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1.
Radon is a radioactive hazardous and ubiquitous gas. It has been recognized to be one of the major contributors to natural radiation even causing lung cancer if present at enhanced levels. There are large variations in data available in the literature for radium content and radon exhalation rates of various materials. It is a well-documented fact that radon exhalation from the ground surface depends upon a number of parameters such as soil grain size, soil porosity and radium content. For this purpose, in this study the so-called can technique has been used to measure radium content and exhalation rates of radon in soil samples collected from different places of Aligarh, Etah and Mathura districts of Uttar Pradesh??a province in northern India. These districts lie within the subtropical region of the Indo-Gangetic plains. The values of effective radium content are found to vary from 8.11 to 112.83?Bq?kg?1 with a mean value of 33.21?Bq?kg?1 and a standard deviation of 28.15. The values of mass exhalation rates of radon vary from 0.76?×?10?6 to 15.80?×?10?6?Bq?kg?1?day?1 with a mean value of 4.21?×?10?6?Bq?kg?1?day?1, while the surface exhalation rates vary from 1.97?×?10?5 to 41.03?×?10?5?Bq?m?2?day?1 with a mean value of 10.93?×?10?5?Bq?m?2?day?1.  相似文献   

2.
Extensive export quality reserves of granite, dolerite and marbles which are used for interior decorations as wall facing, paving floors, kitchen counter tops, etc., are available in Azad Kashmir. Since these stones contain radium in trace amounts, therefore, its use as a building material may be a potential source of indoor radon. In order to assess health hazards due to the use of these stones as a building material, samples were collected from different mining sites. After processing, these samples were placed in plastic containers and box type radon detectors were installed in it at the height of 25 cm above the surface of the samples. The containers were then hermetically sealed. After 60 days of exposure to radon, CR-39 detectors were etched in 6 M NaOH at 70 °C for 9 h and measured track densities were related to radon concentration. Radon exhalation rate form the studied granites, marble and dolerite samples varied from 87 ± 26 to 353 ± 36 mBq m?2h?1, 79 ± 25 to 650 ± 42 mBq m?2h?1 and 90 ± 26 to 324 ± 36 mBq m?2h?1, respectively. These decorative stones are therefore used in buildings and for export purposes as the observed radon exhalation values are smaller than that of the EPA recommended-action level.  相似文献   

3.
Groundwater constitutes the major source of utility water in Ekiti State with the majority of the population depending on groundwater for drinking and other household uses. Soil in the area is commonly used as a component of building materials, which may produce radon in the indoor environment. Excessive concentrations of radon in water and soil can cause radiological health risks to human as witnessed by the increased cases of lung cancer among non-smokers in Nigeria, which may be traceable to the ingestion and inhalation 222Rn in drinking water and indoor air. In the present study, comparative in situ measurements of radon in groundwater and soil gas were carried out at one hundred selected locations across the Ekiti State in southwest Nigeria, using a RAD7 radon detector to generate a radon distribution map and to estimate radiation hazards due to radon. The concentrations of radon in groundwater ranged from 0.9 to 472 Bq L?1 with a mean of 34.7?±?4.4 Bq L?1, while those of soil gas ranged from 0.1 to 315 kBq L?1 with a mean of 38.9?±?1.4 kBq L?1. The total annual effective dose due to inhalation and ingestion of radon in groundwater amounted to 94.7 µSv year?1, which is lower than the reference dose of 100 µSv year?1 recommended by the World Health Organization (WHO). The radon map generated for groundwater and soil gas identified three distinct areas with radon levels ranging from low to high. The results of this study show that some locations (Emure, Gbonyin, Ijero and Ikole) show mean total annual effective doses which are higher than the recommended limit. It can then be inferred that the groundwater samples pose significant radiological hazards to the population and that the noticed increase in lung cancer cases may be attributed to the consumption of groundwater in the area.  相似文献   

