Ozone Vertical Profile Characteristics over Qinghai Plateau Measured by Electrochemical Concentration Cell Ozonesondes

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Quasi-periodic imprints in the equatorial troposphere and stratosphere in three decades of reanalysis data

Wavelet analysis is applied to zonal mean zonal wind and temperature fields to represent characteristics of temporal periodic features different from the annual and semi-annual recurrence in the troposphere and stratosphere. A daily database of reanalyses is used for the period 1979–2008, which comprises the era of satellite-based data, as some discontinuities have been observed around 1978 in previous studies. Levels for this study have been chosen at 400 and 10 hPa, respectively in the middle troposphere and middle stratosphere. As representative for diverse latitudinal regions we have respectively selected 0°, ±20°, ±40°, ±60°, ±80°. Significant features were only found at the equator. The period of the quasi-biennial oscillation (QBO) is found to exhibit a decreasing trend in time over the 30 years studied. Potential harmonics of the QBO are found in the tropical stratosphere but also troposphere. However, they do not exhibit the same tendency. This fact supports in particular the idea that the QBO and the tropospheric biennial oscillation may be unrelated phenomena. Some of the observed features lie within the known range of variability of the El Niño Southern Oscillation. Faint effects of the 11-year solar cycle variability may have been observed in the troposphere and stratosphere, but no firm assertion may be made due to the low number of observed cycles for this kind of phenomenon in the used data-set time span. Short-term solar variabilities leave no relevant imprint.     

Stratospheric climate and variability from a general circulation model and observations

The climate and natural variability of the large-scale stratospheric circulation simulated by a newly developed general circulation model are evaluated against available global observations. The simulation consisted of a 30-year annual cycle integration performed with a comprehensive model of the troposphere and stratosphere. The observations consisted of a 15-year dataset from global operational analyses of the troposphere and stratosphere. The model evaluation concentrates on the simulation of the evolution of the extratropical stratospheric circulation in both hemispheres. The December–February climatology of the observed zonal mean winter circulation is found to be reasonably well captured by the model, although in the Northern Hemisphere upper stratosphere the simulated westerly winds are systematically stronger and a cold bias is apparent in the polar stratosphere. This Northern Hemisphere stratospheric cold bias virtually disappears during spring (March–May), consistent with a realistic simulation of the spring weakening of the mean westerly winds in the model. A considerable amount of monthly interannual variability is also found in the simulation in the Northern Hemisphere in late winter and early spring. The simulated interannual variability is predominantly caused by polar warmings of the stratosphere, in agreement with observations. The breakdown of the Northern Hemisphere stratospheric polar vortex appears therefore to occur in a realistic way in the model. However, in early winter the model severely underestimates the interannual variability, especially in the upper troposphere. The Southern Hemisphere winter (June–August) zonal mean temperature is systematically colder in the model, and the simulated winds are somewhat too strong in the upper stratosphere. Contrary to the results for the Northern Hemisphere spring, this model cold bias worsens during the Southern Hemisphere spring (September–November). Significant discrepancies between the model results and the observations are therefore found during the breakdown of the Southern Hemisphere polar vortex. For instance, the simulated Southern Hemisphere stratosphere westerly jet continuously decreases in intensity more or less in situ from June to November, while the observed stratospheric jet moves downward and poleward.This paper was presented at the Third International Conference on Modelling of Global Climate Change and Variability, held in Hamburg 4–8 Sept. 1995 under the auspice of the Max Planck Institute for Meteorology, Hamburg. Editor for these papers is L. Dümenil.     

