沙尘表面非均相化学过程的气候效应的初步模拟研究

建立了一个包含地表起尘机制的尘粒表面非均相化学模式, 并与区域气候——大气化学模式系统连接. 研究了沙尘气溶胶表面的非均相过程对大气中一些重要微量成分浓度的影响及其所产生的气候效应. 结果表明,非均相过程使得二氧化硫和臭氧的浓度降低,硫酸盐浓度增加,年平均硫酸盐积分浓度增加26mg/m2;在部分地区非均相过程使二氧化氮浓度降低,而在另外一些地区,则使二氧化氮浓度增加. 1,4,7,10月四个月硫酸盐浓度增加造成的辐射强迫最大值分别为-0.24,-1.0,-2.0,-0.6 W/m2,全区域年平均辐射强迫为-0.033 W/m2. 四个月最大降温分别可达0.16,0.35,0.5,0.48K,年平均降温0.021K. 非均相过程对月总降水亦有明显的影响.     

大气模式估算的东亚区域人为硫酸盐和黑碳气溶胶辐射强迫及其时间变化特征

本文利用大气环流模式及大气化学模式所得气溶胶资料,估算了相对1850s时期硫酸盐和黑碳气溶胶引起的全球及东亚区域人为辐射强迫,重点分析其在东亚区域的季节和长期变化特征.结果表明,就当前全球年平均全天空而言,人为硫酸盐气溶胶对大气顶的直接和云反照率强迫分别为-0.37和-0.98 W·m-2,黑碳气溶胶对大气顶和整层大气的辐射强迫值为0.16和0.47 W·m-2;中国东部区域是目前上述气溶胶辐射强迫最强的区域,硫酸盐的直接和间接辐射强迫分别超过-2.0和-4.0 W·m-2,黑碳对大气顶和整层大气的直接辐射强迫分别可达2.0和5.0W·m-2;估算的东亚区域上述气溶胶辐射强迫仍在不断增强,峰值预计出现在2010s时段,而且中国东部较强的辐射强迫还可能维持至2030s左右;在未来中、高排放情景下,东亚区域以上两种气溶胶预计对全球气溶胶辐射强迫有更大的贡献.分析还表明,夏季东亚区域较强的水汽会增强吸湿性硫酸盐气溶胶的光学厚度和晴空直接辐射强迫;云的作用一方面会强化东亚区域全天空条件下大气顶黑碳的辐射强迫,另一方面会影响硫酸盐气溶胶间接云反照率强迫的季节变化;上述气候特征的差异使得东亚区域的气溶胶辐射强迫表现出与欧美区域有所不同的特征.本文所用的气溶胶资料与模式气象场的偏差会给气溶胶辐射强迫计算带来一些不确定性,进一步改进气候模式中气溶胶过程、水汽和云等气象场的模拟将有助于获得更为合理的区域气溶胶辐射强迫估算结果.     

中国不同排放情景下人为气溶胶的气候效应

本文利用区域气候模式RIEMS2.0(Regional Integrated Environmental Model System)和2006年以及2020年三种排放情景下的排放资料,研究了2006年气候背景下的人为气溶胶的浓度分布特征及辐射效应,估算了未来不同排放情景下人为气溶胶的主要成分硫酸盐、硝酸盐、黑碳、有机碳(含二次有机碳)的综合气候效应.结果表明:(1)2006年中国地区人为气溶胶浓度硫酸盐>有机碳>硝酸盐>黑碳,其区域柱浓度平均值分别为6.0、4.0、1.3和0.3 mg/m².(2)2006年硫酸盐、硝酸盐、有机碳和黑碳的平均辐射强迫分别为-1.32、-0.60、-0.40和0.28 W/m².硫酸盐、硝酸盐和有机碳的负辐射强迫超过黑碳的正辐射强迫,人为气溶胶总辐射强迫为-1.96 W/m².(3)人为气溶胶的辐射效应及引起的地面气温变化对排放源非常敏感,未来采取不同排放政策导致的人为气溶胶的含量及辐射效应有较大差异.在未来排放增加的情景下,各区域的气溶胶浓度、辐射强迫、气温下降幅度和降水减少幅度也相应加大.     

