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991.
R. G. Derwent W. J. Collins M. E. Jenkin C. E. Johnson D. S. Stevenson 《Journal of Atmospheric Chemistry》2003,44(1):57-95
A global 3-D Lagrangian chemistry-transport model STOCHEM is used to describe the tropospheric distributions of four components of the secondary atmospheric aerosol: nitrate, sulphate, ammonium and organic compounds. The model describes the detailed chemistry of the formation of the acid precursors from the oxidation of SO2, DMS, NOx, NH3 and terpenes and their uptake into the aerosol. Model results are compared in some detail with the available surface observations. Comparisons are made between the global budgets and burdens found in other modelling studies. The global distributions of the total mass of secondary aerosols have been estimated for the pre-industrial, present day and 2030 emissions and large changes have been estimated in the mass fractions of the different secondary aerosol components. 相似文献
992.
993.
根据中国1950、1960、1970、1980年和1990年地磁三分量绝对测量资料,使用球冠谐和分析方法,分别计算1950~1990年各个年代中国地磁剩余场冠谐模型. 球冠极点位于36°N和104°E,球冠半角为30°,冠谐模型的截断阶数为8. 地磁剩余场冠谐模型的均方偏差分别为:对于X分量,1950年为93.1 nT,1960年为128.9 nT,1970年为107.2 nT,1980年为107.6 nT,1990年为95.2 nT;对于Y分量,1950~1990年依次为74.8 nT,98.1 nT,89.2 nT,89.9 nT和84.0 nT;对于Z分量,分别为122.2 nT(1950年),135.0 nT(1960年),137.7 nT(1970年),110.1 nT(1980年)和107.5 nT(1990年). 根据中国地磁剩余场冠谐模型和全球地磁场DGRF模型,得到中国地磁场的冠谐模型,并对冠谐模型的边界效应进行了分析和讨论. 相似文献
994.
This work presents the temporal evolution and spatial distribution of nitrogen dioxide (NO2) measured with the help of passive diffusion tubes in different environments: rural, sub-urban, urban, at La Réunion Island in December 1997 and November 2000 (austral spring), respectively. NO2 concentration exhibits notable enhancement from 1997 to 2000. For instance, its mean concentration was 16 and 20 μg/m3 in December 1997 and November 2000, respectively, at La Réunion Island, especially in inhabited regions due to increase of local anthropogenic activities, mainly traffic circulation, in the absence of house heating and biomass burning. We also observe a net increase of pollutant levels by a factor two in rural/remote areas within 3 years, which is tied to the extension of inhabited areas and air-flows from enhanced local sources. The increase of atmospheric pollutants is mainly due to enhancement of anthropogenic activities (traffic) since the 1990s at La Réunion Island, which results from a constant increase of population and consequently, from a higher number of vehicles in circulation. Importantly, in cities like Saint-Denis, where traffic network has been subject to notable improvement (e.g. single to double lanes, etc.), pollutant levels exhibit little variability as in temperate continental latitudes. Semi-continuous NO2 concentration measured in parallel with ozone in November 2000 also showed that daytime photochemical ozone production is influenced by pollutant and precursor (NO2) levels at Saint-Denis, while nighttime ozone increase is mainly tied to dynamical processes. The November 2000 ozone diurnal pattern is notably different from that observed in September 1995, during which a daytime ozone loss was observed, pointing out that atmospheric conditions have been subject to notable changes, i.e., clean to moderately polluted, within a few years at La Réunion Island. The results presented here point out that the ‘source enhancement effect’ is superimposed on dynamical and photochemical processes to influence pollutants variability and hence atmospheric chemistry, in a quite ‘pristine’ tropical oceanic region. 相似文献
995.
MODELING THE EFFECTS OF ANTHROPOGENIC SULFATE IN CLIMATE CHANGE BY USING A REGIONAL CLIMATE MODEL 总被引:3,自引:2,他引:3
1 INTRODUCTION Being an important composition of the atmosphere, aerosol attracts increasing attention from the scientific community in recent years, together with the radiative forcing it causes and effects it imposes on the climate system. The anthropogenic aerosol affects the climate both directly and indirectly. The climate is directly affected when solar shortwave radiation is scattered and absorbed in what is known as the 搖mbrella effect? which can be dated back to as early as mor… 相似文献
996.
We compare flux and concentration footprint estimates of athree-dimensional Lagrangian stochastic dispersion modelapplying backward trajectories with the results of ananalytical footprint model by Kormann and Meixner.The comparison is performed for varying stability regimesof the surface layer as well as for different measurementheights. In general, excellent correspondence is found. 相似文献
997.
利用T42L9全球大气环流谱模式进行数值试验 ,以揭示南海夏季风强度异常的特征及其影响。控制试验结果表明 ,该模式不仅能够很好地模拟出气候平均的西风带槽脊和高低空气流分布以及它们的季节性变化 ,而且对于与亚洲季风有关的各个主要系统 ,如南亚高压、副高进退及越赤道气流等都有较强的模拟能力。在亚洲季风区及热带太平洋这一大范围区域的大气内部热源异常强迫下 ,模式显示出了南海夏季风持续异常的特征、北半球热带外环流的响应以及亚洲季风区降水异常分布。南海夏季风长时间强度异常所引起的大气内部热源异常 ,一方面通过三维垂直环流的异常联结着南海夏季风对北半球热带内外环流的影响 ,另一方面它又通过持续异常期的波列传播 ,即能量的传播 ,不仅影响我国长江流域降水 ,还会逐渐影响到北半球中高纬环流结构。这样西风带环流形势将会发生相应的变化和调整 ,南海夏季风持续异常影响到了北半球大气环流和天气气候的变化。 相似文献
998.
应用自然正交函数分解(EOF)方法,分析了甘肃省庆阳地区春末夏初干旱的综合评价指数DH的空间分布特征及随时间演变规律;分析了春末夏初干旱对冬小麦和玉米产量的影响;应用逐步回归方法建立了春末夏初干旱的预测模型,业务使用效果良好。 相似文献
999.
1000.