Indoor radon probability calculated from the Czech soil gas radon data in a grid net for the European Geogenic Radon Map construction: test of feasibility

The construction of the European Geogenic Radon Map in a proposed grid system 10 × 10 km requires the data test to derive the probability of exceeding the indoor action level 200 Bq m⁻³ from the geologically based data. The Czech Republic disposes both indoor and soil gas data sets to test the real probability to exceed 200 Bq m⁻³ from indoor radon measurements and to compare it with the probability calculated from soil gas radon concentrations. Comparison of real and calculated probability enables to delineate the areas, where under- or overestimation can be expected. The results of data processing show minor differences between processing the raw data in generalised polygons of geological units and in a grid net, when using the generalised geological characteristics of grid cells.     

Assessment of radiation hazards due to the concentration of natural radionuclides in the environment

A study of natural radionuclides and radon concentration of Hamirpur District of Himachal Pradesh, India is carried out using various methodologies. The activity concentration of the natural radionuclides viz. ²²⁶Ra, ²³²Th and ⁴⁰K is measured using high-resolution-based HPGe detector. Indoor radon measurements in the dwellings of Hamirpur district is carried out using LR-115 type II cellulose nitrate films in the bare mode. The average activity concentrations of ²²⁶Ra, ²³²Th and ⁴⁰K are 35.58, 54.95 and 580.58 Bq kg^?1, respectively. The annual average indoor radon value in the study area varies from 173.90 to 198.25 Bq m^?3, which is well within the recommended action level given by International Commission on Radiological Protection. The indoor radon values obtained in the present investigation are higher than the world average of 40 Bq m^?3. Radon concentration in water samples is measured using RAD7, an active radon detector. The annual effective dose for stomach and lung is determined from the measured value of radon concentration in water. To assess the radiation hazard of the natural radioactivity in all samples to the people, the radium equivalent activity, external hazard index, lifetime fatality risk, absorbed dose rate and total annual effective dose is estimated. The results signify that the studied area does not possess any radiation hazards due to the presence of natural radioactivity concentration.     

The study of indoor radon in the urban dwellings using plastic track detectors

Radon and its progeny have been recognized as one of the major contributors to the natural radiation and health hazards in the human dwellings. Even lung cancer is expected if it is present in enhanced levels beyond maximum permissible limit. This paper reports the measurements of indoor radon and its progeny in the urban dwellings of the Etah district of Uttar Pradesh province in Northern India using the cellulose nitrate (LR-115 type-II) plastic track detectors. It is found that the values of radon concentration vary from 3.52 to 248.64 Bq m⁻³ with a standard deviation of 69.19. The values of radon progeny concentration vary from 0.38 to 26.88 mWL with a standard deviation of 7.48. The effective dose has been calculated and found to vary from 0.05 to 3.76 mSv year⁻¹ with a standard deviation of 1.05. The lifetime fatality risk is found to vary from 0.04 × 10⁻⁴ to 2.90 × 10⁻⁴. The results have been compared with the results reported in the rural areas of the same district.     

Measurements of indoor radon, thoron, and their progeny using twin cup dosimeters in rural areas of Northern India

Radon, thoron, and their progeny are largest contributors to the radiation dose received by human beings present in the natural environment. The indoor radon depends upon many factors such as building materials, meteorology, ventilation, and occupant’s behavior. This paper presents the measurements of indoor radon, thoron, and their progeny in four villages in rural area of district Kanshiram Nagar (Kasganj) in the state of Uttar Pradesh in Northern India. The concentration of indoor radon and thoron varies from 10.32 to 72.24 and 11.61 to 84.49 Bq m^?3 with a geometric mean (GM) of 29.49 and 31.20 Bq m^?3, respectively. The concentration of radon and thoron daughters was found to vary from 1.11 to 7.80 and 0.31 to 2.28 mWL, respectively. The annual exposure due to radon and thoron mainly vary from 0.05 to 0.30 WLM. The preliminary results (i.e., bare mode exposure of the LR-115 detectors fixed on cards) of this study have been separately published and compared this recent data with those results.     