中间层顶区域大气平均风场年和半年振荡的全球结构

利用2003~2011年TIDI(TIMED Doppler Interferometer)风场观测数据研究了中间层顶区域80~105 km纬向平均风场年振荡和半年振荡振幅和相位的全球分布结构,并给出了它们的年际变化。在热带地区,纬向风半年振荡最显著。振幅峰值中心位于南半球10°S~20°S范围,出现与平流层半年振荡类似的相对于赤道不对称的分布,并且振幅峰值与以前在该区域的研究结果存在较大差别。在中高纬度地区,纬向风和经向风被年振荡所控制。纬向风在高度100 km以下中高纬度都存在振幅大值中心;经向风年振荡只出现在两半球中纬度高度95 km以下,并且南北半球振幅峰值中心分布不一致。分析结果还显示年振荡和半年振荡振幅存在显著地年际变化,相位的年际变化则较小,但北半球热带地区经向风年振荡振幅和相位表现出2年周期的变化。     

Climatic changes associated with a global “2°C-stabilization” scenario simulated by the ECHAM5/MPI-OM coupled climate model

In this study, concentrations of the well-mixed greenhouse gases as well as the anthropogenic sulphate aerosol load and stratospheric ozone concentrations are prescribed to the ECHAM5/MPI-OM coupled climate model so that the simulated global warming does not exceed 2°C relative to pre-industrial times. The climatic changes associated with this so-called “2°C-stabilization” scenario are assessed in further detail, considering a variety of meteorological and oceanic variables. The climatic changes associated with such a relatively weak climate forcing supplement the recently published fourth assessment report by the IPCC in that such a stabilization scenario can only be achieved by mitigation initiatives. Also, the impact of the anthropogenic sulphate aerosol load and stratospheric ozone concentrations on the simulated climatic changes is investigated. For this particular climate model, the 2°C-stabilization scenario is characterized by the following atmospheric concentrations of the well-mixed greenhouse gases: 418 ppm (CO₂), 2,026 ppb (CH₄), and 331 ppb (N₂O), 786 ppt (CFC-11) and 486 ppt (CFC-12), respectively. These greenhouse gas concentrations correspond to those for 2020 according to the SRES A1B scenario. At the same time, the anthropogenic sulphate aerosol load and stratospheric ozone concentrations are changed to the level in 2100 (again, according to the SRES A1B scenario), with a global anthropogenic sulphur dioxide emission of 28 TgS/year leading to a global anthropogenic sulphate aerosol load of 0.23 TgS. The future changes in climate associated with the 2°C-stabilization scenario show many of the typical features of other climate change scenarios, including those associated with stronger climatic forcings. That are a pronounced warming, particularly at high latitudes accompanied by a marked reduction of the sea-ice cover, a substantial increase in precipitation in the tropics as well as at mid- and high latitudes in both hemispheres but a marked reduction in the subtropics, a significant strengthening of the meridional temperature gradient between the tropical upper troposphere and the lower stratosphere in the extratropics accompanied by a pronounced intensification of the westerly winds in the lower stratosphere, and a strengthening of the westerly winds in the Southern Hemisphere extratropics throughout the troposphere. The magnitudes of these changes, however, are somewhat weaker than for the scenarios associated with stronger global warming due to stronger climatic forcings, such as the SRES A1B scenario. Some of the climatic changes associated with the 2°C-stabilization are relatively strong with respect to the magnitude of the simulated global warming, i.e., the pronounced warming and sea-ice reduction in the Arctic region, the strengthening of the meridional temperature gradient at the northern high latitudes and the general increase in precipitation. Other climatic changes, i.e., the El Niño like warming pattern in the tropical Pacific Ocean and the corresponding changes in the distribution of precipitation in the tropics and in the Southern Oscillation, are not as markedly pronounced as for the scenarios with a stronger global warming. A higher anthropogenic sulphate aerosol load (for 2030 as compared to the level in 2100 according to the SRES A1B scenario) generally weakens the future changes in climate, particularly for precipitation. The most pronounced effects occur in the Northern Hemisphere and in the tropics, where also the main sources of anthropogenic sulphate aerosols are located.     

