Concentrations of 222 Rn, Its Short-Lived Daughters And 212 Pb And Their Ratios Under Complex Atmospheric Conditions And Topography

Atmospheric activity concentrations of ²¹²Pb and short-lived ²²²Rndaughters, together with meteorological elements, have been observed continuously atthree sites at Kamisaibara Village in Japan. In addition, atmospheric activity concentrationof ²²²Rn, equilibrium-equivalent concentration of ²²²Rn and conditionsof the lower atmosphere were observed for three intensive observation periods at Akawase,one of the three sites in Kamisaibara Village. The equilibrium-equivalent concentration of²²²Rn is almost the same as the atmospheric activity concentration of short-lived²²²Rn daughters.The activity concentrations of ²¹²Pb and the short-lived ²²²Rn daughtersand their ratio were low in the daytime owing to convective mixing, and high at nightowing to the surface-based inversion during periods of no precipitation. Their variationshave several patterns corresponding to the scale of the drainage wind or weak mixing.Mechanical mixing due to strong winds through both day and night during the first andsecond observation periods made the atmospheric activity concentrations of ²¹²Pb and the short-lived ²²²Rn daughters continuously low. However, their ratios werecontinuously high during the first period yet continuously low during the second period.This difference can be explained by the effect ofextraction of ²²⁰Rn and ²²²Rndue to strong winds and snow cover. There were also cases in which the ratio of theatmospheric activity concentration of ²¹²Pb to that of the short-lived ²²²Rndaughters at night was equal to or less than the ratio in the daytime. Thisinverse trend, asin the periods of no precipitation mentioned above, is considered to be due to near-neutralconditions on these nights.We find a difference in the ratio of the equilibrium-equivalent concentration of²²²Rn (the activity concentration of short-lived ²²²Rn daughters) tothe activity concentration of ²²²Rn during the first observation period and thatduring the second. The difference can be explained by snow cover on the ground. Wealso find differences among the ratios of the activity concentration of the short-lived²²²Rn daughters to that of ²²²Rn during the three observation periods.These differences can be explained by the submergence of paddy fields.     

A Study Of The Atmospheric Boundary Layer Using Radon And Air Pollutants As Tracers

Concentrations of radon ²²²Rn andair pollutants, meteorological parametersnear the surface and vertical profiles of meteorological elements were measured atUchio (Okayama City, Okayama Prefecture, Japan) 12 km north from the coast ofthe Inland Sea of Japan. In the nighttime, the ²²²Rn concentration increased in the case of weak winds, but did not increase as much in the case of moderate or strong winds, as had been expected. In the daytime, the ²²²Rn concentrationheld at a slightly higher than average level for the period from sunrise to about 1100 JST. It is considered that this phenomenon is due to a period of morning calm, that is, a transition period from land breeze to sea breeze.NO, which is sensitive to traffic volume,brought information concerning advection.Oxidant concentrations,which reflect the availability of sunlight,acted in the reverse manner to ²²²Rnconcentrations. Thus, a set of ²²²Rn and air pollutants could provide useful information regarding the local conditions of the atmospheric boundary layer.     

Radon-222 measurements during the Tropoz II campaign and comparison with a global atmospheric transport model

The aim of the ²²²Rn measurements during the airborne campaign TROPOZ II, was first to help in the interpretation of the photochemical studies, and secondly to furnish a data set of ²²²Rn in the troposphere, for validation of atmospheric transport models. In this paper we present the ²²²Rn measurements, and their simulation with a 3-D atmospheric transport model based on observed winds. The ²²²Rn was measured using the active daughters deposit technique with isokinetic aerosol sampling. We have obtained 44 measurements distributed between 65° North and 55° South, from 1 to 11 km height. In 25% of cases, we found relatively high concentrations (> 300 mBq·scm) of ²²²Rn in the high troposphere (>8 km). The results of 3D simulations and the calculations of back-trajectories allow us to find the origins of the high ²²²Rn concentrations. The transport model reproduced most of the observed synoptic variations, but it overestimates the concentrations which implies a vertical transport of excessive velocity.     

