基于CALIPSO卫星探测的2007—2018年西南地区平流层气溶胶的光学特性分析

基于CALIPSO卫星2007-2018年的三级平流层气溶胶廓线资料，本文分析西南地区平流层气溶胶的光学特性。结果表明：首先，在地理和季节上西南地区平流层气溶胶浓度较低。在夏季，西南地区平流层气溶胶光学厚度的均值出现最大值0.0007。其次，平流层气溶胶总衰减后向散射值的廓线分布随着高度的增加而减小，在10~11千米高度处出现最大值。这可能是由于对流层顶部和平流层底部之间气溶胶的相互交换。同时，平流层气溶胶总衰减后向散射值的纬向（北纬22.5°-32.5°）分布在七月出现均值最大值为0.0006×10-3 km-1sr-1，而径向分布（东经90°-110°）在一月出现最大值为0.0018×10-3 km-1sr-1。     

小张庄近地面大气环境特性变化观测分析

根据１９９３年１０月,１９９５年５月和１９９７年４月在农业生态环境“全球５００佳”－安徽省颖上县小张庄（３４°４７′Ｎ,１１６°２３′Ｅ）所进行的近地面污染气体（ＳＯ２,Ｏ３,ＮＯｘ）和气溶胶的观测结果,给出了这些微量气体的浓度平均概况及随时间和季节变化的一些特征,这三次观测表明,小张庄大气环境质量是持续好的,地面Ｏ３浓度主要取决于地面总辐射强度控制下的光化学反应过程;小张庄大气气溶胶粒子９９％是     

WMO资助仪器设备在瓦里关全球本底站安装运行

气溶胶光学厚度监测系统是世界气象组织和中国气象局共同资助瓦里关气溶胶升级系统的重要内容之一。该系统主要包括自动太阳跟踪器和精密滤光辐射计。精密滤光辐射计（PFR）是瑞士世界辐射校正中心Davos物理气象观象台（PMOD）自行研制的,可以自动、连续地在4个窄光谱段对太阳辐射进行准确、可靠的测量,进而获得气溶胶光学厚度。     

根据Dobson和TOMS资料分析北京和昆明大气臭氧总量变化特征

用约２０年 Ｄｏｂｓｏｎ和ＴＯＭＳ资料来分析北京（３９.９３°Ｎ，１１６.４０°Ｅ）和昆明 （２５.０２°Ｎ，１０２．６８°）两地大气臭氧总量的变化特征，结果表明：（１）在１９７９－２０００年间北京大气臭氧长期变化趋势是－０．６４２ ＤＵ／年，而昆明在１９８０－２０００年间的趋势是－０.００９ ＤＵ／年；（２）北京和昆明两地大气臭氧都有很强的季节内变化（尤其冬季更强），与季节性变化强度相当；（３）在北京和昆明，由记录较短的大气臭氧资料分析得到的长期变化趋势，与较长记录得到的结果有显著差异；（４）在北京（中纬度）和昆明（低纬度）大气臭氧都有显著的准两年振荡信号；（５）两个站点大气臭氧的年际变化主要由长期趋势项和准两年振荡信号组成；（６）Ｄｏｂｓｏｎ仪测量得到的臭氧总量与ＴＯＭＳ资料非常一致。     

赤道西太平洋强东风带特征及其形成机制的诊断分析

利用１９９３年ＥＮＳＯ事件（４月）爆发前酝酿阶段，ＴＯＧＡ／ＣＯＡＲＥ关键区强化期（１９９２年１１月－１９９３年２月）立体观测实验“向阳红五号”科学考察船定点（１５５°Ｅ，２°Ｓ）高空大气探测资料，分析了西太平洋暖海域上空对流上升区西侧风的垂直变化，指出：对流层上、下部各有一强风带，随着海－气ＥＮＳＯ异常的发展，高空强东风带和低空强西风带均呈增强趋势，最强时分别连续１４天和１８天达到急流标准，占相     