The Impacts of Two Types of El Ni（n）o on Global Ozone Variations in the Last Three Decades

The effects of E1Nifio Modoki events on global ozone concentrations are investigated from 1980 to 2010 E1 Nifio Modoki events cause a stronger Brewer-Dobson （BD） circulation which can transports more ozone-poor air from the troposphere to stratosphere, leading to a decrease of ozone inthe lower-middle stratosphere from 90~S to 90~N. These changes in ozone concentrations reduce stratospheric column ozone. The reduction in stratospheric column ozone during E1 Nifio Modoki events is more pronounced over the tropical eastern Pacific than over other tropical areas because transport of ozone-poor air from middle-high latitudes in both hemispheres to low latitudes is the strongest between 60°W and 120°W. Because of the decrease in stratospheric column ozone during E1 Nifio Modoki events more UV radiation reaches the tropical troposphere leading to significant increases in tropospheric column ozone An empirical orthogonal function （EOF） analysis of the time series from 1980 to 2010 of stratospheric and tropospheric ozone monthly anomalies reveals that： E1 Nifio Modoki events are associated with the primary EOF modes of both time series. We also found that E1 Nifio Modoki events can affect global ozone more significantly than canonical E1 Nifio events. These results imply that E1 Nifio Modoki is a key contributor to variations in global ozone from 1980 to 2010.     

平流层爆发性增温及其影响研究进展

平流层爆发性增温(stratospheric sudden warming,SSW)是冬季平流层大气环流结构的一种突变现象,在短时间内平流层中高纬度的温度、风和极涡都会发生剧烈变化。因此,SSW也就成为平流层大气环流及其变化研究的重要方面之一。在强SSW期间,高纬地区温度急剧升高,西风被东风取代,极涡几乎全部崩溃。SSW极大地影响着北半球对流层大气,甚至整个中高层大气,包括对平流层乃至中层大气微量气体分布的重要影响。随着临近空间飞行平台的研究应用,以及由此而提出的临近空间环境条件的保障问题,作为临近空间重要组成部分的平流层环流变化将更加引起人们的关注。本文就SSW的特征、发生机制、对上下层相互作用的重要影响,以及SSW与准两年振荡、ENSO等的密切关系和SSW的数值模拟等方面的研究工作,进行了回顾和总结。     

CFSv2 prediction skill of stratospheric temperature anomalies

This study evaluates the prediction skill of stratospheric temperature anomalies by the Climate Forecast System version 2 (CFSv2) reforecasts for the 12-year period from January 1, 1999 to December 2010. The goal is to explore if the CFSv2 forecasts for the stratosphere would remain skillful beyond the inherent tropospheric predictability time scale of at most 2 weeks. The anomaly correlation between observations and forecasts for temperature field at 50 hPa (T50) in winter seasons remains above 0.3 over the polar stratosphere out to a lead time of 28 days whereas its counterpart in the troposphere at 500 hPa drops more quickly and falls below the 0.3 level after 12 days. We further show that the CFSv2 has a high prediction skill in the stratosphere both in an absolute sense and in terms of gain over persistence except in the equatorial region where the skill would mainly come from persistence of the quasi-biennial oscillation signal. We present evidence showing that the CFSv2 forecasts can capture both timing and amplitude of wave activities in the extratropical stratosphere at a lead time longer than 30 days. Based on the mass circulation theory, we conjecture that as long as the westward tilting of planetary waves in the stratosphere and their overall amplitude can be captured, the CFSv2 forecasts is still very skillful in predicting zonal mean anomalies even though it cannot predict the exact locations of planetary waves and their spatial scales. This explains why the CFSv2 has a high skill for the first EOF mode of T50, the intraseasonal variability of the annular mode while its skill degrades rapidly for higher EOF modes associated with stationary waves. This also explains why the CFSv2’s skill closely follows the seasonality and its interannual variability of the meridional mass circulation and stratosphere polar vortex. In particular, the CFSv2 is capable of predicting mid-winter polar stratosphere warming events in the Northern Hemisphere and the timing of the final polar stratosphere warming in spring in both hemispheres 3–4 weeks in advance.     