Distribution of indoor radon concentrations and uranium-bearing rocks in Texas

 The purpose of this study was to compare regional patterns of indoor radon concentration with uranium-bearing rock zones and county populations in Texas. Zones yielding radon concentrations that are relatively high for Texas include shale and sandstone in northwest Texas; red beds in north-central Texas; felsic volcanic rocks in west Texas; and sandstone, limestone, and igneous rocks in central Texas. Located in northwest Texas, only five of the 202 counties evaluated have mean indoor radon concentrations above 4.0 pCi l^–1. Two of those counties have populations above the state median of 20 115. The highest county mean concentration is 8.8 pCi l^–1. Results of this study suggest that (1) regional geology influences indoor radon concentrations in Texas, (2) statewide, the radon concentrations are relatively low, (3) highly populated counties do not coincide with regions of high indoor radon concentration, and (4) regions that may warrant further monitoring include northwest Texas and, to a lesser degree, west and central Texas. Received: 8 August 1995 · Accepted: 6 September 1995     

Estimation of radon concentration in dwellings in and around Guwahati

It has been established that radon and its airborne decay products can present serious radiation hazards. A long term exposure to high concentration of radon causes lung cancer. Besides, it is also known that out of the total radiation dose received from natural and man-made sources, 60% of the dose is due to radon and its progeny. Taking this into account, an attempt has been made to estimate radon concentration in dwellings in and around Guwahati using aluminium dosimeter cups with CR-39 plastic detectors. Results of preliminary investigation presented in this paper show that the mean concentration is 21.31 Bq m^− 3.     

Geochemistry of granites and metasediments of the urban area of Vila Real (northern Portugal) and correlative radon risk

Radon concentration was evaluated in dwellings of the urban area of Vila Real (Northern Portugal). The area is mainly composed of Hercynian granites and Cambrian metasediments, and CR-39 passive detectors (n = 112) were used for the purpose. The results obtained in winter conditions suggest that the most productive geological unit is the Hercynian granite G1 (geometric mean of 364 Bq/m³), while Cambrian metasediments of the Douro Group show the lowest average indoor radon concentration (236 Bq/m³). The geological, geochemical and radiological data obtained suggest that the most effective control on the radon concentrations of the area is related with the uranium content of the rocks; indeed, the highest contents were observed in granite G1 (21 ppm) and the lowest in the metasediments (3 ppm). This is also confirmed by the results obtained for groundwater, where granites present the highest concentrations of dissolved radon (up to 938 Bq/l), uranium (5–18 ppb) and gross α activities (0.47–0.92 Bq/l). No important radiometric anomalies were found in relation with geological structures such as faults, veins and contacts, but a moderate increase of the uranium content can occur locally in such structures. Petrographic observations and SEM studies show that uranium is mainly contained within the rock in heavy accessory minerals (apatite, zircon, monazite, xenotime), which reduces radon emanation. Notwithstanding, due to the high U contents granites show a significant potential to induce indoor radon concentrations in dwellings in excess of the recommended value of 400 Bq/m³. Overall, we can conclude that the region of Vila Real presents a moderate to high radon risk in dwellings and groundwater.     

Estimation of concentration and exposure doses due to radon by using CR-39 plastic track detectors in the residences of Sudhnuti, Azad Kashmir, Pakistan

This paper presents the results of indoor radon concentration measurements in 120 dwellings of district Sudhnuti of Azad Kashmir. Measurements were taken with CR-39 passive alpha track detector. CR-39 based box type radon detectors were installed in a bedroom and living rooms of each house. The detectors were retrieved after exposing to indoor radon for period of 6 months and then etched in 6 M NaOH at 80°C for 16 h, the observed track densities were converted in to the indoor radon concentration. Indoor radon concentration varied from 20 ± 12 to 170 ± 4 Bq m⁻³ for the houses of the district Sudhnuti. Arithmetic mean (AM), geometric mean (GM) and geometric standard deviations (GSD) were found to be 82 ± 6, 77 ± 6 and 1.51, respectively. The minimum value of weighted average radon concentration was recorded in one of the house of Mang town, whereas the maximum value was found in the Pattan Sher Khan region. Doses due to indoor radon exposure vary from 0.50 ± 0.31 to 4.28 ± 0.11 mSv year⁻¹ AM, GM and GSD. of mean effective doses were found to be 2.06 ± 0.13, 1.95 ± 0.18 and 1.51, respectively. According to the recommendations made by the Health Protection Agency, UK (200 Bq m⁻³) all the houses surveyed are within the safe limits.     