10──20天准双周振荡的经向传播及地理特征

本文采用ＥＣＭＷＦ１９８３年７月１日至９月１２日逐日２００ｈＰａ纬向风场资料，用复经验正交方法讨论了１０－２０天低频振荡的经向传播及地理特征。结果表明：（１）１０－－２天振荡有三个显著区域：贝加尔湖附近地区；赤道９０°Ｅ附近以及新加坡、马来西亚地区；８０－１００°Ｅ，２２－３２°Ｎ之间。（２）源于较高纬度地区的振荡与源于赤道附近地区的振荡在１０５°Ｅ，１７—２３°Ｎ附近同位相相遇，在９０°Ｅ，２０°Ｎ附近反位相相叠加，振荡相互削弱，在２５°Ｎ附近同位相相遇。（３）从振荡位相来看，中南半岛东南部、马来西亚北部、菲律宾以西区域的振荡向北传播到中国东南沿海，向西传播到孟加拉湾印度半岛；２０°Ｎ以南低纬度地区的振荡很少能传播到８０°Ｅ以东３０°Ｎ附近地区；位于９０－９５°Ｅ，２５－２７°Ｎ之间的振荡以及贝加尔湖附近地区的振荡可以向南北两个方向传播。     

中国部分清洁地区大气中N2O的浓度

１９９３年４月—１９９５年８月对中国部分清洁地区大气的Ｎ２Ｏ浓度进行了现场观测，结果表明：农田（玉米田和麦田）大气的Ｎ２Ｏ平均浓度高达３２２．１－３４３．４ｐｐｂｖ，这是土壤排放Ｎ２Ｏ的结果；临安、龙风山和瓦里关山大气本底观测站（ＷＭＯ／ＧＡＷ）Ｎ２Ｏ的平均浓度分别为３１８．８±８．４ｐｐｂｖ，３１７．４±４．７ｐｐｂｖ和３１４．０±４．２ｐｐｂｖ。在此基础上，分析了大气Ｎ２Ｏ的分布及变化特征。另外，还对现场取样及Ｎ２Ｏ浓度测量技术作了初步分析和评价     

利用激光雷达观测资料研究兰州气溶胶光学厚度

利用兰州大学半干旱气候与环境观测站（SACOL）2006—2011年晴空无云时激光雷达（CE-370—2）资料,结合2006年12月至2007年5月多波段太阳光度计（CE-318）资料,对比验证了激光雷达资料的反演结果,并分析了兰州地区气溶胶光学厚度的分布特征。结果表明：激光雷达反演得到的光学厚度与光度计观测得到的光学厚度,两者具有较好的相关性,相关系数为0．86。兰州地区气溶胶光学厚度3—5月和11-12月较大,主要原因是3—5月是当地沙尘频发期,11—12月是居民集中采暖期,沙尘排放和燃煤排放显著增加了大气气溶胶光学厚度。气溶胶光学厚度6～10月偏小,湿沉降清除是主要的影响因素。光学厚度季节分布为春季0．42,冬季0．36,秋季0．30,夏季0．21。光学厚度频数分布于0．0～0．3的最多,占总数的一半,且存在季节差异。兰州上空夏季干净,春季浑浊,冬季次浑浊。     

1991—1992年ENSO事件的特征

根据美国国家海洋大气局气候分析中心（ＣＡＣ）和中国气象局气候监测公报所提供的海－气资料，综合分析了１９９１－１９９２年ＥＮＳＯ事件的形成、发展过程。这次ＥＮＳＯ事件的主要特点是：①在ＥＮＳＯ事件爆发前一年内热带太平洋海气特性频频呈现异常，暖水堆积在赤道中太平洋（５°Ｎ－５°Ｓ，１６０°Ｅ－１６０°Ｗ）约１２个月，然后自西向东传输，爆发１９９１－１９９２年ＥＮＳＯ事件。②对ＥＮＳＯ事件作出响应的西太     

用NOAA气象卫星资料对甘肃省河东地区土地覆盖分类

根据不同植被群落植被指数的时空变化特点，利用１９９１－１９９３年ＮＯＡＡ气象卫星ＡＶＨＲＲ资料对３２．５°－３８．０°Ｎ，１００．５°－１０９．０°Ｅ范围内的土地覆盖状况进行了分类，并利用分类结果讨论了不同土地类型植被指数年变化的特点。     

