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91.
Erik Swietlicki Jingchuan Zhou Olle H. Berg Bengt G. Martinsson Gran Frank Sven-Inge Cederfelt Ulrike Dusek Axel Berner Wolfram Birmili Alfred Wiedensohler Brett Yuskiewicz Keith N. Bower 《Atmospheric Research》1999,50(3-4)
The hygroscopic properties of sub-micrometer aerosol particles were studied in connection with a ground-based cloud experiment at Great Dun Fell, in northern England in 1995. Hygroscopic diameter growth factors were measured with a Tandem Differential Mobility Analyser (TDMA) for dry particle diameters between 35 and 265 nm at one of the sites upwind of the orographic cloud. An external mixture consisting of three groups of particles, each with different hygroscopic properties, was observed. These particle groups were denoted less-hygroscopic, more-hygroscopic and sea spray particles and had average diameter growth factors of 1.11–1.15, 1.38–1.69 and 2.08–2.21 respectively when taken from a dry state to a relative humidity of 90%. Average growth factors increased with dry particle size. A bimodal hygroscopic behaviour was observed for 74–87% of the cases depending on particle size. Parallel measurements of dry sub-micrometer particle number size distributions were performed with a Differential Mobility Particle Sizer (DMPS). The inorganic ion aerosol composition was determined by means of ion chromatography analysis of samples collected with Berner-type low pressure cascade impactors at ambient conditions. The number of ions collected on each impactor stage was predicted from the size distribution and hygroscopic growth data by means of a model of hygroscopic behaviour assuming that only the inorganic substances interacted with the ambient water vapour. The predicted ion number concentration was compared with the actual number of all positive and negative ions collected on the various impactor stages. For the impactor stage which collected particles with aerodynamic diameters between 0.17–0.53 μm at ambient relative humidity, and for which all pertinent data was available for the hygroscopic closure study, the predicted ion concentrations agreed with the measured values within the combined measurement and model uncertainties for all cases but one. For this impactor sampling occasion, the predicted ion concentration was significantly higher than the measured. The air mass in which this sample was taken had undergone extensive photochemical activity which had probably produced hygroscopically active material other than inorganic ions, such as organic oxygenated substances. 相似文献
92.
A combination of retention pond and reed bed was tested for its effectiveness in reducing non-point source runoff pollution from an urban area. This paper presents data on the development of reed plants (Phragmites australis Cav. Trin.), on the effectiveness of runoff purification and on the accumulation of contaminants in the pond sediment and the reed bed for the years 1993–1995. P. australis was well established and grew according to normal development. The measured length and biomass values of P. australis were larger on sand than on gravel and coarse materials. Toxic levels of heavy metals in the plants were not reached. Harvested plants can be composted. The purification system is effective within the following ranges: The rate of retention of suspended solids and heavy metals varies between 16% and 91%. For chemical oxygen demand the average values is 25%. Poor retention rates usually occur along with very low input concentrations. Generally retention within the reed bed is higher than in the pond. Between 1993 and 1995 the concentration of contaminants within the organic layer of the reed bed increased by 50% for lead and by 90% for poly aromatic hydrocarbons. Until 1994 the concentrations of mineral oil hydrocarbons also increased by 60%. Between 1994 and 1995 however the concentration of mineral oil hydrocarbons in the reed bed decreased rapidly by more than 50%: Mineral oil hydrocarbons underlie biological degradation within the reed bed. In the pond sediment a significant accumulation of heavy metals, poly aromatic hydrocarbons and mineral oil hydrocarbons has also been found. The concentrations of these contaminants are still far from inhibiting the function of the system. 相似文献
93.
