Soil radon,permeability, and indoor radon prediction

Attempts to predict which geographic areas should be associated with a high percentage of homes with unusually high indoor radon levels have been based on estimates of soil radon and soil permeability for geological units. In northern Virginia and southern Maryland, it appears that predictions of indoor radon based on estimates of homesite soil radon and soil permeability are very useful.     

From radon hazard to risk prediction-based on geological maps,soil gas and indoor measurements in Germany

Mapped geological units can be regarded as proxies standing for a complex series of subsoil geochemical and physical properties including the assigned radon activity concentration in soil gas, which is taken as best estimator of the regional geogenic radon potential. Areal distribution of measuring sites for soil gas in Germany is adapted to spatial variation of geology. A grid-based and distance-weighted interpolation procedure is applied, following geologically defined neighbourhood relations of measuring sites and accounting for isolated outcrops of known geology but without measurements. To investigate the statistical relationship between indoor radon, house type and building ground specifications, measurements of the indoor radon concentration have been carried out in more than 10,000 dwellings in different regions of Germany. Multiple regression analyses of variance reveal that besides region-specific geological properties and building characteristics, various house type and living style variables significantly contribute to the explained variance for ground floor radon concentrations. These parameters are also dominant in controlling the radon transfer relation from soil gas to indoor air. Risk prediction maps for radon in houses indicating the probability to exceed certain indoor threshold values can be useful especially for regions with no or only a few measurements of indoor radon.     

Regional levels of indoor radon in Virginia and Maryland

The levels of Rn-222 in homes located in Fairfax County, Virginia, and Montgomery County, Maryland, are currently being measured during four consecutive three-month seasonal intervals using alpha-track detectors. Significant variations occur between parts of northern Virginia and southern Maryland because the area is part of three very different geologic provinces. Results from the winter period in these three provinces show that the indoor radon levels were about twice as high as anticipated. Approximately 45 percent of the homes had winter indoor radon levels above 4 pCi/l, the EPA’s recommended action level, and in the spring period, more than 30 percent of the homes still had indoor levels above 4 pCi/l. Indoor radon variations due to seasonal control were about as significant as geological control. Worst-case combinations developed over some rock units in the winter, producing areas in which about 70 percent of the homes exceeded 4 pCi/l.     

The indoor radon problem: Studies in the Albuquerque,New Mexico area

Radon buildup in homes is now recognized throughout the world as a potentially major health hazard. The U.S. Nuclear Regulatory Commission and the U.S. Environmental Protection Agency estimate 8,000–30,000 fatalities per year in the United States due to indoor radon. The Albuquerque, New Mexico area was chosen for study because it is representative of metropolitan areas in the southwestern United States where slightly uraniferous source rocks (Sandia granite) have provided the very immature soil for much of the area. The granite contains 4.7 ppm U, and limestone capping the granite 5.7 ppm U. Soils in the area average 4.24 ppm U, and Th/U ratios average 3.2. These data suggest some removal of U from the source rocks, but fixation of the U in the soils (that is, as opposed to widespread removal of the U by solution), thus providing a ready source for soil radon. A pilot study of soil radon in the area in winter of 1983–1984 shows high values, 180 pCi/l, relative to the U.S. average (about 100 pCi/l). In the winter of 1986–1987, 180 dwellings were surveyed for their indoor radon levels, including 20 that had been surveyed in summer of 1986. Twenty-eight percent of those in the winter study yielded indoor radon above the EPA suggested maximum permissible level of 4 pCi/l air, well above the EPA estimate of 10–15 dwellings for the U.S. The indoor radon levels show positive correlation with closeness to the Sandia Mountains, to soil radon, to excess insulation, to homes with solar capacities, and other factors. Building materials may provide a very minor source of some indoor radon. Summer readings are lower than winter readings except when the houses possess refrigerated air conditioning.     