4.
Due to the widespread use of granites as building and ornamental materials, measurements of natural radioactivity for a total 27 selected samples of commercial granites used in Egypt were carried out by using a high pure germanium detector. The activity concentrations of 226Ra, 232Th and 40K of commercial granites ranged from 25 to 356, 5 to 161, and 100 to 1,796?(Bq?kg?1), respectively. The concentrations of these radionuclides are compared with the international recommended values. To evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity, the absorbed dose rate, the effective dose rate, and the hazard index have been calculated. The radium equivalent activity Raeq varied from 41 to 669?(Bq?kg?1) which exceeds the permitted value (370?Bq?kg?1) and the internal hazard index H in varied from 0.2 to 2.8 which is higher than 1. The absorbed dose rate due to the natural radioactivity in the samples under investigation ranged from 19 to 310?(nGy?h?1). The total effective dose rates per person indoors were determined to be 0.09 to 1.5?(mSv?year?1).  相似文献   

5.
为解决大面积多点快速土壤氡析出率测量问题, 设计开发并进行了土壤氡析出率活性炭累积吸附法的方法技术研究.在参考氡析出率装置和野外实验数据的基础上, 进行了测量装置及材料的选择、装置刻度、野外累积暴露时间、活性炭盒吸附氡有效衰变常数等研究.通过2002-2003年22次重复观测, 北京西北郊区粘土类土壤氡析出率平均值为20.15mBq.m-2.s-1, 最大值和最小值分别为26.75和13.49mBq.m-2.s-1, 标准偏差为3.55mBq.m-2.s-1.与仪器静电收集法比对结果表明, 两种方法的相对误差小于±10%.实验结果表明: 活性炭方法测量结果稳定可靠, 简便易行, 适用于全国大面积土壤氡析出率调查.   相似文献   

6.
对长约70 km引水工程洞线上进行的地面伽马能谱测量、陆地伽马剂量率测量、土壤氡浓度测量、岩石表面氡析出率测量以及钻孔岩芯样品的放射性元素U、Ra、Th、K含量分析的综合放射性地质调查,并对获得的测量数据进行分析研究。结果表明,测区引水沿线地质体放射性核素当量含量平均值为:U 1.56×10-6,Th 14.12×10-6,K 2.16×10-2;钻孔岩芯放射性元素分析含量平均值为:U 32.34 Bq/kg,Ra 35.68 Bq/kg,Th 35.29 Bq/kg,K 865.65 Bq/kg。陆地伽马剂量率为90.42 nGy/h;土壤氡浓度平均值为4 272.1 Bq/m3;岩石表面析出率平均值为4.01×10-2 Bq/m2·s。根据测量结果,利用内照射和外照射辐射剂量计算了对施工人员造成的辐照剂量为0.759 mSv,低于国家对公众的剂量限值1 mSv/a,表明引水工程输水隧洞的施工在安全辐射范围内。  相似文献   

7.
The gaseous state and chemical inert behavior of radon make it important tracer for the radon transport study through the building materials. The radon resistant property of building construction materials is important parameter to control the indoor radon levels in living and workplaces. The materials with higher radium content can be made less severe by the use of some building materials of low diffusion coefficient and diffusion length. This makes the study of radon diffusion through building material more important along with the study of exhalation and radioactivity content. Keeping this in mind the radon diffusion study was carried out through different building construction materials used for wall and floor by active and passive techniques. The diffusion coefficient from these building materials measured by passive methods varied from (0.9 ± 0.5) × 10?7 to (22.95 ± 13.19) × 10?6 m2s?1 and radon diffusion length varied from 0.21 to 3.31 m for cement, soil, sand, wall putty and plaster of Paris (POP) etc. The radon diffusion coefficient measured by active technique varied from 1.93 × 10?10 to 1.36 × 10?7 m2s?1 for samples with definite geometry like paper, polyethylene, marble, granite etc. The radon diffusion coefficient and diffusion length depend upon the porosity and density of materials for powder samples.  相似文献   

