Two-moment bulk stratiform cloud microphysics in the grid-point atmospheric model of IAP LASG (GAMIL)

A two-moment bulk stratiform microphysics scheme, including recently developed physically-based droplet activation/ice nucleation parameterizations has been implemented into the Grid-point Atmospheric Model of IAP LASG (GAMIL) as an effort to enhance the model’s capability to simulate aerosol indirect effects. Unlike the previous one-moment cloud microphysics scheme, the new scheme produces a reasonable representation of cloud particle size and number concentration. This scheme captures the observed spatial variations in cloud droplet number concentrations. Simulated ice crystal number concentrations in cirrus clouds qualitatively agree with in situ observations. The longwave and shortwave cloud forcings are in better agreement with observations. Sensitivity tests show that the column cloud droplet number concentrations calculated from two different droplet activation parameterizations are similar. However, ice crystal number concentration in mixed-phased clouds is sensitive to different heterogeneous ice nucleation formulations. The simulation with high ice crystal number concentration in mixed-phase clouds has less liquid water path and weaker cloud forcing. Furthermore, ice crystal number concentration in cirrus clouds is sensitive to different ice nucleation parameterizations. Sensitivity tests also suggest that the impact of pre-existing ice crystals on homogeneous freezing in old clouds should be taken into account.     

Sensitivity Study of Anthropogenic Aerosol Indirect Forcing through Cirrus Clouds with CAM5 Using Three Ice Nucleation Parameterizations

Quantifying the radiative forcing due to aerosol–cloud interactions especially through cirrus clouds remains challenging because of our limited understanding of aerosol and cloud processes. In this study, we investigate the anthropogenic aerosol indirect forcing (AIF) through cirrus clouds using the Community Atmosphere Model version 5 (CAM5) with a state-of-the-art treatment of ice nucleation. We adopt a new approach to isolate anthropogenic AIF through cirrus clouds in which ice nucleation parameterization is driven by prescribed pre-industrial (PI) and presentday (PD) aerosols, respectively. Sensitivities of anthropogenic ice AIF (i.e., anthropogenic AIF through cirrus clouds) to different ice nucleation parameterizations, homogeneous freezing occurrence, and uncertainties in the cloud microphysics scheme are investigated. Results of sensitivity experiments show that the change (PD minus PI) in global annual mean longwave cloud forcing (i.e., longwave anthropogenic ice AIF) ranges from 0.14 to 0.35 W m^–2, the change in global annual mean shortwave cloud forcing (i.e., shortwave anthropogenic ice AIF) from–0.47 to–0.20 W m^–2, and the change in net cloud forcing from–0.12 to 0.05 W m^–2. Our results suggest that different ice nucleation parameterizations are an important factor for the large uncertainty of anthropogenic ice AIF. Furthermore, improved understanding of the spatial and temporal occurrence characteristics of homogeneous freezing events and the mean states of cirrus cloud properties are also important for constraining anthropogenic ice AIF.     

Characterization of cloud microphysical properties in different cloud types over East Asia based on CloudSat/CALIPSO satellite products

利用CloudSat/CALIPSO卫星资料,本文揭示了东亚三个代表性区域的云微物理属性,为评估和改进模式云微物理过程提供重要的观测基础.研究的云微物理量包括云水/冰质量,数浓度和有效半径.研究表明:暖云中云水质量和数浓度随高度增加而减小,有效半径处于8-14μm范围.对于冰云,云冰质量和有效半径随高度增加而减小,而数浓度在垂直方向上变化不大.此外,云微物理属性在不同云型之间存在显著差异:积云的云水质量和数浓度最大,而卷云的云水质量和数浓度最小.从三个区域的对比结果来看,相比于华东和西北太平洋地区,青藏高原地区暖云的云水质量和数浓度较小,而冰云的则较大.     

Latent ice-forming nuclei in the Pacific Northwest

Some cloud condensation nuclei (CCN) constitute a reservoir of latent ice-forming nuclei (IFN) active by condensation-followed-by-freezing and by sorption. Evaporated droplets occasionally left aerosol particles that acted as sorption IFN at temperatures as high as −5°C and water vapor supersaturation over ice of 0.2%. The newly formed aerosol particles (residues of evaporated droplets) are all mixed particles. The discovery of IFN produced from CCN promotes new insights into the process of ice formation in clouds; in an evaporating parcel of a cloud the rate of formation of ice particles will be enhanced by continuous production of IFN. Aerosol particles left behind after evaporation of a cloud may provide a source of IFN for formation of some of the cirrus clouds.     