Increased soil gas radon and indoor radon concentrations in Neoproterozoic olistostromes of the Teplá-Barrandian unit (Czech Republic)

The Neoproterozoic olistostromes were first distinguished as a special geological unit in a generalised geological map of the Czech Republic on a scale 1:500,000. The olistostromes represent a tectonic mélange or subaquatic continental slope-slides formed by a mixture of black shales, greywackes, carbonates and shales, forming an extremely inhomogeneous geological environment. The extreme over-limit values of indoor radon (Rn, ²²²Rn) were first detected during check measurements performed for final building approval by team of the National Radiation Protection Institute in a house situated on bedrock of black shales—lithological component of olistostromes north-eastward from Plzeň. Additional measurements of soil gas Rn performed by the Czech Geological Survey were oriented to cover the whole olistostrome belt extending over 65 × 25 km area NE of Plzeň–Prague general direction. The increased concentrations both of soil gas and indoor Rn were confirmed in the whole extent of Neoproterozoic olistostrome belt compared to neighbouring geological units (Neoproterozoic metasediments on NW and Cambrian Palaeovolcanites and Ordovician sediments on SE). This observation lead to increasing the radon index of olistostromes to medium radon category (from the low one) both in general and detailed Rn index maps. Drawing the attention to this lithological type enables to improve the radon risk prevention for newly built houses and interest of remediation of existing houses not only in the specific area of the Czech Republic, but also in other European countries, where Neoproterozoic olistostromes form the geological basement.     

Indoor radon probability calculated from the Czech soil gas radon data in a grid net for the European Geogenic Radon Map construction: test of feasibility

The construction of the European Geogenic Radon Map in a proposed grid system 10 × 10 km requires the data test to derive the probability of exceeding the indoor action level 200 Bq m⁻³ from the geologically based data. The Czech Republic disposes both indoor and soil gas data sets to test the real probability to exceed 200 Bq m⁻³ from indoor radon measurements and to compare it with the probability calculated from soil gas radon concentrations. Comparison of real and calculated probability enables to delineate the areas, where under- or overestimation can be expected. The results of data processing show minor differences between processing the raw data in generalised polygons of geological units and in a grid net, when using the generalised geological characteristics of grid cells.     

Radon,Lung Cancer Risk and Environmental Geology in Gejiu Area

The incidence of lung cancer in the Gejiu area of Yunnan Province ranks the first in the world.The radon level(indoor,soil) was measured in the Gejiu area by the SSNTD method from 1990 to 1996,The result indicates an extensive high-level of indoor radon in that area though U and Th are lower in local limestones,The indoor radon level of houses located in the geologic fault zone is 6 times high that 2km far from the fault zone.The reason probably is that the radon level of soil in the fault is 6-8 times high that 1 km far from the faults.our data indicate that a lower range of radon levels,0-100Bq.m^-3,exists in healthy families.However,a higher radon level,over 800 Bq.m^-3,is often found corresponding to that of cancer patients‘ homes(the house-owners are suffering from either lung cancer or leukaemia or liver cancer),Obviously,an increase in lung cancer incidence follows an increase in indoor radon level,The risk of cancer induced by indoor radon is no longer an inference,but a fact.     

Radon soil–gas as a geological mapping tool: case study from basement complex of Nigeria

In an effort to quantify the geogenic radon soil–gas potential and appraise the use of radon technique as a geological mapping tool in a crystalline basement rock terrain of Ile–Ife Nigeria, radon measurement concentration were made using a radon detector instrument (EDA RD-200) that measures radon isotopes by a scintillator cell coupled to a photomultiplier tube. The data were collected from soils derived from three different lithologic rock units. The observed values were then correlated with the geology of the area. Significant differences in the radon soil–gas concentrations among the three geologic units were observed. Granite gneiss has the highest concentration, followed by grey gneiss and mica schist in that order. The geometric mean (GM) concentration of radon-222 measured in soils directly overlying the three different rock types were 301.4 pCi/l for granite gneiss, 202.8 pCi/l for the grey gneiss, and 199.4 pCi/l for mica schist. Conversely, the average values for radon-220 averaged 1510.0, 815.4, and 733.0 pCi/l for granite gneiss, grey gneiss, and mica schist rocks, respectively. Statistical t test (α=0.05) results indicated that there was no significant difference in the geometric mean of radon soil–gas measured between low and medium potential zones. However, significant differences were found between the low and high radon potential zones, and between the medium and high zones. The low concentrations of radon soil–gas emission observed in this study is explained in terms of the seasonal variation due to thermal convection fluid movement, while the radon concentrations were found to be controlled by the lithology and geochemistry of the underlying bedrock.     

