60～70oS臭氧总量的QBO和ENSO信号

本文利用Ｎｉｍｂｕｓ－７上搭载的臭氧总量观测光谱仪（ＴＯＭＳ）得到的６０～７０ｏＳ纬圈中臭氧总量资料,分析研究了该地区臭氧总量准两年振荡（ＱＢＯ）和ＥＮＳＯ信号的纬向分布,指出在该纬圈臭氧总量的长期变化中包含着的ＱＢＯ和ＥＮＳＯ信号。同时,本文还分析研究了沿纬圈分布的大气臭氧总量季节变化和长期变化趋势,指出在该纬圈各个季节中臭氧总量呈下降趋势,以６０～１００ｏＷ十月份的下降最大,达到－９．３ＤＵ／ａ。研究同时表明：臭氧总量季节变化、长期变化趋势、以及ＱＢＯ信号的纬向分布都在西南极上空出现异常。本文对此进行了讨论,认为这是西南极海陆分布调整大气环流及大气波动造成对臭氧总量分布和变化的影响     

从雨云7号TOMS资料推算出臭氧总量变化趋势

雨云７号卫星上的臭氧总量测绘分光仪（ＴＯＭＳ），１１年多以来一直测量着全球臭氧柱总量。最近在资料分析上加以改进，得到一种用以确定并消除定标飘移的技术，使记录尽头处的资料相对于记录开头的资料来说可精确到±１．３％（２σ）。由ＴＯＭＳ总臭氧资料时间序列已拟合得出一个统计模式，其中包括季节变化项、线性趋势项、准２年振荡（ＱＢＯ）项、太阳活动周项以及二阶自回归噪音项。就这个统计模式拟合于６５°Ｎ到６５°Ｓ纬圈之间平均的ＴＯＭＳ资料来看，所得到的线性趋势项为－０．２６±０．１４％／年，即从１９７８年１１月到１９９０年５月共１１．６年中变化－３％。这种变化趋势在赤道近于零（０．０００２±０．２％／年），向两极增加。在５０°Ｎ年平均趋势为－０．５±０．２１％／年。在这１１．６年期间５０°Ｎ的趋势，表现出强烈的季节变化，在冬季和初春（即２、３月份）大于－０．８％／年，在夏季（７、８月份）约为－０．２％／年。     

10──20天准双周振荡的经向传播及地理特征

本文采用ＥＣＭＷＦ１９８３年７月１日至９月１２日逐日２００ｈＰａ纬向风场资料，用复经验正交方法讨论了１０－２０天低频振荡的经向传播及地理特征。结果表明：（１）１０－－２天振荡有三个显著区域：贝加尔湖附近地区；赤道９０°Ｅ附近以及新加坡、马来西亚地区；８０－１００°Ｅ，２２－３２°Ｎ之间。（２）源于较高纬度地区的振荡与源于赤道附近地区的振荡在１０５°Ｅ，１７—２３°Ｎ附近同位相相遇，在９０°Ｅ，２０°Ｎ附近反位相相叠加，振荡相互削弱，在２５°Ｎ附近同位相相遇。（３）从振荡位相来看，中南半岛东南部、马来西亚北部、菲律宾以西区域的振荡向北传播到中国东南沿海，向西传播到孟加拉湾印度半岛；２０°Ｎ以南低纬度地区的振荡很少能传播到８０°Ｅ以东３０°Ｎ附近地区；位于９０－９５°Ｅ，２５－２７°Ｎ之间的振荡以及贝加尔湖附近地区的振荡可以向南北两个方向传播。     

对流层大气环流的甚低频振荡

对１９５１—１９９２共４２ａ５００ｈＰａ北半球高度场的月平均资料进行了纬圈谐波分析，计算了３５°Ｎ与５５°Ｎ超长波振幅及位相，以及３５—５５°Ｎ北半球月平均纬向风距平百分比。对超长波振幅及纬向风距平百分比做了小波转换。结果表明，对流层大气环流变化中存在３种准周期性的甚低频振荡：１．年代际的振荡；２．准２ａ周期振荡（ＱＢＯ）；３．半年韵律。同时发现对流层ＱＢＯ和平流层赤道纬向风ＱＢＯ之间可能没有联系。     