Investigation of aerosol optical properties in Bangkok and suburbs

Aerosol optical depth and Angstrom coefficients for three sites in Bangkok and suburbs are examined: Silpakorn University at Nakhon Pathom, NP (13.82°N, 100.04°E), the Asian Institute of Technology at Phatum Thani, AIT (14.08°N, 100.62°E) and the Thai Meteorological Department at Bangkok, BK (13.73°N, 100.57°E). Sunphotometers have been used to measure direct normal spectral irradiance at these sites for a period of 2 years (2004–2005). Cloudless conditions were selected and Bouguer’s law was employed to obtain aerosol optical depth. All three sites exhibit strong seasonal variations, with the highest values occurring at the height of the dry season in April, and the lowest occurring during the rainy season in July. April turbidity conditions are very high, as evidenced by maximum 500 nm optical depths of between 1.4 to 2.0 that were measured at all three locations. The Angstrom exponent α also showed a marked seasonal change, with highest values at the height of the dry season.     

Some features of winter aerosol and water vapor characteristics over Agra, a semi-arid location in India

Reported in this article are the results of the analysis of extensive observations of aerosol optical, micro-physical characteristics, and precipitable water content (PWC) that have been carried out using compact, multi-band solar radiometers, over a semi-arid station, Agra (27°10′N, 78°05′E, 169 m AMSL) during winter 2004. The aerosol optical depth (AOD), Angstrom wavelength exponent (α), and PWC show, higher values on hazy- and foggy-days and lower values on clear-days. The turbidity coefficient (β) shows higher values for smaller values of α and vice versa. The aerosol size spectra exhibit bi-modal distribution with abundance of accumulation-mode particles during fog and haze occasions, and relatively coarse-mode particles on clear-days. The above features have been explained with co-located PWC and surface-level meteorological parameters. The NOAA HYSPLIT five-day back trajectories indicate the influence of trans-boundary pollution transport over the experimental station during the study period.     

基于太湖地区MFRSR遥感大气气溶胶光学特性和大气污染状况

利用2008年5月16日至2009年4月17日太湖地区多光谱旋转遮光辐射仪（multi—filter ro—tating shadow—band radiometer,简称MFRSR）的观测资料进行反演,得出415、500、615、675和870nm5个波段大气气溶胶光学厚度（aerosol optical depth,简称AOD）及各季节浑浊度系数和波长指数的统计结果。结果表明,5个波段AOD的最大值分别为1．9、1．6、1．3、1．2和1．0;它们谱分布的半宽度分别为0．90、0．70、0．55、0．45和0．25;AOD频率分布极大值处所对应的AOD值分别为0．750、0．550、0．475、0．425和0．425。5个波段AOD的平均值在春季最大,夏季次之,除870nm外,均为冬季最小。浑浊度系数变化范围为0～1．25,其中大于0．2的占97％以上,大于0．4的占66％以上。春季、夏季、秋季和冬季的波长指数变化范围分别为0～3．0、0～2．8、0．2～2．0和0．2～2．0,表明太湖地区大气污染较为严重,且受人为源的影响显著。相对于秋冬季,春夏季有较大粒径的气溶胶粒子存在。     

Aerosol radiative properties in the semiarid Western United States

Characterization of aerosol optical properties, such as aerosol optical depth, Angstrom exponent, and volume size distribution at the semiarid site of Tombstone Arizona (31°23′N, 110°05′W, 1408 m) will be presented for one annual cycle. In this region, extensive observations of selected optical parameters such as aerosol optical depth (AOD) have been made in the past and reported on in the literature. Less is known about other optical characteristics that are important in climate modeling and remote sensing. New observational techniques and inversion methods allow for the expansion of the earlier information. Observations have been taken with a state of the art sun photometer for a 1-year period and their analysis will be presented here. Monthly mean AODs at 500 nm were found to be in the range of 0.03–0.12; the monthly mean Angstrom exponent ranged from 0.9 to 1.6, being higher in spring and summer and lower in late fall and winter. Volume size distributions exhibit clear dominance of smaller particles, with a gradual increase in size from winter to spring and into summer. Annual variation of the radii of the smaller and the larger particles ranged between 0.05–0.4 and 4–8 μm, respectively. Radiance measurements at 940 nm were used to estimate precipitable water. The retrieved values compared within limits of uncertainty with independently derived estimates from the National Center for Environmental Prediction (NCEP) regional weather forecast model. An interesting outcome from this study was the consistency found in aerosol optical depths as observed in this study and those derived about two decades ago.     