Geochemistry and ground permeability as determinants of indoor radon concentrations in southernmost Sweden

A study of the indoor radon gas levels was performed in 935 homes in Scania, southernmost Sweden, located on geologically different ground with regard to uranium (U) content. In one of these two areas the bedrock consists of alum shale with U contents exceeding 200 ppm. In the other area there is no U-rich bedrock. Indoor radon levels are influenced by U content and permeability as shown below.For maam nancy for table, please place here. Thanx!The results show that the indoor radon levels were highest in homes located on bedrock with medium to high U content combined with a highly permeable drift covering the bedrock. The difference was statistically significant(P < 0.0001). Other results of the investigation are: 14 homes built from aerated concrete made from U-rich alum shale had higher levels than 767 homes with walls from other material (312 vs 106 Bq/m³;P = 0.0011); 242 homes with a cellar had lower radon levels than 563 without (62 vs 138 Bq/m³;P <0.0001); further, 418 homes with private well had higher levels than 360 with public water supply (140 vs 82 Bq/m³;P <0.0001). The results of the investigation show a profound effect of a combination of high bedrock U content and high cover permeability. The effect of the uraniferous drift on the indoor radon levels is evident. Thus, the geological conditions should be carefully considered when screening for high-risk buildings, as well as when planning for new ones. Also, the construction of the building and its water supply have some influence.     

Radon reduction in homes constructed on saprolite in the Central Appalachians

 A 3-year study of indoor radon in more than 1000 homes in northern Virginia and southern Maryland was conducted using 3-month exposure alpha-track monitors. In a study set of 200 homes, first-floor indoor radon concentrations, which most closely approximates home exposure levels, averaged slightly more than 3 pCi/l. In a study set of 100 homes, sub-slab ventilation was used to reduce indoor radon concentrations. Interest in remediation was related to public perception of the hazardous nature of radon; people living in homes with indoor radon measurements of more than 4 pCi/l were more likely to participate in the remediation phase of the project. Sub-slab ventilation was successful in more than 90% of the homes in reducing indoor radon from concentrations as high as 30 pCi/ to less than 4 pCi/l, at least for the entire year of post-remediation radon measurements. Received: 29 February 1996 · Accepted: 29 May 1996     

A preliminary design of a radon potential map for Canada: a multi-tier approach

Canada is a vast country with most of the population living on a small portion of the land. However, for a national radon potential map, it is mandatory to cover the entire country including sparsely populated areas. Because of these characteristics, the radon map development for Canada is challenging. After briefly reviewing of radon map development in the world, this study considers a multi-tier approach to best use available however limited resources and to generate a national radon map in a timely fashion. In summary, radon potential maps for highly populated areas should be determined by direct indoor radon measurements where enough indoor radon data are available. In areas where indoor radon measurements are limited or not yet available, the radon potential maps could be developed from various data sources with a multi-factor scoring system including geological information on soil permeability, soil gas radon concentration and ground uranium concentration. In sparsely populated areas, radon potential maps can only be generated with geological predictive tools, especially in those areas where no houses have yet been built. Because indoor radon measurement data and geological information relevant to radon are very limited in Canada, a multi-step strategy is also worth considering in addition to the multi-tier approach.     