8.
Some of the rocks and soil-originated materials used in building construction are the serious natural radiation sources. Soil-originated bricks and roof-tiles and their raw material in the Salihli-Turgutlu area were tested in situ for natural radiation levels using a gamma-ray spectrometer. The concentrations of the radioelements 40K, 238U and 232Th and air-absorbed radiation rates were measured for soil, raw material heaps, brick and roof-tile stacks and waste brick heaps. The radium-equivalent activity Raeq of the raw material varied between 187.9 and 216.4 Bq kg?1. The external radiation hazard index Hex values ranged between 0.51 and 0.58. For building material and its products, recommended Raeq and Hex levels are 370 Bq kg-1 and 1.0, respectively. On the other hand, both Raeq and Hex values for waste brick heaps, containing broken brick pieces, coal pieces and ash, were higher than the recommended levels, i.e. Raeq values varied from 473.8 to 651.0 Bq kg-1 and Hex values were within the range 1.15–1.76. The annual dose rate and radium-equivalent activity values of the brick and roof-tiles were below the level of criteria. Annual dose rate ranged between 0.42 and 0.62 mSv y?1 and radium equivalent activity was in the range 172.9–245.2 Bq kg?1. The external and internal radiation hazard indices were all below the value of 1.0 for the Salihli-Turgutlu area bricks and roof-tiles. Results of this study were compared with results of previous studies. Natural radiation levels of construction raw material of study area are generally higher than of those of previous studies.  相似文献   

9.
The activity concentrations and the gamma-absorbed dose rates of the primordial naturally occurring radionuclides 226Ra, 232Th and 40K were determined for sand samples collected from the Baoji Weihe Sands Park, China, using γ-ray spectrometry. The natural radioactivity concentration of sand ranges from 10.2 to 38.3 Bq kg−1 for 226Ra, 27.0 to 48.8 Bq kg−1 for 232Th and 635.8 to 1,126.7 Bq kg−1 for 40K with mean values of 22.1, 39.0 and 859.1 Bq kg−1, respectively. The concentrations of these radionuclides are compared with the typical world values and the average activity of Chinese soil. The measured activity concentration of 226Ra and 232Th in sand is lower than the world average while that of 40K is higher. . To evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity, the external hazard index, the absorbed dose rate, and the effective dose rate have been calculated and compared with internationally approved values. The radium equivalent activity values of all sand samples are lower than the limit of 370 Bq kg−1. The values of the external hazard index are less than unity. The mean outdoor air absorbed dose rate is 69.6 nGy h−1 and the corresponding outdoor effective dose rate is 0.085 mSv y−1.  相似文献   

10.
Tailings resulted from sulphuric acid leaching process of uranium from sedimentary rocks contain high concentrations of 226Ra and its daughters, the most important of which is 222Rn. Movement of radon gas out of the tailings is strongly influenced by the physicochemical characteristics of these tailings especially their radium content and the grain size. So, the tailing samples were size fractionated into four sizes (>?250, 250–125, 125–74 and <?74 µm). The natural radioactivity was investigated using hyper-pure germanium detector and solid-state nuclear track detectors (CR-39) for bulk size and after size fractionation. The activity concentrations of different radionuclides in size-fractionated tailing samples have been shown to be strongly dependent on the size of the particles. In the range of >?250 and <?74 µm, the activity concentrations of 230Th, 226Ra, 214Pb, 214Bi, 210Pb, 232Th and 40K increased throughout with decreasing particle size, while that of 238U, 234U and 235U have an opposite effect. The results revealed an inverse relationship between the radon exhalation rate and size fractionation. Also, the results showed a good correlation between radium activity concentration and radon mass exhalation rate.  相似文献   

11.
Natural radioactivity in sediment of Wei River,China   总被引:1,自引:0,他引:1  
The concentrations of natural radionuclides in sediment of Wei River of China were measured using γ-ray spectrometry with the aim of estimating the radiation hazard as establishing a database for radioactivity levels of river sediment of China. The activity concentrations of 226Ra, 232Th and 40K in sediment samples ranged from 10.4 to 39.9 Bq kg−1, 15.3 to 54.8 Bq kg−1 and 514.8 to 1,175.5 Bq kg−1, respectively. The concentrations of these radionuclides were compared with the typical world values and the average activities of Chinese soil and Shaanxi soil. Radium equivalent activity (Raeq), external hazard index (H ex) and representative level index (I γr) were calculated for the samples to assess the radiation hazards arising due to the use of these sediment samples in the construction of dwellings. All the sediment samples have Raeq lower than the limit of 370 Bq kg−1, H ex less than unity and I γr close to 1 Bq kg−1. The overall mean outdoor terrestrial gamma dose rate is 64.8 nGy h−1 and the corresponding outdoor annual effective dose is 0.079 mSv. None of the studied location is considered a radiological risk and sediment can be safely used in construction.  相似文献   