观测表明1999年南极臭氧洞变小

从ＮＡＳＡ卫星地球探测卫星（ＴＯＭＳ－ＥＰ）装载的臭氧总量绘图光谱仪（ＴＯＭＳ）获得的资料表明，１９９９年南极上空臭氧低值区小于去年。ＮＯＡＡ设在南极的气球探测所得资料也表明南极的臭氧洞尽管还是很大，但比去年有所减小。尽管南极臭氧洞的微小年际变化是预料中的，但与１９９８年比１９９９年臭氧洞不再加深加大是个好征兆。美国科罗拉多州博尔德气候监测与诊断实验室的ＤａｖｉｄＨｏｆｍａｎｎ说∶“该测量事实说明平流层中的氯不再增加，这是臭氧层恢复的第一步。现在我们要做的是，密切监视大气中的臭氧洞和破坏臭氧的物…     

赤道西太平洋强东风带特征及其形成机制的诊断分析

利用１９９３年ＥＮＳＯ事件（４月）爆发前酝酿阶段，ＴＯＧＡ／ＣＯＡＲＥ关键区强化期（１９９２年１１月－１９９３年２月）立体观测实验“向阳红五号”科学考察船定点（１５５°Ｅ，２°Ｓ）高空大气探测资料，分析了西太平洋暖海域上空对流上升区西侧风的垂直变化，指出：对流层上、下部各有一强风带，随着海－气ＥＮＳＯ异常的发展，高空强东风带和低空强西风带均呈增强趋势，最强时分别连续１４天和１８天达到急流标准，占相     

斯堪的那维亚臭氧亏损和地面加热

对ＮＡＳＡ的ＴＯＭＳ臭氧资料进行分析后指出：冬季在北极的斯堪的那维亚地区存在一个明显的臭氧亏损区，亏损区的中心值达－５０ ＤＵ，相当于该区域平均值的 １５％。对臭氧亏损和北大西洋海温的东西向差异作相关分析得到：其季节变化的相关系数为－０．９６，逐月（ １６８个月）变化的相关系数为－０．７０。同样对臭氧亏损与地面加热进行相关分析后指出：斯堪的那维亚地区的臭氧亏损和该地区地面的热通量关系极其密切，其相关系数均在－０．８７以上。由此我们认为：北大西洋暖流向北输送能量，引起斯堪的纳维亚地区地面加热，由此造成了冬季该地区的臭氧亏损。     

东亚和西北太平洋地区气候的准10年尺度振荡及其可能机制

本文基于对气候、大气环流和海表水温的资料分析以及简单的理想化海气耦合模式的分析,研究了东亚和西北太平洋地区气候的准１０年振荡及其可能机制。研究表明,东亚和西北太平洋地区的气候（降水和地面气温等）和大气环流（环流指数和副高活动等）的演变都有明显的准１０年振荡;同赤道太平洋ＳＳＴＡ主要为ＥＮＳＯ循环不同,西北太平洋ＳＳＴＡ主要表现为准１０年尺度的振荡,且同气候和大气环流的准１０年变化密切相关;中纬度海－气相互作用可产生一种甚低频耦合波（１０年左右周期）,它可能是海气系统准１０年振荡的重要机制之一     

南极臭氧的短期气候变化特征

利用1957～1992年南极地区大气臭氧总量地面观测站资料，对南极地区臭氧的时空变化特征进行了研究。结果表明，虽然近35年来南极地区的大气臭氧有较明显的减小趋势，但在不同地区、时段和季节，其变化趋势也不同。近年来南极地区大气臭氧的显著亏损，主要是由南极臭氧洞的形成和发展所造成的。南极地区的大气臭氧存在明显的年振荡、准20个月和准30个月的振荡周期。臭氧变化与天文日照、平流层温度场、平流层冰晶云及人类活动排放到大气中的氟氯烃和溴化烃等污染物质有关。     

TBO的原因－异常东亚冬季风与ENSO循环的相互作用

基于对 ＮＣＥＰ／ ＮＣＡＲ再分析资料以及其他资料（ＯＬＲ，降水和气温等）的分析研究，结果表明东亚和西北太平洋地区的对流层环流和气候变化都有明显的准两年振荡（ＴＢＯ）特征。同时，异常东亚冬季风可以影响次年夏季的大气环流和气候变化，特别是在东亚地区；而异常东亚冬季风和ＥＮＳＯ循环间又有明显相互作用：持续的强（弱）东亚冬季风通过海─气相互作用可以激发 Ｅｌ Ｎｉ　ｏ（Ｌａ Ｎｉ　ａ）， Ｅｌ Ｎｉ　ｏ（Ｌａ Ｎｉ　ａ）反过来又可通过遥相关或遥响应而导致东亚冬季风偏弱（强）。强或弱的冬季风和ＥＮＳＯ循环是相互衔接在一起的，因此可以认为异常东亚冬季风与ＥＮＳＯ循环的相互作用是ＴＢＯ对流层准两年振荡）的基本原因。     