Predicting New Hampshire indoor radon concentrations from geologic information and other covariates

 Generalized geologic province information and data on house construction were used to predict indoor radon concentrations in New Hampshire (NH). A mixed-effects regression model was used to predict the geometric mean (GM) short-term radon concentrations in 259 NH towns. Bayesian methods were used to avoid over-fitting and to minimize the effects of small sample variation within towns. Data from a random survey of short-term radon measurements, individual residence building characteristics, along with geologic unit information, and average surface radium concentration by town, were variables used in the model. Predicted town GM short-term indoor radon concentrations for detached houses with usable basements range from 34 Bq/m³ (1 pCi/l) to 558 Bq/m³ (15 pCi/l), with uncertainties of about 30%. A geologic province consisting of glacial deposits and marine sediments was associated with significantly elevated radon levels, after adjustment for radium concentration and building type. Validation and interpretation of results are discussed. Received: 20 October 1997 · Accepted: 18 May 1998     

Alternative water resources in granitic rock: a case study from Kinmen Island,Taiwan

Kinmen Island is a small, tectonically stable, granitic island that has been suffering from a scarcity of fresh water resources due to excessive annual evapotranspiration over annual precipitation. Recent studies further indicate that shallow (0–70 m) sedimentary aquifers, the major sources of groundwater supply, have already been over-exploited. Therefore, this preliminary study is to investigate the existence of exploitable water resources that can balance the shortage of fresh water on this island. Site characterization data are obtained from island-wide geophysical surveys as well as small-scale tests performed in a study area formed by three deep (maximum depth to 560 m) vertical boreholes installed in mid-east Kinmen northeast to Taiwu Mountain. Vertical fracture frequency data indicate that the rock body is fractured with a spatially correlated pattern, from which three major fracture zones (depths 0–70, 330–360, and below 450 m) can be identified. Geologic investigations indicate that the deepest fracture zone is caused by the large-scale, steeply dipping Taiwushan fault. This fault may have caused a laterally extensive low-resistivity zone, a potential fractured aquifer, near Taiwu Mountain. The middle fracture zone is induced by the Taiwushan fault and intersects the fault approximately 21 m southeast of the study area below a depth of 350 m. Slug testing results yield fracture transmissivity varying from 4.8 × 10⁻⁷ to 2.2 × 10⁻⁴ m²/s. Cross-hole tests have confirmed that hydraulic connectivity of the deeper rock body is controlled by the Taiwushan fault and the middle fracture zone. This connectivity may extend vertically to the sedimentary aquifers through high-angle joint sets. Despite the presence of a flow barrier formed by doleritic dike at about 300 m depth, the existence of fresh as well as meteoric water in the deeper rock body manifests that certain flow paths must exist through which the deeper fractured aquifers can be connected to the upper rock body. Therefore, groundwater stored within the Taiwushan fault and the associated low-resistivity zone can be considered as additional fresh water resources for future exploitation.     

Geological and tectonic influence on water–soil–radon relationship in Mandi–Manali area,Himachal Himalaya