Long-Term Ozone Changes Over the Northern Hemisphere Mid-Latitudes for the 1979–2012 Period

Abstract

The solar backscattered ultraviolet (SBUV/SBUV-2) merged ozone datasets, version 8.6, including column ozone and ozone profiles for the 1979–2012 period are examined for the 35°N–60°N zonal belt in the northern hemisphere mid-latitudes and four sub-regions: central Europe, continental Europe, North America, and East Asia. The residual long-term patterns for total ozone and ozone profiles are extracted by smoothing the time series of differences between the original and the modelled ozone time series. Modelled ozone is obtained using the standard trend model accounting for ozone variability due to changes in stratospheric halogens and various dynamical factors commonly used in previous ozone trend analyses. Since about 2005 spring and summer total ozone in the troposphere and lower stratosphere has decreased in some regions (central and continental Europe, North America, and the 35°N–60°N zonal belt) compared with modelled ozone. The negative departure from modelled ozone in 2010 is approximately 2–3% of the overall 1979–2012 monthly mean level. It seems that this decrease is a result of yet unknown dynamical processes rather than to chemical destruction because the differences have a longitudinal structure, and total ozone in the upper stratosphere still follows changes in stratospheric halogen loading.     

Connection of the stratospheric QBO with global atmospheric general circulation and tropical SST. Part II: interdecadal variations

The interdecadal variation of the association of the stratospheric quasi-biennial oscillation (QBO) with tropical sea surface temperature (SST) anomalies (SSTA) and with the general circulation in the troposphere and lower stratosphere is examined using the ERA40 and NCEP/NCAR reanalyses, as well as other observation-based analyses. It is found that the relationship between the QBO and tropical SSTA changed once around 1978–1980, and again in 1993–1995. During 1966–1974, negative correlation between the QBO and NINO3.4 indices reached its maximum when the NINO3.4 index lagged the QBO by less than 6?months. Correspondingly, the positive correlations were observed when the NINO3.4 index led the QBO by about 11–13?months or lagged by about 12–18?months. However, maximum negative correlations were shifted from the NINO3.4 index lagging the QBO by about 0–6?months during 1966–1974 to about 3–12?months during 1985–1992. During 1975–1979, both the negative and positive correlations were relatively small and the QBO and ENSO were practically unrelated to each other. The phase-based QBO life cycle composites also confirm that, on average, there are two phase (6–7?months) delay in the evolution of the QBO-associated anomalous Walker circulation, tropical SST, atmospheric stability, and troposphere and lower stratosphere temperature anomalies during 1980–1994 in comparison with those in 1957–1978. The interdecadal variation of the association between the QBO and the troposphere variability may be largely due to the characteristic change of El Ni?o-Southern Oscillation. The irregularity of the QBO may play a secondary role in the interdecadal variation of the association.     

北半球准定常行星波气候平均态的资料分析和数值模拟

利用NCEP/NCAR再分析资料和大气环流模式(CCSR/NIES AGCM Ver 5.6),对北半球准定常行星波的气候平均态分布进行分析和模拟.再分析资料分析的结果表明:北半球冬季,准定常行星波沿两支波导向上传播,其中一支在对流层上层转向中低纬度传播,另外一支折向高纬度,通过极地波导上传到平流层.其中,1波和2波可以上传到平流层,因而其振幅分布除在中低纬的对流层上层出现一个次大值外,在高纬度平流层中上层会出现一个最大值,3波则主要限制在对流层,其振幅分布除在副热带对流层上层出现一个次大值外,最大值出现在中纬度对流层上层.北半球夏季,整个平流层为东风环流,极地波导不存在,行星波不能上传到平流层,在对流层活动也较弱,1波、2波、3波的传播情况大致相似,表现为在对流层上层由中纬度向赤道地区的传播.相应的振幅分布是,对1波和2波而言,最大值出现在中低纬对流层顶附近,同时在中高纬对流层上层出现一个次大值,而3波的振幅分布正好相反,最大值出现在中高纬对流层上层,次大值则在中低纬对流层顶附近.利用大气环流模式进行的数值模拟表明,模式可以比较好地模拟冬夏季准定常行星波的传播路径,但模拟的北半球冬季沿极地波导向平流层的传播明显偏弱,其结果是对1波、2波而言,高纬度平流层中上层的振幅最大值明显小于再分析资料的数值.文中还讨论了数值模拟与资料分析中行星波的差异可能对大气环流模拟的影响.     