水合物合成及导热系数测定

设计了一套实验装置，结合瞬态面热源法来测量混合气水合物导热系数及含混气水合物的沙子多孔介质的有效导热系数.在-10℃～5℃，压力66MPa下，含体积比甲烷9001%，乙烷503%，丙烷496%的混合气与0971mol/m3十二烷基磺酸钠水溶液生成的水合物的导热系数约为055W/(m·K)，并且其值随温度的上升而增高，呈玻璃体导热特性.由于“爬壁”效应的存在，混合气与饱含SDS水溶液的沙子多孔介质反应生成含混合气水合物的沙子多孔介质的有效导热系数（约12W/(m·K)）显著低于含四氢呋喃水合物的沙子多孔介质的值（约19W/(m·K)）.虽然本实验使用了SDS来加速和促进水合反应的进行，但是水合物样品中依然存在游离水，因此本研究采用了温度振荡法来进一步促进含SDS水溶液的水合反应进行，研究发现当浴槽温度在-10℃～4℃间周期变化时，游离水在水的相变温度区附近转变为水合物，通过几个周期的温度振荡，样品中的游离水被完全消耗掉.最后通过对含不同浓度SDS的四氢呋喃水合物导热系数测试，讨论了实验中加入SDS对水合物导热系数的影响，结果认为本实验中加入的SDS量对测试结果影响很小（±15%）.     

中国大陆科学钻探主孔动态地温测量

介绍了大陆科学钻探主孔完钻后4次的钻井测温数据,地温梯度随深度的变化趋势,系统的热导率测试结果及其温压校正. 地温测量显示,浅部（100m以上）的4次测量结果有较大的区别,而100m以下测量温度趋于一致.在900～1600m井段,温度略有波动,可能存在地下水活动.到了深部,温度与深度呈现良好的线性关系. 在0～500m,500～2700m,2700～3600m及3600m以下这4个井段范围内,地温梯度随深度降低或增加的趋势交替变化,平均地温梯度248±34℃/km. 198块岩芯样品测试结果表明,热导率变化范围在1711～36 W/(m·K),平均2716±0403 W/(m·K). 依据实测的温度-深度进行温压校正后,热导率为1989～3652 W/(m·K),平均2808±0363 W/（m·K）. 热导率随深度的变化趋势与地温梯度的变化趋势并不能完全相互补偿,表明影响地温梯度的其他因素不容忽视. 大陆科学钻探温度测量,为今后进一步研究超高压变质带深部地热场及其地球动力学含义提供了可靠的基础数据.     

夏季中国西部地区辐射特征的观测分析和能量收支的模式计算

在2000年6-7月新疆阜康地区野外观测资料和美国宇航局Goddard地球观测系统资料同化系统计算相应时间能量收支基础上分析了夏季我国西部干旱地区辐射特征和能量收支.新疆阜康地区观测的夏季中午平均吸收辐射为664 W/m2左右,反照率为17%,夜间长波净辐射值为60W/m2左右.模式计算的相应地区的辐射特征与观测结果相当接近.模式计算结果表明,夏季新疆、甘肃西部、内蒙一带为感热通量高值区,其最大值在华北、东北地区,其值可达300W/m2.广大西北地区潜热通量都很低,其高值区在华东、华南、西藏东部和四川一带,最大值可达250-300W/m2.     

青藏高原一次地闪放电过程的分析

利用成像率为1000 幅/s的高速摄像系统和快、慢电场变化仪以及宽带干涉仪系统等探测仪器在青藏高原那曲地区所观测的地闪资料,对一次地闪回击及其之前的持续时间较长的云内放电过程进行了分析.结果表明：地闪先导前的云内放电过程发生于雷暴云下部正电荷区和中部负电荷区之间;云中部负电荷区距离地面的高度为28～45 km;闪电的起始放电发生区域距离地面的高度为10～17 km;初始流光在云外发展时具有很大的水平分量和较多的分支;梯级先导的速度为1×105 m/s,在向地面发展时出现较大的弯曲;首次回击放电过程与低海拔地区没有差异,通道中的峰值电流有241 kA;继后回击相对较弱.     

青藏高原班公湖－怒江缝合带域岩石密度结构及意义

班公湖-怒江缝合带分隔了青藏高原拉萨地块和羌塘地块, 该带域岩样采集与分析对于该区地球物理资料深化解释、拉萨地块和羌塘地块拼贴碰撞过程的理解等均具有重要意义. 1995年在措勤盆地中采集了3条剖面、从奥陶纪至第四系不同地质年代地层岩石标本共计2500块. 通过岩石密度测试, 获得了研究区不同地质年代岩石密度测量结果. 结果表明, 岩石由老到新密度变化范围为278～253 g/cm3；各相邻地质时代间岩石密度差基本上为010 g/cm3, 白垩与侏罗、二叠与三叠之间岩石密度差最大为012～013 g/cm3 在措勤盆地内不同构造单元间岩石密度存在明显的纵横向非均一性.     

一个新的双向反射地表-大气辐射耦合模式

一个精确而又适用的双向反射地表-大气辐射耦合模式对空间遥感应用是非常重要的. 基于太阳辐射与地表和大气相互作用的物理过程, 发展了一个新的双向反射地表-大气辐射耦合模式. 如数值试验所表明的, 本模式的精度明显优于6S的双向反射地表-大气辐射耦合模式. 由本模式计算的总共110112组亮度样本的标准差只有0.49%, 只为6S标准差的1/4左右. 在太阳天顶角小于75symbol 176 \f "Symbol" \s 10皚和视天顶角小于60°条件下, 本模式的误差一般小于2.5%.     