Model studies on the effect of nitric acid vapour on cirrus cloud activation

The effect of elevated nitric acid concentrations on cloud particle number concentrations and sizes of mixed phase cirrus cloud (containing both supercooled liquid and frozen ice particles) is studied using a detailed multicomponent condensation model. Our model calculations suggest that high nitric acid volume mixing ratios (VMRs), corresponding to upper tropospheric measurements, can increase the ice crystal number concentrations substantially especially in the case of freezing of non-activated solution droplets (as opposed to freezing of supercooled cloud droplets). This is due to increased droplet sizes caused by nitric acid absorption and the resulting uptake of water.     

热带深对流云砧数值模拟及云凝结核数浓度对其影响的初步试验

利用中国科学院大气物理研究所发展的三维强风暴模式，对Egrett Microphysics Experiment with Radiation Lidar and Dynamics（EMERALD）试验期间的一次长寿命热带深对流个例进行对流产生、发展、消亡过程以及云砧的数值模拟，并与实测资料［包括C波段双线偏振雷达图像资料、机载云粒子成像仪（CPI）探测的云砧卷云微物理特性以及激光雷达探测的云砧宏观特性资料］进行了细致的对比，然后通过改变模式中最大云滴数浓度进行有关云凝结核数浓度影响云砧卷云冰晶含水量和数浓度的敏感性试验。模式较好地模拟出系统的一些重要宏观特征，如爆发性增长阶段、各高度雷达水平反射率因子的最大值、对流云主体移动方向、云砧底部和顶部高度。对云砧冰相粒子含水量、数浓度以及平均直径等微观特征的模拟结果与实测也比较接近。对于本文个例而言，异质核化为冰晶形成的最主要方式，其次为过冷云滴的均质核化。敏感性试验结果表明:当云凝结核数浓度增加时，爆发性增长阶段的垂直速度减小，使得对流云从中低层向高层的水物质输送量减少，从而使云砧卷云冰晶的数量减少。     

京津冀地区夏季降水冰云和非降水冰云云特征对比分析

利用2013～2016年的Aqua MODIS卫星和CloudSat卫星的二级产品资料,对发生在京津冀地区夏季的降水冰云和非降水冰云进行了统计。基于此,对比分析了两类冰云的云类型,研究了二者在云特征参数、云层数及垂直结构上的差异,并且探究了二者在不同通道下云特征参数的相对大小。结果表明:1）京津冀地区的降水冰云以深对流云和雨层云为主,分别占48.63%和34.65%,而非降水冰云以高层云和卷云为主,分别占55.62%和31.58%。2）降水冰云和非降水冰云的平均云顶温度、云顶高度、光学厚度、积分云水总量、有效粒子半径分别为230.99 K、10.90 km、53.26、937.98 g/m2、31.45m和236.17 K、10.10 km、12.81、209.00 g/m2、27.54 μm。3）降水冰云以单层云为主,占80.39%,双层云占18.75%;而非降水冰云仍以单层云为主,占85.35%,双层云则占14.38%,比降水冰云低。4）相较于非降水冰云,降水冰云中卷云和高积云云体位置较高,而高层云和深对流云位置较低。5）随高度变化,降水冰云冰水含量是双峰结构,而非降水冰云是单峰结构;二者的粒子数浓度则差异不大;非降水冰云的粒子有效半径在5～7.5 km随高度变化不大,而降水冰云则随高度减小。6）降水冰云的积分云水总量、光学厚度和粒子有效半径>≥模态[、、分别代表该云特征参数在1.6、2.1、3.7 μm通道中的数值,当n=1, 2, 3时,分别代表光学厚度（b₁）、积分云水总量（b₂）、有效半径这三种（b₃）]的比例都高于非降水冰云,而二者在云参数≥≥模态的比例则有差异。     

基于CloudSat资料对中国低纬度陆地区域卷云物理特征的研究

利用2008年9月—2016年8月的CloudSat卫星资料对发生在我国低纬度陆地区域(5°~36.5°N,78°~124°E)的卷云物理特征进行统计分析,并分别讨论东部沿海、中部、西部3个子区域的卷云物理特征的季节变化。结果表明:卷云的整层发生率西部地区整体低于中部与东部沿海地区。3个子区域整层发生率均在夏季最高、冬季最低。卷云的主要发生高度在5.04~18.71 km,垂直分布中卷云发生率的最大值出现在春季中部地区,为15.34%,高度为9.83 km。冰水路径最大值出现在夏季的东部沿海,液水路径最大值在秋季的西部地区。冰水含量、冰粒数浓度、冰粒有效半径的主要分布高度与卷云的发生高度一致,液水含量、液滴数浓度、液滴有效半径的主要分布高度在5.04~9.35 km。3个子区域卷云冰水含量、冰粒数浓度、冰粒有效半径垂直分布中大多集中在中上部;液水含量垂直分布主要集中在分布高度的中下部。四季卷云雷达反射率因子的最大值在-19.89~-16.78 dBZ,分布高度在7.19~10.55 km。     