2010年秋季鞍山气溶胶光学特征变化

利用2010年9-11月鞍山大气成分监测站CE-318太阳光度计观测资料,依据气溶胶光学厚度测量原理,计算得到2010年鞍山秋季大气气溶胶光学厚度、波长指数等大气光学特性数据,通过统计分析,给出鞍山秋季气溶胶光学特性分布特征。结果表明：随着测量AOD波段的降低,AOD值逐渐增大,9月的AOD平均值最大,10月AOD平均值次之,11月AOD平均值最小。从频率分布看,2010年9月 AOD日均值集中分布在0.4-0.6之间,10月和11月AOD日均值集中分布在0.0-0.4之间,表明10-11月大气较为清洁|波长指数日均值的频率分布说明鞍山秋季大气污染物以细粒子为主。500 nm 的AOD值与波长指数成对数关系,两者在9、10月和11月的相关系数分别为0.5145、0.8412和0.2715;9月AOD与PM₁₀、PM_2.5、PM_1.0质量浓度为较小负相关,10月和11月AOD与PM₁₀、PM_2.5、PM_1.0质量浓度成正相关,且10、11月AOD与气溶胶细粒子相关性较为显著。AOD值与能见度在趋势上呈较小的负相关性,可能是由于高层气溶胶粒子对气溶胶光学厚度产生了主要影响。     

An Empirical Method for Estimating Background Stratospheric Aerosol Extinction Profiles over China

The current paper introduces an empirical method for estimating the vertical distribution of background stratospheric aerosol extinction profiles covering the latitude bands of 50±5°N,40±5°N,30±5°N,and 20±5°N and the longitude range of 75 135°E based on Stratospheric Aerosol and Gas Experiment (SAGE) II aerosol extinction measurements at wavelengths of 1020 nm,525 nm,452 nm,and 386 nm for the volcanically calm years between 1998 2004.With this method,the vertical distribution of stratospheric aerosol extinction coefficients can be estimated according to latitude and wavelength.Comparisons of the empirically calculated aerosol extinction profiles and the SAGE II aerosol measurements show that the empirically calculated aerosol extinction coefficients are consistent with SAGE II values,with relative differences within 10% from 2 km above the tropopause to 33 km,and within 22% from 33 km to 35 km.The empirically calculated aerosol stratospheric optical depths (vertically integrated aerosol extinction coefficient) at the four wavelengths are also consistent with the corresponding SAGE II optical depth measurements,with differences within 2.2% in the altitude range from 2 km above the tropopause to 35 km.     

A study of aerosol properties over Lahore (Pakistan) by using AERONET data

It is well established that aerosols affect the climate in a variety of ways. In order to understand these effects, we require an insight into the properties of aerosols. In this paper we present a study of aerosol properties such as aerosol optical depth (AOD), single scattering albedo (SSA) and aerosol radiative forcing (ARF) over mega city of Lahore (Pakistan). The data from Aerosol Robotic Network (AERONET) have been used for the period December 2009 to October 2011. The seasonal average values of AOD, asymmetry parameter (ASY) and volume size distribution in coarse mode were observed to be highest in summer. On the other hand, the average values of Angstrom exponent (AE) and imaginary part of refractive index (RI) were found to be maximum in winter. The average value of real part of RI was found to be higher in spring than in all other seasons. The SSA exhibited an increasing trend with wavelength in the range 440 nm–1020 nm in spring, summer and fall indicating the dominance of coarse particles (usually dust). However, a decreasing trend was found in winter in the range 675 nm–1020 nm pointing towards the dominance of biomass and urban/industrial aerosols. As far as aerosol radiative forcing (ARF) is concerned, we have found that during the spring season ARF was lowest at the surface of Earth and highest at top of the atmosphere (TOA). This indicates that the atmosphere was warmer in spring than in all the remaining seasons.     