香河地基观测臭氧柱总量数据分析及臭氧变化趋势研究

大气臭氧变化在全球气候和环境中具有重要作用,是当今大气科学领域的重要研究对象之一。对比分析了中国科学院大气物理研究所河北香河大气综合观测试验站2014～2016年Dobson和Brewer两种臭氧总量观测仪器探测结果的一致性,并使用1979～2016年Dobson观测数据分析了香河地区臭氧总量的长期变化趋势。结果表明:进行有效温度修正后,两种臭氧总量仪器观测结果一致性较好,平均偏差仅为-0.14DU(多布森单位),平均绝对偏差为8.00 DU,标准差为36.09 DU,相关系数达0.964。整体来说,两类仪器观测臭氧总量吻合较好。SO2浓度对Dobson仪器数据精度有一定影响,两组仪器数据在SO2浓度为0～0.2DU、0.2～0.4DU和0.4DU大气条件情况下的平均偏差分别为4.8 DU、7.0 DU和8.0 DU,平均偏差随SO2浓度升高而增大。过去38年香河地区的臭氧总量季节差异性强,春、冬两季臭氧总量高,夏、秋两季臭氧总量相对低,季节变化趋势差异明显。从长期变化上看,臭氧总量变化波动有不同的周期,在4个大的时间段变化趋势不同,2000～2010年臭氧层有显著恢复,但最近几年又有变薄的趋势。     

地基与星载仪器观测大气臭氧总量分析

本文选取多个臭氧总量观测站点,采用"三重制约法"分别对下列3组仪器观测臭氧总量数据进行统计分析,解算出不同观测资料的误差标准差,进而对比研究各种仪器的精度特征:1)1996~2003年期间地基WOUDC(World Ozone and Ultraviolet Radiation Data Centre)观测网络仪器(包括Brewer、Dobson和Filter臭氧测量仪)与星载TOMS(Total Ozone Mapping Spectrometer)和GOME(The Global Ozone Monitoring Experiment)仪器;2)2004~2013年期间WOUDC与星载OMI(ozone monitoring instrument)和SCIAMACHY(scanning imaging absorption spectrometer for atmospheric chartography)仪器;3)2004~2013年期间地基SAOZ(Système D’Analyse par Observations Zénithales)与星载OMI和SCIAMACHY仪器。结果表明,1996~2003年期间TOMS V8和GOME观测精度相当,分别为7.6±2.8 DU/46(其中,7.6±2.8 DU为所分析站点观测资料的平均精度及其标准差,46为站点数目)和7.6±1.5 DU/46。TOMS V8观测精度优于TOMS V7(8.5±3.0 DU/46),验证了前者对后者有所改进。2004~2013年期间OMI和SCIAMACHY在WOUDC地基站点观测精度接近,分别为6.6±1.4 DU/21和6.0±1.6 DU/21。SAOZ地基仪器精度为8.4±3.6 DU/8。对于3类WOUDC地基仪器,Brewer站点观测资料的平均精度最优(7.9±3.3 DU/12),Dobson次之(8.7±2.3 DU/19),Filter最差(14.7±4.0 DU/15)。相比于卫星,3种地面仪器观测平均精度较差(10.5±4.3 DU/46),这主要是由于Filter精度较差引起。中国境内的瓦里关(Brewer)、香河(Dobson)和昆明(Dobson)3个地基站点仪器观测精度均较优,分别为7.8 DU、6.7 DU和6.6 DU。尽管不同站点之间存在一定差异,但整体来说,地基与卫星仪器在中国境内3个站点观测臭氧总量吻合较好。     

中国4个地点地基与卫星臭氧总量长期观测比较

对我国河北香河、云南昆明、青海瓦里关及黑龙江龙凤山地基观测臭氧总量与不同时期、不同卫星反演的产品差别特点进行比较,评估地基和卫星观测臭氧总量数据的质量信息以及近30年来我国不同区域臭氧总量的变化趋势特征。结果表明:4个站点的地基与卫星观测臭氧总量的绝对和相对差别分别为-5~10 DU和-5%~4%;日平均相对差别基本上呈现随机分布特征。TOMS算法反演的卫星臭氧总量与地基差别总体上要优于与DOAS算法反演的同期产品。地基与卫星臭氧总量差别呈明显的区域特点,可能反映了卫星反演计算中所需的臭氧、温度垂直分布等初始条件的纬度分布差异对卫星产品精度的影响。在过去30年,4个站点的臭氧总量在经历1993年前的显著降低后于1995—1996年逐渐回升,而瓦里关站在2001年前后的回升更为明显。     