Radon measurements in soil and groundwater (springs, thermal springs and handpumps) were made in a variety of lithological units including major thrusts between Mandi and Manali in Himachal Himalaya. Analysis of radon data in light of lithological controls and influence of deep-seated thrusts has been made to elucidate the causative factors for anomalous emanation of radon. The lithological types include banded gneisses, schists, quartzite, granite, phyllites, volcanics and mylonites. The low-grade metasedimentries of Shali and Dharamsala generally show low and narrow range of radon concentration in water (5.6–13.4 Bq/l) as well as in soil (1.8–3.2 kBq/m³) except for the samples related to thrusts. On the other hand, sheared and deformed rocks of Chail and Jutogh show moderate radon content (average 5.03 kBq/m³, range 2.9–11.1 kBq/m³) in soil. However, the groundwater radon concentration shows wide variation in different types of sources (2.1–80.8 Bq/l). The quartzite and volcanic rocks of Rampur formation in this area present as a window separated by Chail thrust. Radon emanations on these rock types are relatively high (6.3–68.1 Bq/l in water and 5.5–15.9 kBq/m³ in soil) and are exceptionally high in samples that are related to uranium mineralization, deep-seated thrusts and hot springs (13.5–653.5 Bq/l). It is generally observed that anomalous high radon content is associated with mineralization, deeper source and tectonic discontinuities. Whereas it is obvious that subsurface radioactive mineralization would facilitate enhanced radon production, however, thrust plains provide easy pathways for escape of gases from the deeper sources. Shallow and deep sources of the groundwater have contrasting radon content particularly in the deformed and metamorphosed rocks of Jutogh and Chail. Shallow groundwater sources, mainly handpumps, have lower radon concentration due to limited superficial water circulation, whereas deeper sources, mainly perennial springs, show higher radon content because of larger opportunity for water–rock interaction.     

The indoor radon problem: Studies in the Albuquerque,New Mexico area

Radon buildup in homes is now recognized throughout the world as a potentially major health hazard. The U.S. Nuclear Regulatory Commission and the U.S. Environmental Protection Agency estimate 8,000–30,000 fatalities per year in the United States due to indoor radon. The Albuquerque, New Mexico area was chosen for study because it is representative of metropolitan areas in the southwestern United States where slightly uraniferous source rocks (Sandia granite) have provided the very immature soil for much of the area. The granite contains 4.7 ppm U, and limestone capping the granite 5.7 ppm U. Soils in the area average 4.24 ppm U, and Th/U ratios average 3.2. These data suggest some removal of U from the source rocks, but fixation of the U in the soils (that is, as opposed to widespread removal of the U by solution), thus providing a ready source for soil radon. A pilot study of soil radon in the area in winter of 1983–1984 shows high values, 180 pCi/l, relative to the U.S. average (about 100 pCi/l). In the winter of 1986–1987, 180 dwellings were surveyed for their indoor radon levels, including 20 that had been surveyed in summer of 1986. Twenty-eight percent of those in the winter study yielded indoor radon above the EPA suggested maximum permissible level of 4 pCi/l air, well above the EPA estimate of 10–15 dwellings for the U.S. The indoor radon levels show positive correlation with closeness to the Sandia Mountains, to soil radon, to excess insulation, to homes with solar capacities, and other factors. Building materials may provide a very minor source of some indoor radon. Summer readings are lower than winter readings except when the houses possess refrigerated air conditioning.     

Upwellings in Lake Baikal

Based on shipboard and satellite observations, the characteristics of upwelling in Lake Baikal in the period of direct temperature stratification have been determined for the first time. Coastal upwellings appear annually under the effect of run-down and alongshore winds and are traced along the coast to a distance of up to 60–100 km and up to 250 km in North Baikal. Analogous to the way it occurs in seas, water rises from the depths of 100–200 m (350 m as a maximum) at the velocity of 0.1 × 10⁻²−6.5 × 10⁻² cm/s. Divergence in the field of intràbasin cyclonic macrovortices produces upwelling in the Baikal pelagic zone and downwelling in the vicinity of shores; this lasts from 7 to 88 days and covers the depth interval of 80–300 m in August and up to 400–800 m in early-mid November. The area of upwellings occupies up to 20–60% of the separate basins of the lake. Vertical circulation of water in the field of pelagic upwellings leads to intensification of coastal currents and to formation of the thermobar with a heat inert zone in the central part of the lake in November, and this thermobar is not observed in other lakes, at that.     