Development of an indoor radon risk map of the Walloon region of Belgium,integrating geological information

A radon risk map for the Walloon region of Belgium, based on the two databases available, has been calculated and is presented in this work. The data are organized into geological units. For each unit, an average logarithmic standard deviation is calculated, after correcting the higher variability of short term data. The region is divided with an 1-km grid. For each node, the local geological unit is determined, as well as the corresponding logarithmic standard deviation. The logarithmic mean is evaluated by smoothing the data belonging to the same geological unit as the node. Assuming a log-normal distribution, a map that shows for each node the predicted percentage of buildings with an indoor radon concentration above the Action level (400 Bq/m³) is constructed. This is the first radon risk map for this region that fully takes into account the geological information.     

氡气灾害调查的一些结果

氡气灾害是一种广泛分布的地质灾害。室内氡气浓度偏高会使居民患肺癌的几率增高，而室内氡气主要来自房屋地基所在的地质单元。笔者在美国犹他大学研究所工作期是，研究了瑞丁普朗花岗片麻岩带近地表氡的浓度与铀含量的关系以及铀的分布与居民癌症死亡率之间的相关关系。铀的区域性分布是利用航空伽马能谱测量资料求得的，说明利用航空伽马能谱测量资料开展氡气灾害区域评价的可能性。文中还举例说明氡气调查在制定建设规划方面的作     

Radon variations in a Hungarian village

 A steady radon exhalation is assumed in most publications. In a village of North-East Hungary, however, high radon concentrations have been measured, differing strongly in neighbouring houses and varying in time, due to the interplay of geochemical phenomena. Received: 20 November 1995 · Accepted: 18 June 1996     

Impact of the deeper geological basement on soil gas and indoor radon concentrations in areas of Quaternary fluvial sediments (Bohemian Massif,Czech Republic)

The relationship of soil gas radon Rn²²² and indoor radon was studied within the Quaternary fluvial sediments of the Czech Republic. The processing of data selection from the radon database of the Czech Geological Survey and indoor radon data (database of the National Radiation Protection institute) has proved the concentration dependence of radon in Quaternary fluvial sediments on deeper bedrock. The ArcGIS processing was accompanied by the field verification in five profiles, intersecting the granitoid Central Bohemian Plutonic Complex and its rim rock types. Both theoretical and experimental results show dependence of soil gas radon and indoor radon concentrations in Quaternary fluvial sediments on deeper geological basement, thus leading to the conclusion that the lateral transport of Quaternary sediments does not play such a dominant role in radon concentrations, as was thought previously. This fact will enable to determine precisely the radon index of Quaternary sediments (in the Czech radon mapping classified as an intermediate index) into three categories according to the lithology of their geological basement.     

Mapping radon-prone areas - a geophysical approach

 Radon-prone areas in Israel were mapped on the basis of direct measurements of radon (²²²Rn) in the soil/rock gas of all exposed geological units, supported by the accumulated knowledge of local stratigraphy and sub-surface geology. Measurements were carried out by a modified alpha-track detection system, resulting in high radon levels mainly in rocks of the Senonian-Paleocene-aged Mount Scopus Group, comprised of chert-bearing marly chalks, rich in phosphorite which acts as the major uranium source. Issues of source depth, seasonal variations and comparison with indoor radon levels are addressed as well. This approach could be applied to other similar terrains, especially the Mediterranean Phosphate Belt.     

Indoor radon correlated with soil and subsoil radon potential—a case study

High indoor radon concentrations in a uranium-radium low-level area in the Eifel region, Germany, near the village of Döttingen are caused by ascending radon migration following the convection of groundwater and soil gas along pathways (fractures and faults) in the bedrock sediments of Lower Devonian age. Positive radon anomalies in the soil gas are found to coincide with the locations of houses showing the highest concentrations. These houses are older buildings without concrete foundation slabs. Normally radon concentrations in soil gas are highly correlated with the values of emanated radon calculated on the basis of radium content in the surrounding soils and rocks (diffusive radon potential). However, close to zones of tectonic fractures and faults around the maar-type volcano of Döttingen abnormally high radon concentrations, which were transported by circulating groundwater and postvolcanic exhalation of CO₂ (convective radon potential) were detected.     