The Relationship between Total Ozone and Local Climate at Kunming Using Dobson and TOMS Data

This paper uses Dobson spectrometer total ozone data,Total Ozone Mapping Spectrometer(TOMS) data and radiosonde reports from Kunming,which is located in southwest China,from 1980 to 2008 to analyze the total ozone-climate relationship.The total ozone decadal long-term trend and abrupt change were studied using enhanced Dobson data whose missing data were amended by the TOMS data.Stepwise linear regression was used for the selection of the key factors that influence total ozone,including temperatures,geopotential heights,depressions of the dew point,wind velocities,and total solar radiation.The relationship between the selected factors and total ozone was analyzed using the methods of stepwise regression and partial least squares regression(PLSR).Results showed that although the PLSR method was slightly better and more reasonable to study the relationship than stepwise regression,while the two regression results were only slightly different.It was also suggested that local climate,especially local circulation and temperature,were important for the variations in total ozone,and the local climate could almost linearly explain 80% of the variance of total ozone.The relationship also indicated that the abrupt change of total ozone in the year 1994 may be related to abrupt local climate change.     

Formation of the Summertime Ozone Valley over the Tibetan Plateau: The Asian Summer Monsoon and Air Column Variations

The summertime ozone valley over the Tibetan Plateau is formed by two influences,the Asian summer monsoon(ASM) and air column variations.Total ozone over the Tibetan Plateau in summer was ～33 Dobson units(DU) lower than zonal mean values over the ocean at the same latitudes during the study period 2005-2009.Satellite observations of ozone profiles show that ozone concentrations over the ASM region have lower values in the upper troposphere and lower stratosphere(UTLS) than over the non-ASM region.This is caused by frequent convective transport of low-ozone air from the lower troposphere to the UTLS region combined with trapping by the South Asian High.This offset contributes to a ～20-DU deficit in the ozone column over the ASM region.In addition,along the same latitude,total ozone changes identically with variations of the terrain height,showing a high correlation with terrain heights over the ASM region,which includes both the Tibetan and Iranian plateaus.This is confirmed by the fact that the Tibetan and Iranian plateaus have very similar vertical distributions of ozone in the UTLS,but they have different terrain heights and different total-column ozone levels.These two factors(lower UTLS ozone and higher terrain height) imply 40 DU in the lower-ozone column,but the Tibetan Plateau ozone column is only ～33 DU lower than that over the non-ASM region.This fact suggests that the lower troposphere has higher ozone concentrations over the ASM region than elsewhere at the same latitude,contributing ～7 DU of total ozone,which is consistent with ozonesonde and satellite observations.     

QBO Signal in total ozone over Tibet

1. IntroductionOzone is one of the trace gases in the atmosphere distributed in 10--50 km altitude withthe maximum in 20--28 km. Ozone is significant in the following three aspects impacting theclimate and environment: 1) Ozone absorbs harmful solar ultra--violet radiation for protecting the ecological system on the Earth; 2) ozone heats the stratosphere and forces the circulation systems in this layer; 3) ozone variation in the stratosphere can change the incomingradiation at the surface leve…     

青藏高原臭氧的准两年振荡

通过对臭氧卫星观测资料及大气环流资料的分析,研究了青藏高原上空臭氧的季节和年际变化.通过分析青藏高原地区臭氧准两年振荡(QBO),并与同纬度无山区及赤道地区臭氧QBO进行比较,指出:青藏高原臭氧QBO的平均周期为29个月,平均振幅为8DU.青藏高原臭氧QBO变化位相与热带平流层纬向风场QBO相反,即热带平流层纬向西风时,青藏高原上空臭氧总量偏小,东风时臭氧总量偏大.还讨论了与青藏高原臭氧QBO相关的大气环流物质输送理论.     