Cirrus Cloud Macrophysical and Optical Properties over North China from CALIOP Measurements

Two years of mid-latitude cirrus cloud macrophysical and optical properties over North China are described from Earth-orbiting Cloud-Aerosol Lidar with Orthogonal Polarization(CALIOP) satellite measurements. Global cloud climatological studies based on active remote sensing data sets benefit from more accurate resolution of vertical structure and more reliable detection of optically thin layers.The mean values for cirrus cases over North China are 0.19±0.18 for infrared emittance,0.41±0.68 for visible optical depth, 0.26±0.12 for integrated depolarization ratio,and 0.72±0.22 for integrated color ratio.When studied using reasonable assumptions for the relationship between extinction and ice crystal backscatter coefficients,our results show that most of the cirrus clouds profiled using the 0.532μm channel data stream correspond with an optical depth of less than 1.0.The dependence of cirrus cloud properties on cirrus cloud mid-cloud temperature and geometry thickness are generally similar to the results derived from the ground-based lidar, which are mainly impacted by the adiabatic process on the ice cloud content.However,the differences in macrophysical parameter variability indicate the limits of spaceborne-lidar and dissimilarities in regional climate variability and the nature and source of cloud nuclei in different geographical regions.     

Simulation of the influence of aerosol particle characteristics on clouds and precipitation with LM-SPECS: Model description and first results

The novel model system LM-SPECS is presented combining a spectral bin microphysics scheme and the three-dimensional Lokalmodell (LM, today called COSMO) of the German Weather Service (“Deutscher Wetterdienst”). The model is designed to investigate in detail the interaction of atmospheric aerosol particles, clouds and precipitation. The microphysics scheme includes a combined spectrum of wetted aerosols, cloud droplets and rain drops. As a first application of the model, sensitivity studies on an artificial deep convective cloud were done. The results produced by LM-SPECS are satisfying. The studies show, e.g., that a diminished initial particle number leads to larger cloud droplets and thus to a higher efficiency of coalescence. This results in a larger amount of precipitation. Furthermore, studies on mixed phase clouds show the influence of varying ice nuclei, such as bacteria, kaolinite and soot, on cloud properties. Here, a more effective freezing leads to an increased number of ice particles with smaller radii. The results point to the importance of a detailed knowledge of the underlying microphysical processes in order to understand the formation of clouds and precipitation more accurately. Though to date the model was applied to artificial cases only, the use of the mesoscale weather model allows for more complex realistic cases which are subject to further studies.     

CloudSat/CALIPSO卫星资料分析云的全球分布及其季节变化特征

全球气候模式（GCM）中云的参数化方案具有不确定性,了解云的时、空变化能为参数化方案提供有效参考。利用搭载在属于A-Train卫星序列的CloudSat和CALIPSO上的94 GHz云廓线雷达（CPR）以及正交极化云-气溶胶激光雷达（CALIOP）联合的2级云分类产品,分析了2007年3月-2010年2月8种云类及三相态的云量地理分布、纬向垂直分布的季节变化特征以及云层分布概率。结果发现,卷云的分布体系与深对流云相似,主要集中在西太平洋暖池、全球各季风区及赤道辐合带,分布格局与气压带、风带季节性移动一致。层云与层积云主要分布在中低纬度非季风区以及中高纬度的洋面上。高积云与高层云的分布形成明显的海陆差异,雨层云与积云的分布形成明显的纬度差异。冰云分布与卷云相似,云高随纬度递增而递减;水云分布与层积云相似,平均分布于2 km高度;混合云集中于高纬度地区及赤道辐合带,中纬度地区随纬度变化集中于海拔0-10 km的弧形带。层状云多以多层云形式出现,积状云多以单、双层云的形式出现,层状云的云重叠现象比积状云更显著。积状和层状云的分布特征与积云和层云降水的分布特征基本一致,验证了不同类型降水的卫星观测结果,同时为气候模式的云量诊断方案提供对比验证的数据。      

Simulation of the influence of aerosol particle characteristics on clouds and precipitation with LM-SPECS: Model description and first results