On the Formation of an Elevated Nocturnal Inversion Layer in the Presence of a Low-Level Jet: A Case Study

We report on observed nocturnal profiles, in which an inversion layer is located at the core of a low-level jet, bounded between two well-mixed layers. High-resolution vertical profiles were collected during a field campaign in a small plain in the Israeli desert (Negev), distant 100 km from the eastern shore of the Mediterranean Sea. During the evening hours, the synoptic flow, superposed on the late sea breeze, forms a low-level jet characterized by a maximum wind speed of 12 m s ⁻¹ at an altitude of 150 m above the ground. The strong wind shear at the jet maximum generates downward heat fluxes that act against the nocturnal ground cooling. As a result, the typical ground-based nocturnal inversion is “elevated” towards the jet centre, hence a typical early morning thermal profile is observed a few hours after sunset. Since the jet is advected into the region, its formation does not depend on the presence of a surface nocturnal inversion layer to decouple the jet from surface friction. On the contrary, here the advected low-level jet acts to hinder the formation of such an inversion. These unusual temperature and wind profiles are expected to affect near-ground dispersion processes.     

Luminosity characteristics of leaders in natural cloud-to-ground lightning flashes

Using high-speed cameras, we have recorded the leaders contained in four natural negative cloud-to-ground (CG) lightning flashes in the summers of 2006 and 2007 at Conghua, Guangdong, China. It was found that the downward negative leaders preceding the first return stroke could propagate at quite different speeds. In one flash, the average speed of the downward negative stepped leader with no branches is about 2.2 × 10⁶ m s^− 1, while that of the other 3 flashes are all of the order of 10⁵ m s^− 1 with multilevel branches. The luminosity of the leaders shows an increasing tendency in propagating downward to the ground. For the leaders preceding the subsequent strokes, although all of them exhibit high speeds as reported previously. One subsequent leader exhibits an increasing speed from 5.2 × 10⁵ m s^− 1 to 1.7 × 10⁶ m s^− 1 during its propagation from about 1.26 to 0.36 km above the ground, and its luminosity also increased. The speed and luminosity of a leader between subsequent strokes of a natural lightning appear to decrease as it developed downward. Its speed ranges from 1.1 × 10⁶ to 1.1 × 10⁵ m s^− 1, with a height between 1.15 and 0.81 km above the ground.     

Boundary-layer effects on mountain waves: a new look at some historical studies

Early studies of mountain waves reported various results that have rarely been investigated since. These include: large-amplitude mountain waves above an unstable boundary layer much higher than the mountains; a repeated downwind drift and upwind jump of mountain waves; and larger vertical wind magnitude near sunrise and/or sunset. These are investigated using over 3,000 radiosondes and meso-strato-troposphere (MST) radar. Superadiabatic temperature gradients are found beneath mountain waves, explainable by convection which appears to raise the mountain-wave launching height. Movement of mountain-wave patterns is studied by a new method using height–time vertical wind data. A swaying motion of mountain waves, with period of a few minutes, appears to be equally upwind and downwind, rather than asymmetric at the heights measurable. Also, vertical wind shows no change in mean, variance or extreme values near sunrise and sunset, despite the expected diurnal changes of boundary-layer structure. An explanation for differences between MST radar and other measurements and models of mountain waves is suggested in terms of more than one variety of mountain wave. Type 1 has stable air near the ground; type 2 is above a convective/turbulent boundary layer of significant height as compared to the mountains.     

Variations of Total Nitrogen Oxide Content in the Atmosphere over the North Caucasus

The data are presented on total nitrogen dioxide (NO₂) content in the atmosphere from 1979 to 2009 at the high-mountain scientific station located in the unpolluted area in the North Caucasus at the height of 2070 m above the sea level (43.7° N, 42.7° E). The total content of NO₂ was measured on the basis of attenuation of direct solar radiation over slope pathways after the sunrise and before the sunset. Characteristics features are analyzed of temporal variability of total NO₂ content in the atmosphere related to its diurnal and seasonal variations, 11-year solar activity, volcanic eruptions, quasi-biennial oscillations of tropical circulation, and the El Niño effect.     