In 1983 the regional authority in Schleswig-Holstein (North Germany) started their long term monitoring programme in 29 lakes. During the following years the number increased to 68 lakes in 1993. The monitoring programme includes the parameter carbon (DOC, TOC), nitrogen (NH4-N, NO2-N, NO3-N, TDN) phosphorus (PO4-P, TDP), conductivity and temperature. Water samples are taken only once a year during late winter overturn in the main outflow of every lake. In this study TOC, TDN and TDP are chosen as most independent variables by correlation tests. Average concentrations of the years 1983 to 1985 and 1992 to 1993 as well as the concentration difference between 1992/93 and 1983/85 are clustered using the Average Linkage Method. It is necessary to use averages of a few years to reduce effects of interannual variability.Between 1983/85 and 1992/93 the average TDP-concentration in all 29 lakes was reduced by 40% from 0.68 to 0.041 mg/l. TDN-concentrations declined by 13% from 2.6 to 2.3 mg/l. The strong reduction of phosphorus concentrations clearly reflect the success of local sewage purification during the last two decades. The high importance of diffuse input sources for lakes is the reason for the less pronounced decline in TDN concentrations.The increase in TOC-concentrations by 14% (from 9.3 to 10.6 mg/l) between 1983/85 and 1992/93 is no indicator for an increased average annual algae biomass in the lakes. It is a result of unusual algae blooms during the warm winters between 1989 and 1993.Beside some similarities, the dendrogram on the basis of 1983/85 data and the one using 1992/93 values show that a lot of lakes are located to different clusters. The classification on the basis of concentration differences (1992/93–1983/85) yield three larger groups of lakes with a similar development and 5 groups containing only one or two lakes with extraordinary changes in their properties during the decade. To a certain degree, TOC, TDN and TDP can be seen as trophic state indicators. During the decade most lakes have been subject to significant changes and some main cluster with different directions of the trophic development become obvious. On the other hand a considerable number of lakes show a very special behaviour.The results underline that cluster methods are a useful tool to discover and analyse different developments in lakes. The calculation of T-values on the basis of classification results permit the identification of most representative individuals for every group of lakes. Representatives are valuable for a detailed discussion of driving forces and future investigations. They allow to handle a reduced number of lakes with minimal information loss about the entity.Lake Belau is the best representative for the average TOC-, TDN- and TDP-changes in all lakes. Its changes in water qualtity during the decade is discussed in detail. The high interannual variability of Chlorophyll a-, TDP- and TDN-concentrations in this lake clearly reflect the problems of long term analysis on the basis of this very limited monitoring programme. 相似文献
94.
Ocean Dynamics - Eddies in the global and coastal ocean play a key role in mixing and transport processes. Here, we present an eddy census for the Baltic Sea covering the years 2008–2010. The... 相似文献
95.
Ulrike Löptien Olga Zolina Sergey Gulev Mojib Latif Vladimir Soloviov 《Climate Dynamics》2008,31(5):507-532
Cyclone activity and life cycle are analysed in the coupled GCMs ECHAM5/OM and ECHAM4/OPYC3. First, the results for the present
climate (1978–1999) are compared with ERA-40 and NCEP/NCAR reanalyses, showing a drastic improvement in the representation
of cyclone activity in ECHAM5/OM compared to ECHAM4/OPYC3. The total number of cyclones, cyclone intensity, propagation velocity
and deepening rates are found to be much more realistic in ECHAM5/OM relative to ECHAM4/OPYC3. Then, changes in extra tropical
cyclone characteristics are compared between present day climate and future climate under the emission-scenario A1B using
ECHAM5/OM. This comparison is performed using the 20-year time slices 1978–1999, 2070–2090 and 2170–2190, which were considered
to be representative for the various climate conditions. The total number of cyclones does not undergo significant changes
in a warmer climate. However, regional changes in cyclone numbers and frequencies are evident. One example is the Mediterranean
region where the number of cyclones in summer increases almost by factor 2. Some noticeable changes are also found in cyclone
life cycle characteristics (deepening rate and propagation velocity). Cyclones in the future climate scenario tend to move
slower and their deepening rate becomes stronger, while cyclone intensity does not undergo significant change in a warmer
climate. Generally, our results do not support the hypothesis of enhanced storminess under future climate conditions. 相似文献
96.
Many problems in geology, especially structural geology, can only be solved by detailed mapping. Presently, mapping is still
mainly carried out on paper using techniques from the 19th Century. However, tools are now available to carry out most mapping tasks on microcomputers in the field without any need
of paper. This speeds up geological mapping and reduces the errors involved in the mapping process. Digital mapping also allows
work in featureless areas and areas of great structural complexity that would not be possible using paper maps. We present
two practical examples of the new technology of digital mapping using microcomputers, from Namibia and Greece. 相似文献
97.
Ulrike Hoff Oleg Dirksen Veronika Dirksen Ulrike Herzschuh Hans-Wolfgang Hubberten Hanno Meyer Christel van den Bogaard Bernhard Diekmann 《Journal of Paleolimnology》2012,47(4):549-560
Fossil diatom assemblages in a sediment core from a small lake in Central Kamchatka (Russia) were used to reconstruct palaeoenvironmental
conditions of the late Holocene. The waterbody may be a kettle lake that formed on a moraine of the Two-Yurts Lake Valley,
located on the eastern slope of the Central Kamchatka Mountain Chain. At present, it is a seepage lake with no surficial outflow.