The novel model system LM-SPECS is presented combining a spectral bin microphysics scheme and the three-dimensional Lokalmodell (LM, today called COSMO) of the German Weather Service (“Deutscher Wetterdienst”). The model is designed to investigate in detail the interaction of atmospheric aerosol particles, clouds and precipitation. The microphysics scheme includes a combined spectrum of wetted aerosols, cloud droplets and rain drops. As a first application of the model, sensitivity studies on an artificial deep convective cloud were done. The results produced by LM-SPECS are satisfying. The studies show, e.g., that a diminished initial particle number leads to larger cloud droplets and thus to a higher efficiency of coalescence. This results in a larger amount of precipitation. Furthermore, studies on mixed phase clouds show the influence of varying ice nuclei, such as bacteria, kaolinite and soot, on cloud properties. Here, a more effective freezing leads to an increased number of ice particles with smaller radii. The results point to the importance of a detailed knowledge of the underlying microphysical processes in order to understand the formation of clouds and precipitation more accurately. Though to date the model was applied to artificial cases only, the use of the mesoscale weather model allows for more complex realistic cases which are subject to further studies.     

冰云短波辐射特性参数化

该文对卷云和高层云分别构造了15种冰晶尺度分布，3种云高和云厚，总共30种冰水含量、90种冰水程长模式。对尺度小于与大于30 μm的冰晶粒子的单次散射特性分别用表面积等效冰球Mie理论和射线光学理论进行计算。采用delta-Eddington法计算了在4种不同地面反射率下冰云的多重散射辐射传输特性，提出了冰云辐射特性的参数化公式，指出参数化公式可以用于气候模式或大气环流模式。     

大气冰核对雷暴云电过程影响的数值模拟

利用已有的二维雷暴云起、放电模式模拟了一次雷暴天气,并通过敏感性试验研究了冰核浓度变化对雷暴云动力、微物理及电过程的影响。结果表明：随着大气冰核浓度的增加,雷暴云发展提前,上升气流速度和下沉气流速度均呈现降低的趋势。大气冰核浓度提升有利于异质核化过程增强,冰晶在高温区大量生成,而同质核化过程被抑制,因此冰晶整体含量降低,引起低温区中霰粒含量降低和高温区中霰粒尺度降低。在非感应起电过程中,正极性非感应起电率逐渐减小,负极性非感应起电率逐渐增大。由于液态水含量随大气冰核浓度的增加逐渐降低,高温度冰晶携带电荷的极性由负转变为正的时间有所提前。在感应起电过程中,由于霰粒尺度减小及云滴的快速消耗,感应起电率极值逐渐降低。冰晶优先在高温区生成而带负电,不同大气冰核浓度下的雷暴云空间电荷结构在雷暴云发展初期均呈现负的偶极性电荷结构。在雷暴云旺盛期,随着冰核浓度增加,空间电荷结构由三极性转变为复杂四极性。在雷暴云消散阶段不同个例均呈现偶极性电荷结构,且随着冰核浓度的增加电荷密度值逐渐减小。     

CPR雷达探测北半球夏季多层云系结构统计特征分析

利用2007~2010年北半球夏季（6~8月）CloudSat卫星搭载的云廓线雷达（Cloud Profile Radar,CPR）探测结果对0°~60°N区域单层、双层和三层云系的水平分布、垂直结构特征及各云层云类组成、云水路径等物理量分布进行分析。云量的统计结果表明CPR探测的单层、双层和三层云系的云量分别为36.63%、8.26%和1.40%,云量的水平分布表明其高值区主要位于对流旺盛区域,且高值区的云层云顶高、厚度大,而低值区则多位于副热带高压区域。对不同云类的出现频率统计分析结果表明,单层云系中各云类的出现频率相近;多层云系的上层以卷云为主,下层以层积云为主。对比海陆差异发现洋面卷云和层积云的出现频率显著高于陆面,但高层云和高积云的出现频率低于陆面。云水路径分析表明,单层云系的冰水路径和液水路径均最大,而在多层云系中云层越高、厚度越大、冰水路径越大,液水路径则随着云层的降低增大。     

Relative importance of acid coating on ice nuclei in the deposition and contact modes for wintertime Arctic clouds and radiation

Aerosols emitted from volcanic activities and polluted mid-latitudes regions are efficiently transported over the Arctic during winter by the large-scale atmospheric circulation. These aerosols are highly acidic. The acid coating on ice nuclei, which are present among these aerosols, alters their ability to nucleate ice crystals. In this research, the effect of acid coating on deposition and contact ice nuclei on the Arctic cloud and radiation is evaluated for January 2007 using a regional climate model. Results show that the suppression of contact freezing by acid coating on ice nuclei leads to small changes of the cloud microstructure and has no significant effect on the cloud radiative forcing (CRF) at the top of the atmosphere when compared with the effect of the alteration of deposition ice nucleation by acid coating on deposition ice nuclei. There is a negative feedback by which the suppression of contact freezing leads to an increase of the ice crystal nucleation rate by deposition ice nucleation. As a result, the suppression of contact freezing leads to an increase of the cloud ice crystal concentration. Changes in the cloud liquid and ice water contents remain small and the CRF is not significantly modified. The alteration of deposition ice nucleation by acid coating on ice nuclei is dominant over the alteration of contact freezing.     