Aerosols and their influence on radiation partitioning and savanna productivity in northern Australia

Aerosols have been shown to affect the quantity and quality of solar radiation on the Earth’s surface. Savanna regions are subject to frequent burning and release of aerosols that may impact on radiation components and possibly vegetation productivity in this region. Therefore, in this study, we have analyzed the optical properties of aerosols (aerosol optical depth (AOD) and Angstrom coefficient) from the Atmospheric Radiation Measurement site in Darwin for the periods from April 2002 to June 2005 as measured by a multifilter rotating shadowband radiometer. The influence of aerosols and their effect on surface shortwave incoming solar radiation and savanna productivity were examined for the dry season using sky radiation collection of radiometers and eddy covariance measurements from the Howard Springs flux site. Results indicated that aerosol concentrations in the region were relatively low compared to other savanna regions with the maximum monthly average AOD over the period being the greatest in October (0.29?±?0.003 standard error at 500 nm). The highest monthly average Angstrom exponent was also found in October (1.38?±?0.008). The relatively low aerosol concentration in this region can be attributed to the mixture of smoke aerosols with humidity haze and local circulations. Over a range of AODs from 0.1 to 0.4, we found a modest increase in the fraction of diffuse radiation to total radiation from 11% to 21%. This small increase in diffuse fraction did not affect the carbon flux significantly. However, because the current range of AOD in the region is relatively low, the region could be sensitive to increases in aerosols and diffuse fraction in the future.     

灰霾过程中的气溶胶特性观测研究

结合太阳光度计、激光雷达以及其他相关数据对河北香河县2007年4月初的一次灰霾天气过程中的气溶胶特性进行了遥感研究。研究表明,在这次灰霾的爆发期间,能见度从20 km下降到3 km左右;气溶胶光学厚度（AOD）在3个波段上都明显增加,特别是380 nm处的AOD从6日的031增长到10日的140;Angstrom指数(ALPHA)也明显下降,例如340~440 nm处的ALPHA从7日的145下降到10日的099。从AOD和ALPHA在短波处的较大变化、体积浓度谱的粗模态粒子的大量增加和PM10浓度值的变化分析来看,这次灰霾过程中的气溶胶数浓度明显增加,其中还含有大颗粒物的大量导入。激光雷达探测消光系数的垂直分布也显示气溶胶在垂直高度上达到了近3 000 m左右。从微物理特征的变化上看,这次灰霾过程中局地气溶胶的散射能力增强,吸收能力减弱。另外,通过HYSPLIT模式对后向轨迹的模拟和对NCEP数据的分析,发现这次灰霾过程中所包含的大颗粒物的主要源地可能是蒙古地区,所以气溶胶呈现了一定的沙尘气溶胶特征。     

气溶胶光学厚度谱特征判断粒子大小方法初探

当气溶胶谱满足Junge分布时,Angstrom指数 (α) 可以准确地描述粒子大小,但真实大气气溶胶很少完全满足这一条件,仅用α判断粒子大小会有较大出入。基于北京、香河、兴隆、太湖4个Aeronet观测站21世纪以来各站历时都超过1年的气溶胶光学厚度资料,获得5511组lnτ与lnλ的二次拟合参数a₂,a₁,尝试找到一种结合α,a₂,a₁判断粒子大小的方法。结果表明:当气溶胶为粗粒子时 (V_fine/V_total＜0.2),α均小于0.75,仅用α就可以较好地判断粒子大小,但当气溶胶以细粒子为主时 (V_fine/V_total＞0.7),该方法会有较大出入,此时a₂,a₁可以有效地辅助α判断粒子大小,α＞0.75,a₂＜-0.5或a₂＜-0.5,a₁＜-1.0是较好的判据。此外,分析发现国外研究提出的用a₂-a₁判断粒子大小的方法效果并不理想,尤其在1＜a₂-a₁＜2的情况下,粒子的组成有多种可能。