沁水盆地大地热流与地温场特征

分析了20口井的温度数据和39个岩石样品的热导率数据,计算了20个大地热流值.结果表明：沁水盆地具有偏高的大地热流背景,现今热流变化于448～1018 mW/m2之间,平均627±152 mW/m2,现今地温梯度介于209～476 ℃/km之间,平均地温梯度282±103 ℃/km. 热流的分布与本区上、下主煤层含气量的分布特征相似,在一定程度上反映了现代热流继承了煤层气生气期的古地热背景.     

Spatio-temporal characteristics of aerosol distribution over Tibetan Plateau and numerical simulation of radiative forcing and climate response

In this paper we have analyzed aerosol distribution over the Tibetan Plateau by using the global monthly mean satellite data of Stratospheric Aerosol and Gas Experiment II (SAGE II). The results are as follows: (1) Stratospheric aerosol optical depth can oscillate in the four seasons. It means that the aerosol optical depth is the thickest in winter and a little thinner in spring and the thinnest in summer and then a little thicker in autumn. We have found that the oscillation is caused by the oscillation of tropopause in different seasons. (2) Stratospheric aerosol comes mainly from sprays of volcano. After eruption of Mount Pinatubo aerosol optical depth in stratosphere over the Tibetan Plateau increases 10 times compared with before. (3) The characteristic of aerosol vertical distribution over the Tibetan Plateau is that there is an extremely high value at the altitude of 70 hPa. The most interesting thing is that the extremely high value can oscillate between 50 hPa and 100 hPa. We have verified that the oscillation is a unique characteristic over the Tibetan Plateau by comparing it with South China and North China. Then the radiative forcing and regional climate response over the Tibetan Plateau of aerosol are investigated. We have discovered such things as followed by: (1) The radiative forcing is positive because the parameterized aerosol optical depth is less than 0.14 which is the optical depth of the uniform background boundary aerosol layer. It is 0–3 W/m² in January and 0–4 W/m² in April and less than 3 W/m² in July and 3–6 W/m² in October. (2) Ground temperature rises 0.1–0.2 K in October which is the biggest increasing magnitude, and 0.01–0.02 in July which is the smallest one. It rises about 0.05-0.01 K in January and April. (3) Air temperature near the earth’s surface and the one at the altitude of 500 hPa rise too, but the increasing magnitude is less than the former one.

     

Persistent, Widespread, and Strongly Absorbing Haze Over the Himalayan Foothills and the Indo-Gangetic Plains

We examine the impact of the Atmospheric Brown Clouds on the direct radiative forcing of the Himalayan foothills and the Indo-Gangetic Plains (IGP) regions, home for over 500 million S. Asians. The NASA-Terra MODIS satellite data reveal an extensive layer of aerosols covering the entire IGP and Himalayan foothills region with seasonal mean AODs of about 0.4 to 0.5 in the visible wavelengths (0.55 micron), which fall among the largest seasonal mean dry season AODs for the tropics. We show new surface data which reveal the presence of strongly absorbing aerosols that lead to a large reduction in solar radiation fluxes at the surface during the October to May period. The three-year mean (2001 to 2003) October to May seasonal and diurnal average reduction in surface solar radiation for the IGP region is about 32 (±5) W m⁻² (about 10% of TOA insolation or 20% of surface insolation). The forcing efficiency (forcing per unit optical depth) is as large as −27% (note that the forcing is negative) of top-of-atmosphere (TOA) solar insolation, and exceeds the forcing efficiency that has been observed for other polluted regions in America, Africa, East Asia, and Europe. General circulation model sensitivity studies suggest that both the local and remote influence of the aerosol induced radiative forcing is to strengthen the lower atmosphere inversion, stabilize the boundary layer, amplify the climatological tendency for a drier troposphere, and decrease evaporation. These aerosol-induced changes could potentially increase the life times of aerosols, make them more persistent, and decrease their single scattering albedos, thus potentially leading to a detrimental positive feedback between aerosol concentrations, aerosol forcing, and aerosol persistence. In addition, both the model studies and observations of pan evaporation suggest that the reduction in surface solar radiation may have led to a reduction in surface evaporation of moisture. These results suggest the vulnerability of this vital region to air pollution related direct and indirect (through climate changes) impacts on agricultural productivity of the region.     