Hydraulic properties of the crystalline basement

Hydraulic tests in boreholes, up to 4.5 km deep, drilled into continental crystalline basement revealed hydraulic conductivity (K) values that range over nine log-units from 10⁻¹³−10⁻⁴ m s⁻¹. However, K values for fractured basement to about 1 km depth are typically restricted to the range from 10⁻⁸ to 10⁻⁶ m s⁻¹. New data from an extended injection test at the KTB research site (part of the Continental Deep Drilling Program in Germany) at 4 km depth provide K=5 10⁻⁸ m s⁻¹. The summarized K-data show a very strong dependence on lithology and on the local deformation history of a particular area. In highly fractured regions, granite tends to be more pervious than gneiss. The fracture porosity is generally saturated with Na–Cl or Ca–Na–Cl type waters with salinities ranging from <1 to >100 g L⁻¹. The basement permeability is well within the conditions for advective fluid and heat transport. Consequently, fluid pressure is hydrostatic and a Darcy flow mechanism is possible to a great depth. Topography-related hydraulic gradients in moderately conductive basement may result in characteristic advective flow rates of up to 100 L a⁻¹ m⁻² and lead to significant advective heat and solute transfer in the upper brittle crust. An erratum to this article can be found at     

Environmental aspect of radon potential in terra rossa and eutric cambisol in Slovenia

Terra rossa and eutric cambisol soils were surveyed in Slovenia. At both sites, 6–13 boreholes were drilled in a regular 24 m × 24 m square grid. Soil samples from various depths were taken for gamma spectrometric analysis, and radon in soil gas was measured at a depth of 80 cm using an AlphaGuard instrument. The following ranges of activity concentration (Bq kg⁻¹) were obtained for ²³⁸U, ²²⁶Ra, ²²⁸Ra, ⁴⁰K and ¹³⁷Cs: in terra rossa, 64–74, 70–84, 45–49, 293–345, 20–30 and, in eutric cambisol, 55–80, 132–147, 50–57, 473–529, 106–272. Radon activity concentrations in both soils ranged from about 100 kBq m⁻³ to 370 kBq m⁻³.     

Erosion rates evaluated by the <Superscript>137</Superscript>Cs technique in the high altitude area of the Qinghai–Tibet plateau of China

Studying spatial and temporal variation of soil loss is of great importance because of global environmental concerns. Understanding the spatial distribution of soil erosion and deposition in the high-cold steppe is important for designing soil and water conservation measures. Measured ¹³⁷Cs losses (Bq m⁻²) from long-term high altitude (4,000 m above sea level) watershed plots on the Qinghai–Tibet plateau and derived soil erosion estimates (Mg ha⁻¹ year⁻¹) were significantly correlated to directly measured soil losses from the same plots, over the same period (1963–2005). The local reference inventory was estimated to be 2,468 Bq m⁻². The result of analyzing ¹³⁷Cs distribution and its intensity in the soil profiles in this area shows similarities to ¹³⁷Cs distribution in other areas. ¹³⁷Cs is basically distributed in the topsoil layer of 0–0.3 m. Soil erosions vary greatly in the entire sampled area, ranging from 5.5 to 23 Mg ha⁻¹ year⁻¹, with an average of 16.5 Mg ha⁻¹ year⁻¹ which is a moderate rate of erosion.     

Geology and vein tin mineralization in the Dadoushan deposit,Gejiu district,SW China

Vein-type tin mineralization in the Dadoushan deposit, Laochang ore field, Gejiu district, SW China, is predominantly hosted in Triassic carbonate rocks (Gejiu Formation) over cupolas of the unexposed Laochang equigranular granite intrusion. The most common vein mineral is tourmaline, accompanied by skarn minerals (garnet, diopside, epidote, phlogopite) and beryl. The main ore mineral is cassiterite, accompanied by minor chalcopyrite, pyrrhotite, and pyrite, as well as scheelite. The tin ore grade varies with depth, with the highest grades (~1.2 % Sn) prevalent in the lower part of the vein zone. Muscovite ⁴⁰Ar–³⁹Ar dating yielded a plateau age of 82.7 ± 0.7 Ma which defines the age of the vein-type mineralization. Measured sulfur isotope compositions (δ ³⁴S = −4.1 to 3.9 ‰) of the sulfides (arsenopyrite, chalcopyrite, pyrite, and pyrrhotite) indicate that the sulfur in veins is mainly derived from a magmatic source. The sulfur isotope values of the ores are consistent with those from the underlying granite (Laochang equigranular granite, −3.7 to 0.1 ‰) but are different from the carbonate wall rocks of the Gejiu Formation (7.1 to 11.1 ‰). The calculated and measured oxygen and hydrogen isotope compositions of the ore-forming fluids (δ ¹⁸O_H2O = −2.4 to 5.5 ‰, δD = −86 to −77 ‰) suggest an initially magmatic fluid which gradually evolved towards meteoric water during tin mineralization.     