Fossil diatom assemblages show an almost constant ratio between planktonic and periphytic forms throughout the record. Downcore
variations in the relative abundances of diatom species enabled division of the core into four diatom assemblage zones, mainly
related to changes in abundances of Aulacoseira subarctica, Stephanodiscus minutulus, and Discostella pseudostelligera and several benthic species. Associated variations in the composition and content of organic matter are consistent with the
diatom stratigraphy. The oldest recovered sediments date to about 3220 BC. They lie below a sedimentation hiatus and likely
include reworked deposits from nearby Two-Yurts Lake. The initial lake stage between 870 and 400 BC was characterized by acidic
shallow-water conditions. Between 400 BC and AD 1400, lacustrine conditions were established, with highest contributions from
planktonic diatoms. The interval between AD 1400 and 1900 might reflect summer cooling during the Little Ice Age, indicated
by diatoms that prefer strong turbulence, nutrient recycling and cooler summer conditions. The timing of palaeolimnological
changes generally fits the pattern of neoglacial cooling during the late Holocene on Kamchatka and in the neighbouring Sea
of Okhotsk, mainly driven by the prevailing modes of regional atmospheric circulation. 相似文献
98.
99.
Larisa Nazarova Ulrike Herzschuh Sebastian Wetterich Thomas Kumke Ludmila Pestryakova 《Journal of Paleolimnology》2011,45(1):57-71
We investigated the subfossil chironomid fauna of 150 lakes situated in Yakutia, northeastern Russia. The objective of this
study was to assess the relationship between chironomid assemblage composition and the environment and to develop chironomid
inference models for quantifying past regional climate and environmental changes in this poorly investigated area of northern
Russia. The environmental data and sediment samples for chironomid analysis were collected in 5 consecutive years, 2003–2007,
from several regions of Yakutia. The lakes spanned wide latitudinal and longitudinal ranges and were distributed through several
environmental zones (arctic tundra, typical tundra, steppe-tundra, boreal coniferous forest), but all were situated within
the zone of continuous permafrost. Mean July temperature (TJuly) varied from 3.4°C in the Laptev Sea region to 18.8°C in central Yakutia near Yakutsk. Water depth (WD) varied from 0.1 to
17.1 m. TJuly and WD were identified as the strongest predictor variables explaining the chironomid communitiy composition and distribution
of the taxa in our data set. Quantitative transfer functions were developed using two unimodal regression calibration techniques:
simple weighted averaging (WA) and weighted averaging partial least squares (WA-PLS). The two-component TJuly WA-PLS model had the best performance. It produced a strong coefficient of determination (r
2
boot = 0.87), root mean square error of prediction (RMSEP = 1.93), and max bias (max biasboot = 2.17). For WD, the one-component WA-PLS model had the best performance (r
2
boot = 0.62, RMSEP = 0.35, max biasboot = 0.47). 相似文献
100.
Klaus Peter Jochum Brigitte Stoll Ulrike Weis Dorrit E. Jacob Regina Mertz‐Kraus Meinrat O. Andreae 《Geostandards and Geoanalytical Research》2014,38(3):265-292
LA‐ICP‐MS is one of the most promising techniques for in situ analysis of geological and environmental samples. However, there are some limitations with respect to measurement accuracy, in particular for volatile and siderophile/chalcophile elements, when using non‐matrix‐matched calibration. We therefore investigated matrix‐related effects with a new 200 nm femtosecond (fs) laser ablation system (NWRFemto200) using reference materials with different matrices and spot sizes from 10 to 55 μm. We also performed similar experiments with two nanosecond (ns) lasers, a 193 nm excimer (ESI NWR 193) and a 213 nm Nd:YAG (NWR UP‐213) laser. The ion intensity of the 200 nm fs laser ablation was much lower than that of the 213 nm Nd:YAG laser, because the ablation rate was a factor of about 30 lower. Our experiments did not show significant matrix dependency with the 200 nm fs laser. Therefore, a non‐matrix‐matched calibration for the multi‐element analysis of quite different matrices could be performed. This is demonstrated with analytical results from twenty‐two international synthetic silicate glass, geological glass, mineral, phosphate and carbonate reference materials. Calibration was performed with the certified NIST SRM 610 glass, exclusively. Within overall analytical uncertainties, the 200 nm fs LA‐ICP‐MS data agreed with available reference values. 相似文献