A two-way stratosphere-troposphere coupling of submonthly zonal-mean circulations in the Arctic

This paper examines the dominant submonthly variability of zonally symmetrical atmospheric circula- tion in the Northern Hemisphere （NH） winter within the context of the Northern Annular Mode （NAM）, with particular emphasis on interactive stratosphere-troposphere processes. The submonthly variability is identified and measured using a daily NAM index, which concentrates primarily on zonally symmetrical circulation. A schematic lifecycle of submonthly variability is developed that reveals a two-way coupling pro- cess between the stratosphere and troposphere in the NH polar region. Specifically, anomalous tropospheric zonal winds in the Atlantic and Pacific sectors of the Arctic propagate upwards to the low stratosphere, disturbing the polar vortex, and resulting in an anomalous stratospheric geopotential height （HGT） that subsequently propagates down into the troposphere and changes the sign of the surface circulations. From the standpoint of planetary-scale wave activities, a feedback loop is also evident when the anoma- lous planetary-scale waves （with wavenumbers 2 and 3） propagate upwards, which disturbs the anomalous zonally symmetrical flow in the low stratosphere, and induces the anomalous HGT to move poleward in the low stratosphere, and then propagates down into the troposphere. This increases the energy of waves at wavenumbers 2 and 3 in the low troposphere in middle latitudes by enhancing the land-sea contrast of the anomalous HGT field. Thus, this study supports the viewpoint that the downward propagation of stratospheric NAM signals may not originate in the stratosphere.     

Diurnal variations of winds over an upwelling region off Oregon

The diurnal variation of surface winds off the coast of Oregon is described and compared with a recent analysis of winds off the coast of Peru. The Oregon wind speeds have a distinct 24-h periodicity, while the Peru wind speeds were reported to have an irregular 12-h variation. The long-and trans-shore components of both winds exhibit 24-h periodicities; the ratio of the long-shore to trans-shore diurnal amplitudes off Oregon is 2.8, twice the ratio found off Peru. Although meteorological conditions off Oregon were quasi-stationary during the period investigated, there were considerable day-to-day variations in diurnal amplitudes and phases. Diurnal amplitudes were found to be correlated with the daily mean long-shore winds.     

2007/2008和2008/2009冬季平流层强、弱极涡事件对应的行星波活动的对比分析

在对逐日气象资料进行纬向谐波分析的基础上, 对比和讨论了2007/2008年冬季强极涡期间和2008/2009冬季弱极涡期间平流层和对流层不同波数的行星波的变化特征, 特别关注强极涡或弱极涡发生之后, 500 hPa 沿60°N和30°N行星波1波和2波振幅和位相的差异, 以及相应的500 hPa位势场的差异, 进而讨论为什么不同的平流层极涡异常会对东亚有不同的影响, 特别讨论为什么同一种极涡异常, 对我国南北方近地面气温的影响会不同。结果表明:平流层极涡发生异常时, 平流层行星波活动有明显的异常。随着极涡异常的下传, 对流层行星波的振幅和位相也有明显的变化, 而且, 对于不同的纬度带, 其变化又有不同, 表现为:2008年1月强极涡发生之后, 500 hPa行星波1波和2波的扰动都向南伸, 而2009年1月的弱极涡(SSW)期间和之后, 1波和2波的扰动都偏北; 在对流层, 强极涡和弱极涡发生之后不但行星波1波和2波的振幅有所差异, 其位相也有明显的不同。特别是, 其位相的差异还随纬度而变化。就同一年(或者说对于同是强极涡或者同是弱极涡)而言, 无论是1波还是2波, 在60°N和30°N附近的扰动相比, 几乎反位相。这样就使得它们的500 hPa 位势场也有明显不同:在东半球, 主要表现为乌拉尔高压和东亚大槽的强度和位置不同。2008年1月强极涡发生之后, 乌拉尔高压和东亚大槽东移, 不利于冷空气向欧亚大陆北部(包括我国北方)的输送, 使这些地区的温度偏高;而2009年1月弱极涡之后, 东亚大槽西退, 利于冷空气向欧亚大陆北部输送, 导致这些地区较冷。对于同一种极涡异常(如2008强极涡或者2009弱极涡)由于南方和北方行星波扰动的位相不同, 对南方和北方冷暖空气的输送也就不一样。所以同一种极涡异常对(我国)南北地区的温度影响是不同的。     