Impact of the Bergeron–Findeisen process on the release of aerosol particles during the evolution of cloud ice

The paper focuses on the redistribution of aerosol particles (APs) during the artificial nucleation and subsequent growth of ice crystals in a supercooled cloud. A significant number of the supercooled cloud droplets during icing periods (seeding agents: C₃H₈, CO₂) did not freeze as was presumed prior to the experiment but instead evaporated. The net mass flux of water vapour from the evaporating droplets to the nucleating ice crystals (Bergeron–Findeisen mechanism) led to the release of residual particles that simultaneously appeared in the interstitial phase. The strong decrease of the droplet residuals confirms the nucleation of ice particles on seeding germs without natural aerosol particles serving as ice nuclei. As the number of residual particles during the seedings did not drop to zero, other processes such as heterogeneous ice nucleation, spontaneous freezing, entrainment of supercooled droplets and diffusion to the created particle-free ice germs must have contributed to the experimental findings. During the icing periods, residual mass concentrations in the condensed phase dropped by a factor of 1.1–6.7, as compared to the unperturbed supercooled cloud. As the Bergeron–Findeisen process also occurs without artificial seeding in the atmosphere, this study demonstrated that the hydrometeors in mixed-phase clouds might be much cleaner than anticipated for the simple freezing process of supercooled droplets in tropospheric mid latitude clouds.     

NUMERICAL SIMULATION OF MICROPHYSICAL PROCESSES IN CUMULONIMBUS——PART Ⅰ:MICROPHYSICAL MODEL

A comprehensive parameterized model of microphysical processes in cumulonimbus clouds is presented.The transformation rates of the water contents and number concentrations of the cloud droplets,rain drops,ice crystals,graupels and hails are deduced on theoretical and experimental results for 26 kinds of micro-physical processes,which include condensation,deposition,evaporation,collection,ice nucleation,ice mul-tiplication,melting,freezing,and autoconversions of cloud to rain,ice to graupel and graupel to hail.     

Ice microphysics and climatic temperature feedback

The potential effects of ice microphysics involving ice crystal size distribution and ice water path (IWP) on climatic temperature perturbations are investigated by using a one-dimensional radiative-turbulent climate model. We define a mean effective size, denoting the width of ice crystals weighted by the geometric cross section area, to represent ice crystal size distribution. Based on aircraft measurements, both the mean effective size and IWP are related to temperature and may be parameterized as functions of temperature. The radiative properties of cirrus clouds are further parameterized in terms of these two basic cloud physics parameters. Using CO₂ doubling as the radiative forcing, feedbacks among temperature, the mean effective size and IWP, and the radiative properties of clouds are analyzed from the model results. We show that overall, a positive feedback associated with ice microphysics and the coupled radiative transfer is produced by temperature increase.     

Satellite remote sensing of the optical depth and mean crystal size of thin cirrus and contrails

Summary Crystal size and optical depth of optically thin cirrus clouds and contrails over the North Sea and Adriatic Sea on the 18^th of October 1989 are retrieved by comparison of NOAA AVHRR/2 brightness temperatures of channel 4 (9.97 µm–11.56 µm) and channel 5 (11.075 µm–12.76 µm) with one dimensional radiative transfer calculations. Measured brightness temperatures in all three infrared channels and their differences show higher values for contrails than for cirrus. The radiative properties of young contrails are consistent only, if smaller crystal size than those given for natural cirrus are adopted for the calculations. However, there is a continuous transition in radiative parameters between clouds classified as natural cirrus or contrails. For the test areas ice clouds are classified with respect to optical depth and mean crystal size. Finally infrared fluxes and heating rates in the spectral range 4 µm–40 µm are calculated for an atmosphere with a 500 m thick contrail or cirrus uncinus. At given ice content a far stronger atmospheric warming is found for a contrail with relatively small ice crystals: up to 80 K/day at cloud base for an ice content of 0.05 gm^–3 compared to 10 K/day for a cirrus uncinus with large crystals.With 11 Figures