苏州城区大气边界层低空急流特征分析

利用2012年苏州城区风廓线雷达的观测资料,从低空急流个例分析入手,选取1、4、7、10月四个典型月份,分析该地区边界层低空急流的时空分布及强度变化特征。结果表明:冬春两季低空急流发生频率最高,夏季出现频率最低。在4个典型月份里低空急流均表现出日落后出现频率升高,夜间保持稳定,日出后出现频率降低的特征。全年有80%的低空急流分布在900 m以下高度上,冬、夏季平均高度最低。全年低空急流风速70%以上集中在4~12 m·s~(-1),小于4 m·s~(-1)和大于20 m·s~(-1)的低空急流出现频率较低。     

The behavior of vertically integrated boundary-layer winds

This research provides a study of the behavior of vertically integrated boundary-layer winds (IBLWs). This information should be helpful for both theoretical and practical applications, e.g., boundary-layer parameterization in general circulation models, air pollution models, and low-level parachuting operations. The study concerned itself with winds integrated up to a height of 300 m in the United States. The only data suitable for studying the behavior of IBLWs for such heights were measurements taken on tall towers. An extensive search indicated that data were readily available from only four towers instrumented to or above 300 m. These were located in rural locations in Texas, Oklahoma, Nevada, and South Carolina. At each location, means and coefficients of variation of IBLWs were computed, plotted as a function of time since sunrise/sunset, and compared. The research shows that IBLWs may differ appreciably in magnitude at different locations; may have considerable universality in behavior, and may also be ‘regionally’ dependent; and that IBLWs have a pronounced diurnal variation linked to sunrise/sunset time.     

Distribution of222Rn over the north Pacific: Implications for continental influences

The atmospheric distribution of²²²Rn over the north Pacific is simulated with a three-dimensional chemical tracer model using meteorological input from the NASA-GISS general circulation model (4°×5° resolution). Radon-222 (half-life 3.8 days) is a tracer of continental air. Model results are in good agreement with measurements from ships and aircraft. Strong Asian influence is found throughout the tropospheric column over the north Pacific in spring, reflecting a combination of frequent convection over the continent, strong westerly winds at altitude, and subsidence over the ocean. In summer, the upper troposphere over the north Pacific is heavily affected by deep convection over China; however, Asian influences at the surface are then at their yearly minimum. In winter, strong Asian influence is found near the surface but not at high altitudes. Transport of American air over the Pacific is important only at low latitudes. American sources account for 11% of total²²²Rn in the model at Midway, 30% at Mauna Loa and 59% at Oahu. Results for Hawaii indicate two seasonal peaks of American influence, one in summer and one in winter. The tropical western Pacific is particularly remote from continental influences year round.     

Measurements of solar occulation: the error in a naive retrieval if the constituent's concentration changes

The stratospheric concentrations of many minor constituents change rapidly at sunrise or sunset. If this happens, there is an inherent error when retrieving the vertical profiles of the constituents from measurements of their absorption of sunlight. For retrievals of NO at sunset the error can be estimated from in-situ measurements alone, without appeal to a model of stratospheric photochemistry. Below 20 km this error can approach 100% so that the retrieved NO is zero. But at 40 km, and at 25 km when the absorption is strong and Lorentzian, it can be less than 20%. Precise calculations of the error, even if small, require model calculations of the sunset and sunrise changes. With a model, we have calculated the error for NO, NO₂, OH and ClO.     

Vertical atmospheric structure of the late summer clear days over the east Gansu loess plateau in China

In this paper, by using the sounding data collected in LOPEX05, we have analyzed the vertical atmospheric structure and boundary layer characteristics of temperature and humidity in the late summer over the east Gansu loess plateau. The results show that the bottom of the stratosphere is at about 16 500 m and varies between 14 000 m and 18 000 m above the ground. The center of the westerly jet is located between 8300 m and 14 300 m above the ground and its direction moves between 260° and 305°. There is an ...     

Microclimatological characteristics of a miscanthus (Miscanthus cv. giganteus) stand during stable conditionsat night in the nonvegetative winter period

Summary ?Microclimatological data obtained during a field experiment in the nongrowing winter period were used to study the microclimatologically stable night conditions of a 200 × 150 m miscanthus (Miscanthus cv. giganteus) stand and compared to open field conditions. The microclimatological pattern within the miscanthus canopy was characterized by long-wave radiative cooling of the plant stand and by an established temperature inversion within the canopy at calm nights. The results show that there are significant differences in air temperature and energy balance components between the open field and the miscanthus field during calm and clear nights. In general, net radiation difference during the cold and calm nights was relatively constant and about 20 W m⁻² less negative in miscanthus (because of lower surface temperatures) than at the open field. Air temperature differences also remained fairly constant and were up to 3 °C lower than at the open field (at the height of 1 m). Through thermal inversion cold air accumulated in the lower parts of the canopy as shown by the vertical air temperature profiles. They showed a greater amplitude within the diurnal cycle in the miscanthus stand than in the open field. Through the onset of wind, temperature profiles changed rapidly and differences diminished. Vertical katabatic air drainage into the canopy layers was estimated indirectly by using the energy balance approach. It was calculated from the significant energy balance closure gap and showed a mean air exchange rate of up to 22 m³ m⁻² h⁻¹, related to a stand volume of 1 m² area and 4 m height, during the mostly calm and clear nights, depending on the canopy net radiation and turbulent heat exchange forced by slight wind spells. Quantitative uncertainties in calculated cold air drainage which are introduced by the measurement method and certain assumptions in the calculations, were considered in a sensitivity analysis. In spite of these uncertainties evidence of katabatic cold air flow is given. Received July 29, 1999; revised June 11, 2001; accepted March 14, 2002     