12.
Soil gas radon measurements were made in Chamba and Dharamshala regions of Himachal Pradesh, India, to study the correlation, if any, between the soil gas radon, radium activity concentration of soil, and the geology/active tectonics of the study region. Soil gas radon surveys were conducted around the local fault zones to check their tectonic activities using the soil gas technique. Soil gas radon activity concentration at thirty-five different locations in Dharamshala region has been found to be varying from 13.2 ± 1.5 to 110.8 ± 5.0 kBq m?3 with a geometrical mean of 35.9 kBq m?3 and geometrical standard deviation of 1.8. Radon activity concentration observed in the thirty-seven soil gas samples collected from the Chamba region of Himachal Pradesh varies from 5.2 ± 1.0 to 35.6 ± 2.5 kBq m?3, with geometrical mean of 15.8 kBq m?3 and geometrical standard deviation of 1.6. Average radium activity concentrations in thirty-four soil samples collected from different geological formations of Dharamshala region and Chamba region are found to be 40.4 ± 17 and 38.6 ± 1.7 Bq kg?1, respectively. It has been observed that soil gas radon activity concentration has a wide range of variation in both Dharamshala and Chamba regions, while radium activity concentrations in soil samples are more or less same in both the regions. Moreover, soil gas radon activity concentration has a better positive correlation with the radium activity concentration in soil samples collected from Chamba region as compared to Dharamshala region.  相似文献   

13.
Indoor radon measurements were carried out in a total of 420 dwellings and 17 schools in Hail region of Saudi Arabia, using NTDs based radon dosimeters. The duration of the measurements was one year, from April 2008 to April 2009. The indoor radon concentrations varied from 4 to 513 Bq/m3 with an overall average of 45 Bq/m3 for all surveyed dwellings. These passive measurements were confirmed by the active measurements. The anomalous concentrations above 200 Bq/m3 were observed in 13 dwellings, representing 3.1 % of the total surveyed dwellings. In Inbowan village alone, it was found that 7.6 % of the dwellings have indoor radon concentration above 200 Bq/m3. The highest average indoor radon concentration of 64 Bq/m3 was found in Inbowan village while the lowest average of 24 Bq/m3 was found in Majasah village. The city of Hail showed an average indoor radon concentration of 49 Bq/m3. The average indoor radon concentration in one area located at the edge of the Aja Mountain in Hail city was 111 Bq/m3. The elevated indoor radon concentrations in many dwellings in the Hail region, prompted us to measure outdoor ground radon in such locations using gas monitor. It was found that radon concentrations at a depth of 0.5 m varied significantly from place to place ranging from 1.2 to 177 kBq/m3. The outdoor radon concentrations are generally correlated with the indoor radon measurements. Radon exhalations from construction materials and soil samples from the Hail region were also measured. It was found that radon exhalations from soil samples are higher than that of construction materials by a factor of at least 3 and reaching up to 11. These results indicate that soil is the main source of indoor radon. Geological interpretations of the results are also given.  相似文献   

14.
In this study, the environmental radioactivity measurements for Tokat and Sivas provinces in the northeast of Turkey were performed. Using gamma ray spectrometry, the activity concentrations of natural radionuclides in soil and travertine samples (232Th, 226Ra, and 40K) were determined. The annual effective dose equivalent, the absorbed doses rate in air, the radium equivalent, and the external hazard index were obtained from these activities. The activity concentrations vary from 9.09 to 17.04 Bq kg?1 for 232Th, from 36.53 to 76.95 Bq kg?1 for 226Ra, and from 216.56 to 576.59 Bq kg?1 for 40K in soil samples. The activity concentrations in travertines vary from 15.99 to 21.01 Bq kg?1 for 232Th, from 19.89 to 67.71 Bq kg?1 for 226Ra, and from 179.89 to 314.43 Bq kg?1 for 40K. The average dose rate in air for soil and travertine samples was 43.41 and 41.05 nGy h?1 respectively. The obtained results are presented and compared with other studies, and the results of this study are lower than the international recommended value (55 nGy h?1) given by UNSCEAR ( 2000). The results show that the region has a background radiation level within the natural limits.  相似文献   