The Tibetan Ozone Low and Its Long-Term Variation During 1979–2010

A Tibetan ozone low was found in the 1990s after the Antarctic ozone hole.Whether this ozone low has been recovering from the beginning of the 2000s following the global ozone recovery is an intriguing topic.With the most recent merged TOMS/SBUV(Total Ozone Mapping Spectrometer/Solar Backscatter Ultra Violet) ozone data,the Tibetan ozone low and its long-term variation during 1979-2010 are analyzed using a statistical regression model that includes the seasonal cycle,solar cycle,quasi-biennial oscillation(QBO),ENSO signal,and trends.The results show that the Tibetan ozone low maintains and may become more severe on average during 1979-2010,compared with its mean state in the periods before 2000,possibly caused by the stronger downward trend of total ozone concentration over the Tibet.Compared with the ozone variation over the non-Tibetan region along the same latitudes,the Tibetan ozone has a larger downward trend during 1979-2010,with a maximum value of-0.40±0.10 DU yr 1 in January,which suggests the strengthening of the Tibetan ozone low in contrast to the recovery of global ozone.Regression analyses show that the QBO signal plays an important role in determining the total ozone variation over the Tibet.In addition,the long-term ozone variation over the Tibetan region is largely affected by the thermal-dynamical proxies such as the lower stratospheric temperature,with its contribution reaching around 10% of the total ozone change,which is greatly different from that over the non-Tibetan region.     

云对中国区域卫星观测臭氧总量精度影响的检验分析

根据卫星和地基观测, 比较了我国香河、 昆明、 瓦里关和龙凤山四个站点臭氧总量自1979年以来的变化。卫星与地基观测的臭氧总量长期趋势比较一致, 表明臭氧总量均有下降趋势, 但是卫星与地基各自观测的结果仍存在着显著的差别。为研究卫星与地基臭氧总量的差别, 以地基观测臭氧总量为参考, 检验云对历史TOMS (Total Ozone Mapping Spectrometer) 和GOME (Global Ozone Monitoring Experiment) 臭氧总量精度的影响。结果显示: 云 (云量或云顶高度) 增加了卫星臭氧总量误差, 降低数据精度。随着地面云量的增加, TOMS、 GOME臭氧总量相对误差在上述四个地点呈现明显的上升趋势 (瓦里关最为明显), 但最大变化幅度没有超过2.0%。TOMS臭氧总量相对误差随地面云量变化呈现区域性特点, 香河与龙凤山 (代表着中纬度高臭氧总量区域)、 昆明与瓦里关 (代表中、 低纬度高原低臭氧总量区域) 分别为两个变化特点接近的区域。GOME臭氧总量相对误差与云之间关系的区域特征不明显。利用卫星遥测FRESCO (Fast Retrieval Scheme for Clouds from the Oxygen A\|band) 云信息检验GOME卫星臭氧总量精度的表明, 只有当云量大于5成后GOME臭氧总量才显示出相对误差增加的现象, 但无明显趋势; 随着FRESCO云顶高度的增加, GOME臭氧相对误差在香河、 瓦里关均呈现明显的上升趋势并有3%左右幅度的变化。TOMS臭氧总量相对误差随着地面有效反射率的增加而增大, 且误差幅度超过2%; TOMS\|N7臭氧总量比TOMS\|EP约高2.0%~3.0%。分析还表明, 云内和云以下臭氧柱浓度在反演的卫星臭氧总量中的贡献很可能被高估了。     

Statistical analysis and comparison of external factor effects on the total ozone field over the Russian territory in 1973–2007

The analysis of external factors, which are most significant for the formation of the monthly mean total ozone (TO) field and ozone transport over the Russian Federation, based on observation data obtained from about 30 ground-based stations of the ozonometric network averaged over a year, December through March and June through August, over five climatic regions, is considered. Performed spectrum and discriminant analysis allowed obtaining quantitative estimates of the impact of the Arctic Oscillation, deviation of the winter temperature of the lower polar stratosphere, quasi-biennial oscillations (QBO), 11-year solar cycle, El Niño-Southern Oscillation (ENSO) on the TO and to assess the regional differences in the effects of these factors. In December–March, in the years with a negative Arctic Oscillation phase, warm stratosphere, and the easterly QBO phase (QBO-E), the ozone content increases significantly relative to the opposite phases of oscillations on average by 35, 28, and 26 Dobson units (DU), respectively. The spectra, similar to the discriminant function, demonstrate strong influence of the 11-year solar cycle and QBO on the TO even in the summer months, while the QBO is more pronounced in the eastern part of the Russian Federation. The ENSO effect was not singled out against the general “noisy” background of the cold six-month period, when many atmospheric processes become active: however, during the summer months, in warm periods of the ENSO, the TO, at the 97% significance level, increases over most of the Russian area. The rest of the obtained results are significant at the 95–99.9% level.