亚洲东部冬季地面温度变化与平流层弱极涡的关系

利用NCEP资料计算NAM指数和标准化温度距平,对17次平流层弱极涡事件时亚洲东部温度变化进行了研究。结果表明:平流层环流异常比对流层温度变化超前约15天,地面温度变化的最大距平出现在平流层弱极涡后期,大约以40°N为界,北部比正常年份偏冷而南部偏暖。文中通过位势涡度的分布和变化以及500 hPa东亚大槽的变化讨论了其影响过程和机理,在弱极涡初期和中期,自平流层向下,高位涡冷空气主要局限于60°N以北。从弱极涡的后期开始,在45°N以北地区,高位涡冷空气向南扩张,在对流层中上层,极地附近的高位涡冷空气扩张到45°N附近。同时,500 hPa东亚大槽虽有加强,但低压区向东延伸,而贝加尔湖附近的高压脊显著减弱,致使槽后的偏北气流减弱,槽后冷空气主要影响中国华北、东北及其以北地区,造成这些地区偏冷。而40°N以南地区,从弱极涡的后期开始有南方低位涡偏暖空气向北运动,同时冷空气活动减少,地面显著偏暖。     

2019年4月广州白云机场持续暴雨前对流层顶和平流层异常信号分析

利用欧洲中心ERA5再分析资料和广州白云机场自动观测系统降水资料,分析2019年4月白云机场持续暴雨前对流层顶和平流层的信号特征。分析发现,2019年4月中下旬,广州白云机场出现了3次持续时间长、降水量大的持续性暴雨过程,降水较往年同期显著偏多。研究结果表明,3次持续暴雨发生前,对流层顶高度出现了下降,平流层高位涡冷空气入侵,机场上空位涡升高;在环流场中,中低纬地区对流层顶和平流层东风偏强,向北和向下传播,广州白云机场终端区在暴雨发生前西风持续下传;广州白云机场上空暴雨发生前对流层顶至平流层位势高度正异常。暴雨发生前,平流层冷空气高位涡移入、对流层顶下降、西风的下传均有利于持续性暴雨的生成。     

Observational Subseasonal Variability of the PM2.5 Concentration in the Beijing-Tianjin-Hebei Area during the January 2021 Sudden Stratospheric Warming

It is still not well understood if subseasonal variability of the local PM_2.5 in the Beijing-Tianjin-Hebei (BTH) region is affected by the stratospheric state. Using PM_2.5 observations and the ERA5 reanalysis, the evolution of the air quality in BTH during the January 2021 sudden stratospheric warming (SSW) is explored. The subseasonal variability of the PM_2.5 concentration after the SSW onset is evidently enhanced. Stratospheric circumpolar easterly anomalies lasted for 53 days during the January–February 2021 SSW with two evident stratospheric pulses arriving at the ground. During the tropospheric wave weakening period and the intermittent period of dormant stratospheric pulses, the East Asian winter monsoon weakened, anomalous temperature inversion developed in the lower troposphere, anomalous surface southerlies prevailed, atmospheric moisture increased, and the boundary layer top height lowered, all of which favor the accumulation of pollutant particulates, leading to two periods of pollution processes in the BTH region. In the phase of strengthened East Asian winter monsoon around the very beginning of the SSW and another two periods when stratospheric pulses had reached the near surface, opposite-signed circulation patterns and meteorological conditions were observed, which helped to dilute and diffuse air pollutants in the BTH region. As a result, the air quality was excellent during the two periods when the stratospheric pulse had reached the near surface. The increased subseasonal variation of the regional pollutant particulates after the SSW onset highlights the important role of the stratosphere in the regional environment and provides implications for the environmental prediction.     