15.
The activity concentration and the gamma-absorbed dose rates of the terrestrial naturally occurring radionuclides (232Th, 226Ra and 40K) were determined in soil samples collected from ten different locations of Sirsa district of Haryana, using HPGe detector based on high-resolution gamma spectrometry system. The range of activity concentrations of 226Ra, 232Th and 40K in the soil samples from the studied areas varies from 19.18 Bq kg−1 (Moriwala) to 40.31 Bq kg−1 (Rori), 59.43 Bq kg−1 (Pipli) to 89.54 Bq kg−1 (Fatehpur) and 223.22 Bq kg−1 (Moriwala) to 313.32 Bq kg−1 (SamatKhera) with overall mean values of 27.94, 72.75 and 286.73 Bq kg−1 respectively. The absorbed dose rate calculated from activity concentration of 226Ra, 232Th and 40K ranges between 8.84 and 18.58, 37.02 and 55.78, and 9.24 and 12.97 nGy h−1, respectively. The total absorbed dose in the study area ranges from 60.40 to 82.15 nGy h−1 with an average value of 70.12 nGy h−1. The calculated values of external hazard index (H ex) for the soil samples of the study area range from 0.36 to 0.49 with an average value of 0.42.  相似文献   

16.
The recommended concentrations of 239Pu, 240Pu and 239+240Pu in reference material IAEA‐315 (marine sediment) were estimated by three analytical methods: isotope dilution thermal ionisation mass spectrometry (TIMS), isotope dilution inductively coupled plasma‐mass spectrometry (ICP‐MS) and alpha spectrometry. The determination of 239Pu and 240Pu (239+240Pu by alpha spectrometry) was carried out with samples from randomly selected bottles using each method. Plutonium‐238 was also measured by alpha spectrometry. A plutonium‐242 reference material was used as a spike for the quantitative analysis. The influence of 242Pu in the samples was therefore calculated; however, this contribution was less than the range of uncertainty and did not influence the final results. The obtained data were statistically analysed using variance component analysis and paired comparison. The combined standard uncertainties from “method/measurement”, “bottle” and “sub‐sample” were in the order of 3 to 6%. The main contributions to the uncertainty were from the material heterogeneity and from systematic differences between methods. Based on this study with twenty‐seven analyses using 10–14 g sample mass, concentrations of (38 ± 3) Bq kg?1, (28 ± 3) Bq kg?1 and (66 ± 4) Bq kg?1 are proposed as recommended values for 239Pu, 240Pu and 239+240Pu, respectively, and (9.5 ± 0.4) Bq kg?1 for 238Pu as an information value in reference material IAEA‐315. In mass concentration units, these amount to (16.4 ± 1.2) ng kg?1, (3.3 ± 0.4) ng kg?1 and (0.015 ± 0.003) ng kg?1 for 239Pu, 240Pu and 238Pu, respectively. The certified reference materials NIST 4350B and NIST 4354 were also analysed by TIMS for quality assurance of the method used in this study.  相似文献   

17.
Gamma activity from the naturally occurring radionuclides namely, 226Ra, 232Th, the primordial radionuclide 40K was measured in the soil of Cuihua Mountain National Geological Park, China using γ-ray spectrometry technique. The mean activity of 226Ra, 232Th and 40K were found to be 27.2 ± 6.5, 43.9 ± 6.2 and 653.1 ± 127.6 Bq kg−1, respectively. The concentrations of these radionuclides were compared with the typical world values and the average activities of Chinese soil. The radium equivalent activity, the air absorbed dose rate, the annual effective dose rate, and the external hazard index were evaluated and compared with the internationally approved values. All the soil samples have Raeq lower than the limit of 370 Bq kg−1 and H ex less than unity. The overall mean outdoor terrestrial gamma dose rate is 66.3 nGy h−1 and the corresponding outdoor annual effective dose is 0.081 mSv.  相似文献   