CO2-rich thermomineral groundwater in the Betic Cordilleras, southeastern Spain: Genesis and tectonic implications

The CO₂-rich thermal groundwater in the Betic Cordilleras in Spain has been studied with regard to the geological and hydrogeological setting, physical and chemical characteristics, and ¹³C-isotope content. The study area is about 60 km northeast of Almería city, in southeastern Spain. The thermomineral waters are plentiful and are related to regional geothermal anomalies. Temperatures of 20 −41°C, high bicarbonate concentrations (183–1824 mg/L), and high amounts of PCO₂ (<1.1 bar) characterize the groundwater. CO₂ spatial variations are related to proximity to the Carboneras, Palomares, and Guadalentín fault systems, which may be the surface representation of the zone of crustal thinning and magmatism. δ ¹³C values probably indicate a deep source for the CO₂, either the mantle or perhaps carbonate rocks in the metamorphic substratum. The high amount of CO₂ in the groundwater causes problems in wells and severely restricts water usage. The hydrothermal features of this area are probably related to neotectonic activity. Received, September 1998/Revised, June 1999, September 1999/Accepted, December 1999     

Radon in groundwater as a tracer to assess flow velocities: two test cases from Israel

 Two test cases from Israel are presented herein employing the decay rate of radon along the flow path to assess groundwater flow velocities. Groundwater flow reaching the fault zone emerges in several places along the rift fault zone as thermal springs because of deep water confinement. The high water temperature of the surface is indicative of high vertical flow velocities, which maintains the original high temperatures. Knowing the Rn content at a source point and at a given down-gradient, and assuming no Rn addition from the water itself or along the flow path, one can calculate the flow velocity based on the Rn half-life time. The decay of Rn in western Galilee was found to be ∼570–150 pCi/l, and in the Dead Sea area from 5000–2000 pCi/l along a respective flow path of 1000 and 200 m, Based on the above, the calculated flow velocities were compared with those obtained from pumping tests in the study area. The method is applicable, because of the short Rn half-life, to cases of high Rn contents, short distances and high flow velocities. Received: 18 January 2000 · Accepted: 21 March 2000     

Heat flow and crustal thermal structure in the Late Archaean Closepet Granite batholith,south India

The Late Archaean Closepet Granite batholith in south India is exposed at different crustal levels grading from greenschist facies in the north through amphibolite and granulite facies in the south along a ∼400 km long segment in the Dharwar craton. Two areas, Pavagada and Magadi, located in the Main Mass of the batholith, best represent the granitoid of the greenschist and amphibolite facies crustal levels respectively. Heat flow estimates of 38 mW m⁻² from Pavagada and 25 mW m⁻² from Magadi have been obtained through measurements in deep (430 and 445 m) and carefully sited boreholes. Measurements made in four boreholes of opportunity in Pavagada area yield a mean heat flow of 39 ± 4 (s.d.) mW m⁻², which is in good agreement with the estimate from deep borehole. The study, therefore, demonstrates a clear-cut heat flow variation concomitant with the crustal levels exposed in the two areas. The mean heat production estimates for the greenschist facies and amphibolite facies layers constituting the Main Mass of the batholith are 2.9 and 1.8 μW m⁻³, respectively. The enhanced heat flow in the Pavagada area is consistent with the occurrence of a radioelement-enriched 2-km-thick greenschist facies layer granitoid overlying the granitoid of the amphibolite facies layer which is twice as thick as represented in the Magadi area. The crustal heat production models indicate similar mantle heat flow estimates in the range 12–14 mW m⁻², consistent with the other parts of the greenstone-granite-gneiss terrain of the Dharwar craton.