热带加热异常影响冬季平流层极涡强度的数值模拟

本文利用大气环流模式SAMIL/LASG,通过选择两种对流参数化方案,研究了热带加热异常对热带外平流层模拟的影响。结果表明,因不同对流参数化方案引起的热带对流加热状况的差异,可显著影响模式对北半球冬季平流层极涡强度的模拟偏差。与采用Manabe对流参数化方案相比,采用Tiedtke参数化方案可以显著改善对平流层极涡强度的模拟,使平流层极涡“过强”及极区“过冷”的模拟偏差得到明显改善。研究其中的影响过程发现,由于Manabe方案最大凝结潜热加热高度过低,在对流层中低层;而Tiedtke方案的最大凝结潜热加热位置在对流层中上层,因而Tiedtke(Manabe)方案时热带大气温度在对流层中上层较为偏暖(偏冷),在平流层低层较为偏冷(偏暖)。自秋季开始,与热带对流层高层温度的暖偏差相联系,热带外对流层高层以及热带平流层低层出现伴随的温度冷偏差;与之对应,平流层中纬度从秋季开始也出现持续的温度暖偏差。另外,随着秋冬季节平流层行星波活动的出现,Tiedtke方案时热带外地区行星波1波的强度也明显强于Manabe方案,使得秋冬季节涡动引起的向极热通量在Tiedtke方案时明显偏强,从而造成了冬季平流层极区温度偏暖、极涡强度偏弱。     

Global warming mitigation by sulphur loading in the stratosphere: dependence of required emissions on allowable residual warming rate

An approach to mitigate global warming via sulphur loading in the stratosphere (geoengineering) is studied, employing a large ensemble of numerical experiments with the climate model of intermediate complexity IAP RAS CM. The model is forced by the historical+SRES A1B anthropogenic greenhouse gases+tropospheric sulphates scenario for 1860–2100 with additional sulphur emissions in the stratosphere in the twenty-first century. Different ensemble members are constructed by varying values of the parameters governing mass, horizontal distribution and radiative forcing of the stratospheric sulphates. It is obtained that, given a global loading of the sulphates in the stratosphere, among those studied in this paper latitudinal distributions of geoengineering aerosols, the most efficient one at the global basis is that peaked between 50°N and 70°N and with a somewhat smaller burden in the tropics. Uniform latitudinal distribution of stratospheric sulphates is a little less efficient. Sulphur emissions in the stratosphere required to stop the global temperature at the level corresponding to the mean value for 2000–2010 amount to more than 10 TgS/year in the year 2100. These emissions may be reduced if some warming is allowed to occur in the twenty-first century. For instance, if the global temperature trend S _g in every decade of this century is limited not to exceed 0.10 K/decade (0.15 K/decade), geoengineering emissions of 4–14 TgS/year (2–7 TgS/year) would be sufficient. Even if the global warming is stopped, temperature changes in different regions still occur with a magnitude up to 1 K. Their horizontal pattern depends on implied latitudinal distribution of stratospheric sulphates. In addition, for the stabilised global mean surface air temperature, global precipitation decreases by about 10%. If geoengineering emissions are stopped after several decades of implementation, their climatic effect is removed within a few decades. In this period, surface air temperature may grow with a rate of several Kelvins per decade. The results obtained with the IAP RAS CM are further interpreted employing a globally averaged energy–balance climate model. With the latter model, an analytical estimate for sulphate aerosol emissions in the stratosphere required climate mitigation is obtained. It is shown that effective vertical localisation of the imposed radiative forcing is important for geoengineering efficiency.