Temperature fluctuations inside a cloud-laden airstream flowing over a hill station

Observations of temperature in a cloud-laden monsoon airstream at a height of 12 m above ground at a hill station, Mahabaleshwar (elevation 1390 m asl), were obtained for ten hours using a linearised thermistor (YSI Part 44202) as a temperature sensor, and analysed. It was found that the frequency distributions of temperatures were multimodal. The horizontal temperature gradients in the air stream were symmetrically distributed. The temperature spectra in the frequency range (0.001 to 0.1 Hz) studied can be classified into a lower frequency regime and a higher frequency regime separated approximately at the frequency 0.01 Hz or the wave number 3 km^–1. The spectra in the higher range conform to Kolmogorov's power law for the inertial subrange and those in the lower range exhibit a steeper negative slope of the order of -1.3. There is very little variation of air temperature associated with rainfall intensities greater than 4 mm hr^–1; for lower intensities, the smaller the intensity, the greater the variation.     

Water Loss and Canopy Resistance of a Young Sitka Spruce Plantation

Transpiration of a 7 m-high Stika spruce forest was investigated using measurements of net radiation, sensible heat and ground heat fluxes in an energy balance to give latent heat flux, and hence canopy resistance from the Penman-Monteith equation. Sensible heat flux was measured by the eddy-correlation method using a Fluxatron circuit. During six consecutive days of measurement in July/August, canopy resistance typically followed a decreasing trend from high values (≈150 s m⁻¹) at dawn to around 40 s m⁻¹ at midday and then returning steadily to >100 s m⁻¹ at sunset. Transpiration was 3 mm day⁻¹ on average over the period studied and changes in the rate within the day were significantly correlated with changes in net radiation. Comparisons are drawn with published data from other forest sites and the conclusion is reached that it is imprudent to generalise about transpiration rates and canopy resistances of different species at different sites from results gathered at one or two places.     

Dew Formation,Eddy-Correlation Latent Heat Fluxes,and the Surface Energy Imbalance at Cabauw During Stable Conditions

Observations collected between 2000 and 2008 at the Cabauw meteorological measurement platform in the Netherlands were conditionally sampled to select nights with stably stratified atmospheric conditions, clear skies and weak horizontal wind speeds (<3 m s⁻¹). For these conditions the eddy-correlation latent heat fluxes are found to be negligibly small, while the conditionally sampled surface energy balance exhibits a maximum residual. However, inspection of the specific humidities for these conditions reveals systematic drying trends that are a maximum at the lowest measurement level above the surface. These drying trends occur for any prevailing wind direction. Latent heat fluxes are calculated from the humidity budget equation and from a Penman-Monteith dewfall model, with the results suggesting that during clear, stable nights the observed latent heat fluxes as obtained from the eddy-correlation technique are erroneously small.     

Turbulent Flow at 190 m Height Above London During 2006–2008: A Climatology and the Applicability of Similarity Theory

Flow and turbulence above urban terrain is more complex than above rural terrain, due to the different momentum and heat transfer characteristics that are affected by the presence of buildings (e.g. pressure variations around buildings). The applicability of similarity theory (as developed over rural terrain) is tested using observations of flow from a sonic anemometer located at 190.3 m height in London, U.K. using about 6500 h of data. Turbulence statistics—dimensionless wind speed and temperature, standard deviations and correlation coefficients for momentum and heat transfer—were analysed in three ways. First, turbulence statistics were plotted as a function only of a local stability parameter z/Λ (where Λ is the local Obukhov length and z is the height above ground); the σ _i /u _* values (i = u, v, w) for neutral conditions are 2.3, 1.85 and 1.35 respectively, similar to canonical values. Second, analysis of urban mixed-layer formulations during daytime convective conditions over London was undertaken, showing that atmospheric turbulence at high altitude over large cities might not behave dissimilarly from that over rural terrain. Third, correlation coefficients for heat and momentum were analyzed with respect to local stability. The results give confidence in using the framework of local similarity for turbulence measured over London, and perhaps other cities. However, the following caveats for our data are worth noting: (i) the terrain is reasonably flat, (ii) building heights vary little over a large area, and (iii) the sensor height is above the mean roughness sublayer depth.     