18.
A study of natural radionuclides and radon concentration of Hamirpur District of Himachal Pradesh, India is carried out using various methodologies. The activity concentration of the natural radionuclides viz. 226Ra, 232Th and 40K is measured using high-resolution-based HPGe detector. Indoor radon measurements in the dwellings of Hamirpur district is carried out using LR-115 type II cellulose nitrate films in the bare mode. The average activity concentrations of 226Ra, 232Th and 40K are 35.58, 54.95 and 580.58 Bq kg?1, respectively. The annual average indoor radon value in the study area varies from 173.90 to 198.25 Bq m?3, which is well within the recommended action level given by International Commission on Radiological Protection. The indoor radon values obtained in the present investigation are higher than the world average of 40 Bq m?3. Radon concentration in water samples is measured using RAD7, an active radon detector. The annual effective dose for stomach and lung is determined from the measured value of radon concentration in water. To assess the radiation hazard of the natural radioactivity in all samples to the people, the radium equivalent activity, external hazard index, lifetime fatality risk, absorbed dose rate and total annual effective dose is estimated. The results signify that the studied area does not possess any radiation hazards due to the presence of natural radioactivity concentration.  相似文献   

19.
This study was conducted primarily to measure and map radon activity concentration in soil gas and to understand the effect of geology and lithology and meteorology on radon concentration. Portable radon meter has been used for the measurement of soil gas radon at 30 different locations around Uro and Korn area in eastern Nuba Mountain South Kordofan State. The results indicate that the activity concentrations of 222Rn in soil gas fall within the range of 20–1,359 Bq/m3 with geometric mean of 102.80 Bq/cm3. The obtained data show that samples around Uro have anomaly of 222Rn concentrations than the sample around Korn. The reason could be attributed to differences in the geological structure, lithology and climate parameters. GIS predicative map has shown that the elevated levels of radon concentration were measured in North study area. Upon comparing the results with global data, it was found that the obtained values are far below the reported range of India, Slovenia, Portugal and Syria. However, the range of 222Rn concentrations in the soil observed in this study is significantly high relative to similar data reported from Libya. The regression analysis has shown that no correlation was noted between radon concentrations, climatic parameters and trace element.  相似文献   

20.
High indoor radon in approximately 30 percent of private dwellings in the Albuquerque, New Mexico area has been reported previously. The present study explains the areas of high indoor radon as a function of different soil and/or bedrock in the area. Soils were sampled during summer and winter periods using alpha track radon detectors. The values range from 40 to 890 pCi/I air at a depth of 38 cm. The gross mean average is 360 pCi/I for the area for summer readings and 200 pCi/I for winter readings; both values are well over the average U.S. soil radon values of approximately 100 pCi/I. Analyses of soil uranium show a range in values of 1–6 ppm, with a mean of 3.1 ppm. Thorium values range from 3.3 to 28.8 ppm, and Th/U ratios range from 2.9 to 4.6.These values for U, Th, and Th/U suggest that soil U and Th are close to the values reported for the Sandia granite, the source of most of the pediment on which Albuquerque is built. Soil infiltration rates range from ~6 × 10–4 to 4.5 × 10–3 cm/sec for the samples, and soil moisture content ranges from 1.4 to 7.2 percent. A fair correlation of summer soil radon with infiltration rate is noted. Correlation of soil radon with moisture content and/or with percent silt, silt + clay, clay size fraction material is not established by this study. Soil radon values do correlate with regions in the Albuquerque area where high indoor radon is common. A better correlation of high indoor radon values with soils developed immediately over bedrock is observed. Furthermore, all values of average soil and indoor radon increase significantly with proximity of the stations to the Sandia Mountains. Soil uranium also shows this trend. The data argue that regions of potentially high radon can thus be identified.  相似文献   

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