Measurements of level-crossing statistics of concentration fluctuations in plumes dispersing in the atmospheric surface layer

The statistics of level crossings and local extremes in concentration fluctuations in plumes dispersing in the atmosphere have been investigated. A set of concentration fluctuation tracer experiments has been utilized to measure the statistical propertics of the upcrossing interval (inter-arrival time between consecutive concentration bursts), excursion duration (persistence or width of concentration bursts), and concentration amplitude (difference between the maximum and minimum concentrations between successive upcrossings) with respect to a range of concentration crossing levels. In particular, the effect of downwind distance and atmospheric stratification on the level-crossing statistics has been studied in detail. It is shown that the effect of increasing atmospheric stability on level-crossing statistics is similar to the effect of increasing distance from the source in the sense that level-crossing statistics of concentration fluctuations in stable stratification resemble those in neutral stratification, but at a greater downwind distance. It is also found that the distribution of the interval between consecutive upcrossings of a concentration level, as well as the duration of an excursion across a concentration level, can be approximated by a lognormal distribution, whereas the distribution of the concentration amplitude is best characterized by a gamma distribution. Some implications of these results for the modeling of level-crossing statistics of concentration fluctuations are discussed.