Simultaneous optical and electrical observations on the initial processes of altitude-triggered negative lightning

Using a high-speed camera system and two electric field antenna systems, we have documented the initial processes of an altitude-triggered negative lightning (ATNL). The optical records clearly show that ATNL begins with the inception and propagation of an upward positive leader (UPL) and then a simultaneous propagation of UPL and downward negative leader (DNL), known as the bidirectional leader process, follows. Based on the optical records, it is inferred that (1) the triggering height is about 371 m; (2) the two-dimensional (2D) propagation speed of the UPL in its inception phase is about 3.8–5.5 × 10⁴ m s^− 1 during its propagation from about 393 to 452 m above the ground; (3) the grey levels of the DNL are about one order of magnitude higher than that of the UPL in their inception phase; (4) a discharge phenomenon propagating along the elevated triggering wire part of the lightning channel occurs after the mini-return stroke (MRS), with a 2D propagation speed of about 1.6–2.0 × 10⁵ m s^− 1. Combined with the simultaneous electric field change records, it is further inferred that (1) the UPL incepts about 932 μs earlier than the unstable DNL and about 4.1 ms earlier than the stable DNL; (2) the unstable DNL propagates downward intermittently three times with a time interval of about 1 ms, and each propagation contains a different number of steps with an average step length of about 7 m; (3) the stable DNL incepts at the tip of the unstable one, with a 2D propagation speed of about 1.9 × 10⁵ m s^− 1, an average step length of about 3 m, and a stepping time interval varying from 6 to 31 µs with a mean value of 15 µs.     

梯度法观测大气与森林生态系统间羰基硫(COS)的交换通量

本工作用梯度法测定了大气与其下垫的森林间ＣＯＳ的交换通量。测量在德国哥廷根大学的一座５０ｍ高的森林观测塔上进行，该塔坐落在德国中部的Ｓｏｌｌｉｎｇ自然保护区的森林中。观测现场生长着树龄分别为１２０ａ和８０ａ的山毛榉和云杉。树冠线约２８ｍ高。在塔上离地面３２ｍ，３８ｍ和５０ｍ的地方用冷以法同时采集了空气样品。样品用气相色谱－火焰光度检测法测定。ＣＯＳ通量由其梯度及扩散系数求出。扩散系数由与ＣＯＳ一起测得的感热和水蒸气通量导出。在稳定边界层条件下共获得２０条廓线。每条廓线都显示ＣＯＳ浓度随高度下降而降低的趋势，说明森林吸收ＣＯＳ。总的结果表明，ＣＯＳ向森林中的平均输送通量为（１４３±５４）ｎｇＣＯＳｍ－２·ｓ－１．     

Strong Updraft at a Sea-Breeze Front and Associated Vertical Transport of Near-Surface Dense Aerosol Observed by Doppler Lidar and Ceilometer

To study the wind field within the atmospheric boundary layer over the Tokyo metropolitan area, Doppler lidar observations were made 45 km north of Sagami Bay and 30 km west of Tokyo Bay, from 14 May to 15 June 2008. Doppler lidar on 27 May 2008 observed the vertical and horizontal wind structure of a well-developed sea-breeze front (SBF) penetrating from Sagami Bay. At the SBF, a strong updraft (maximum w approximately equal to 5 m s⁻¹) was formed with a horizontal scale of about 500 m and vertical scale of 2 km. The spatial relationship between the strong updraft over the nose of the SBF and prefrontal thermal suggests that the strong updraft was triggered by interaction between the SBF and the thermal. After the updraft commenced, a collocated ceilometer observed an intense aerosol backscatter up to 2 km above ground level. The observational results suggest that the near-surface denser aerosols trapped in the head region of the SBF escaped from the nose of the SBF and were then vertically transported up to the mixing height by the strong updraft at the SBF. This implies that these phenomena occurred not continuously but intermittently. The interaction situations between the SBF and prefrontal thermal can affect the wind structure at the SBF and the regional air quality.