Predicting New Hampshire indoor radon concentrations from geologic information and other covariates

 Generalized geologic province information and data on house construction were used to predict indoor radon concentrations in New Hampshire (NH). A mixed-effects regression model was used to predict the geometric mean (GM) short-term radon concentrations in 259 NH towns. Bayesian methods were used to avoid over-fitting and to minimize the effects of small sample variation within towns. Data from a random survey of short-term radon measurements, individual residence building characteristics, along with geologic unit information, and average surface radium concentration by town, were variables used in the model. Predicted town GM short-term indoor radon concentrations for detached houses with usable basements range from 34 Bq/m³ (1 pCi/l) to 558 Bq/m³ (15 pCi/l), with uncertainties of about 30%. A geologic province consisting of glacial deposits and marine sediments was associated with significantly elevated radon levels, after adjustment for radium concentration and building type. Validation and interpretation of results are discussed. Received: 20 October 1997 · Accepted: 18 May 1998     

A geostatistical approach for mapping and uncertainty assessment of geogenic radon gas in soil in an area of southern Italy

Spatial distribution of concentrations of radon gas in the soil is important for defining high risk areas because geogenic radon is the major potential source of indoor radon concentrations regardless of the construction features of buildings. An area of southern Italy (Catanzaro-Lamezia plain) was surveyed to study the relationship between radon gas concentrations in the soil, geology and structural patterns. Moreover, the uncertainty associated with the mapping of geogenic radon in soil gas was assessed. Multi-Gaussian kriging was used to map the geogenic soil gas radon concentration, while conditional sequential Gaussian simulation was used to yield a series of stochastic images representing equally probable spatial distributions of soil radon across the study area. The stochastic images generated by the sequential Gaussian simulation were used to assess the uncertainty associated with the mapping of geogenic radon in the soil and they were combined to calculate the probability of exceeding a specified critical threshold that might cause concern for human health. The study showed that emanation of radon gas radon was also dependent on geological structure and lithology. The results have provided insight into the influence of basement geochemistry on the spatial distribution of radon levels at the soil/atmosphere interface and suggested that knowledge of the geology of the area may be helpful in understanding the distribution pattern of radon near the earth’s surface.     

Geochemistry of granites and metasediments of the urban area of Vila Real (northern Portugal) and correlative radon risk

Radon concentration was evaluated in dwellings of the urban area of Vila Real (Northern Portugal). The area is mainly composed of Hercynian granites and Cambrian metasediments, and CR-39 passive detectors (n = 112) were used for the purpose. The results obtained in winter conditions suggest that the most productive geological unit is the Hercynian granite G1 (geometric mean of 364 Bq/m³), while Cambrian metasediments of the Douro Group show the lowest average indoor radon concentration (236 Bq/m³). The geological, geochemical and radiological data obtained suggest that the most effective control on the radon concentrations of the area is related with the uranium content of the rocks; indeed, the highest contents were observed in granite G1 (21 ppm) and the lowest in the metasediments (3 ppm). This is also confirmed by the results obtained for groundwater, where granites present the highest concentrations of dissolved radon (up to 938 Bq/l), uranium (5–18 ppb) and gross α activities (0.47–0.92 Bq/l). No important radiometric anomalies were found in relation with geological structures such as faults, veins and contacts, but a moderate increase of the uranium content can occur locally in such structures. Petrographic observations and SEM studies show that uranium is mainly contained within the rock in heavy accessory minerals (apatite, zircon, monazite, xenotime), which reduces radon emanation. Notwithstanding, due to the high U contents granites show a significant potential to induce indoor radon concentrations in dwellings in excess of the recommended value of 400 Bq/m³. Overall, we can conclude that the region of Vila Real presents a moderate to high radon risk in dwellings and groundwater.