Comparison of dust emissions,transport, and deposition between the Taklimakan Desert and Gobi Desert from 2007 to 2011

The Taklimakan Desert(TD) and Gobi Desert(GD) are two of the most important dust sources in East Asia, and have important impact on energy budgets, ecosystems and water cycles at regional and even global scales. To investigate the contribution of the TD and the GD to dust concentrations in East Asia as a whole, dust emissions, transport, and deposition over the TD and the GD in different seasons from 2007 to 2011 were systematically compared, based on the Weather Research and Forecasting model coupled with Chemistry(WRF-Chem). Dust emissions, uplift, and long-range transport related to these two dust source regions were markedly different due to differences in topography, elevation, thermal conditions, and atmospheric circulation. Specifically,the topography of the GD is relatively flat, and at a high elevation, and the area is under the influence of two jet streams at high altitudes, resulting in high wind speeds in the upper atmosphere. Deep convective mixing enables the descending branch of jet streams to continuously transport momentum downward to the mid-troposphere, leading to enhanced wind speeds in the lower troposphere over the GD which favors the vertical uplift of the GD dust particles. Therefore, the GD dust was very likely to be transported under the effect of strong westerly jets, and thus played the most important role in contributing to dust concentrations in East Asia. Approximately 35% and 31% of dust emitted from the GD transported to remote areas in East Asia in spring and summer, respectively. The TD has the highest dust emission capabilities in East Asia, with emissions of about 70.54 Tg yr.1 in spring, accounting for 42% of the total dust emissions in East Asia. However, the TD is located in the Tarim Basin and surrounded by mountains on three sides. Furthermore, the dominant surface wind direction is eastward and the average wind speed at high altitudes is relatively small over the TD. As a result, the TD dust particles are not easily transported outside the Tarim Basin, such that most of the dust particles are re-deposited after uplift, at a total deposition rate of about 40 g m.2. It is only when the TD dust particles are uplifted above 4 km, and entrained in westerlies that they begin to undergo a long-range transport. Therefore,the contribution of the TD dust to East Asian dust concentrations was relatively small. Only 25% and 23% of the TD dust was transported to remote areas over East Asia in spring and summer, respectively.     

辽河盆地东部凹陷现今地温场及热历史的研究

依据10口系统测温井数据和61块岩石热导率测试结果，计算了辽河盆地东部凹陷10个 高质量的大地热流数据，并在此基础上，利用镜质体反射率（Ro）资料对该区的热历史 进行了恢复. 结果表明：东部凹陷下第三系平均地温梯度为36.5℃/km，岩石平均热导率为1 .667W/(m·K)，热流密度变化于49.5～70.0mW/m2之间，平均为58.0mW/m2；东部凹陷热 流呈现古热流高现今热流低的变化特征，从沙三期到东营期，古热流值是逐渐增大的，到东 营期末达到最大值，晚第三纪至现今表现为持续冷却；构造沉降史分析显示，盆地经历了早 期的裂谷阶段（43～25Ma）和后期的热沉降阶段. 盆地现今较低的大地热流和较高的古热流 及典型的裂谷型构造沉降样式为东部凹陷的构造-热演化提供了重要认识.     

Regional variability in dust‐on‐snow processes and impacts in the Upper Colorado River Basin

Dust deposition onto mountain snow cover in the Upper Colorado River Basin frequently occurs in the spring when wind speeds and dust emission peaks on the nearby Colorado Plateau. Dust loading has increased since the intensive settlement in the western USA in the mid 1880s. The effects of dust‐on‐snow have been well studied at Senator Beck Basin Study Area (SBBSA) in the San Juan Mountains, CO, the first high‐altitude area of contact for predominantly southwesterly winds transporting dust from the southern Colorado Plateau. To capture variability in dust transport from the broader Colorado Plateau and dust deposition across a larger area of the Colorado River water sources, an additional study plot was established in 2009 on Grand Mesa, 150 km to the north of SBBSA in west central, CO. Here, we compare the 4‐year (2010–2013) dust source, deposition, and radiative forcing records at Grand Mesa Study Plot (GMSP) and Swamp Angel Study Plot (SASP), SBBSA's subalpine study plot. The study plots have similar site elevations/environments and differ mainly in the amount of dust deposited and ensuing impacts. At SASP, end of year dust concentrations ranged from 0.83 mg g^?1 to 4.80 mg g^?1, and daily mean spring dust radiative forcing ranged from 50–65 W m^?2, advancing melt by 24–49 days. At GMSP, which received 1.0 mg g^?1 less dust per season on average, spring radiative forcings of 32–50 W m^?2 advanced melt by 15–30 days. Remote sensing imagery showed that observed dust events were frequently associated with dust emission from the southern Colorado Plateau. Dust from these sources generally passed south of GMSP, and back trajectory footprints modelled for observed dust events were commonly more westerly and northerly for GMSP relative to SASP. These factors suggest that although the southern Colorado Plateau contains important dust sources, dust contributions from other dust sources contribute to dust loading in this region, and likely account for the majority of dust loading at GMSP. Copyright © 2015 John Wiley & Sons, Ltd.