon concentrations in natural gas.     

Predicting New Hampshire indoor radon concentrations from geologic information and other covariates

 Generalized geologic province information and data on house construction were used to predict indoor radon concentrations in New Hampshire (NH). A mixed-effects regression model was used to predict the geometric mean (GM) short-term radon concentrations in 259 NH towns. Bayesian methods were used to avoid over-fitting and to minimize the effects of small sample variation within towns. Data from a random survey of short-term radon measurements, individual residence building characteristics, along with geologic unit information, and average surface radium concentration by town, were variables used in the model. Predicted town GM short-term indoor radon concentrations for detached houses with usable basements range from 34 Bq/m³ (1 pCi/l) to 558 Bq/m³ (15 pCi/l), with uncertainties of about 30%. A geologic province consisting of glacial deposits and marine sediments was associated with significantly elevated radon levels, after adjustment for radium concentration and building type. Validation and interpretation of results are discussed. Received: 20 October 1997 · Accepted: 18 May 1998     

Measurement of Radon Concentration in Drinking Water in Bhiwani District of Haryana

This investigation aims to evaluate the concentration of dissolved radon in drinking water and to assess the associated radiation doses for infants, children and adults in Bhiwani district of Haryana The radon concentrations were measured in 82 drinking water samples collected from 32 villages/towns in the Bhiwani district. The measurements were performed by RAD7, an electronic radon detector manufactured by Durridge Company Inc. The mean radon concentration ranged between 1.3 ± 0.4 and 13.4 ± 2.2 Bq l^-1. The mean radon concentrations from two locations exceeded the maximum contamination level (MCL) of 11 Bq l^-1 recommended by United States Environmental Protection Agency. The total annual effective doses due to ingestion and inhalation of radon in drinking water varied from 10.1 to 104.4 μSv y^-1 for infants, 5.8 to 59.6 μSv y^-1 for children and 6.6 to 67.7 μSv y^-1 for adults and the average values were found to be 46.3, 26.5 and 30.1 μSv y^-1, respectively.     

Natural Radon and Radium Isotopes for Assessing Groundwater Discharge into Little Lagoon,AL: Implications for Harmful Algal Blooms

Naturally occurring isotopes of radon (²²²Rn) and radium isotopes (^{223,224,226,228}Ra) were used as tracers to assess submarine groundwater discharge (SGD) into Little Lagoon, AL (USA), a site of recurring harmful algal blooms (HABs). The radium isotopic data suggests that there are two groundwater sources of these tracers to the lagoon, a shallow (A1) and deeper (A2) aquifer. We estimated the fraction of each source via a three-end-member mixing model consisting of Gulf of Mexico seawater, shallow and deep groundwater. The estimated lagoonwide SGD rates based on a radium mass balance and the mixing model were 1.22?±?0.53 and 1.59?±?0.20 m³ s^-1 for the shallow and deep groundwater discharges, respectively. To investigate temporal variations in SGD, we performed several radon surveys from 2010 through 2012, a period of generally declining groundwater levels due to a drought in the southeastern USA. The total SGD rates based on a radon mass balance approach were found to vary from 0.60 to 2.87 m³ s^-1. We observed well-defined relationships between nutrients and chlorophyll-a in lagoon waters during a period when there was an intense diatom bloom in April 2010 and when no bloom existed in March 2011. A good correlation was also found between radium (groundwater-derived) and nutrients during the April 2010 period, while there was no clear relationship between the same parameters in March 2011. Based on multivariate analysis of chemical and environmental factors, we suggest that nutrient-rich inputs during high SGD may be a significant driver of algal blooms, but during low SGD periods, multiple drivers are responsible for the occurrence of algal blooms.     

Radon,Lung Cancer Risk and Environmental Geology in Gejiu Area

The incidence of lung cancer in the Gejiu area of Yunnan Province ranks the first in the world.The radon level(indoor,soil) was measured in the Gejiu area by the SSNTD method from 1990 to 1996,The result indicates an extensive high-level of indoor radon in that area though U and Th are lower in local limestones,The indoor radon level of houses located in the geologic fault zone is 6 times high that 2km far from the fault zone.The reason probably is that the radon level of soil in the fault is 6-8 times high that 1 km far from the faults.our data indicate that a lower range of radon levels,0-100Bq.m^-3,exists in healthy families.However,a higher radon level,over 800 Bq.m^-3,is often found corresponding to that of cancer patients‘ homes(the house-owners are suffering from either lung cancer or leukaemia or liver cancer),Obviously,an increase in lung cancer incidence follows an increase in indoor radon level,The risk of cancer induced by indoor radon is no longer an inference,but a fact.     

Soil-gas radon anomalies in three study areas of Central-Northern Calabria (Southern Italy)

Soil-gas radon concentrations and exhalation rates have generally been observed to be anomalously high along active faults in many parts of the world. The soil-gas method is based on the principle that faults and fractures in rocks are highly permeable pathways along which gases can migrate upward from deep crust and mantle to soil cover, retaining their source signatures. The present study summarizes the influence of fault zones on anomalous radon concentrations in soil by integrated geophysical and geo-structural analyses in three study areas of Central-Northern Calabria (Southern Italy). Soil-gas radon surveys have been carried out by means of an alpha scintillation counting system, at 12,509 locations between 2002 and 2004. A geostatistical approach has been used to estimate the spatial distribution of soil radon concentrations. Relations among soil-gas distribution and geo-structural features have been evaluated by ordinary multi-Gaussian kriging. Highest soil radon concentrations (ca. 90 kBq m^?3) have been measured in the Rossanese sector. In the three study areas, no appreciable differences can be noticed among lithotypes, with the highest concentration values (ca. 89 kBq m^?3) measured in alluvial deposit and in clay. Measurements of soil-gas radon reveal anomalies clearly connected to the tectonic structures. Increased signals are linearly distributed along regional WNW–ESE trending shear zones, with main pathways of concentration also recognizable along the E–W fault system in the Rossanese sector, the N–S fault system in the Crati Graben and the Catanzaro Trough, and the NE–SW fault system in the Catanzaro Trough. The distribution of epicentres of historical earthquakes occurred between 1184 and 2001 confirms the recent activity of the same fault systems. Soil-gas radon concentrations generally increase, as expected, with decreasing distance to the faults.