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Development of Emission Models and Improvement of Emission Data for Germany
Authors:R Friedrich  B Wickert  P Blank  S Emeis  W Engewald  D Hassel  H Hoffmann  H Michael  A Obermeier  K Schäfer  T Schmitz  A Sedlmaier  M Stockhause  J Theloke  F-J Weber
Institution:(1) Institut für Energiewirtschaft und Rationelle Energieanwendung (IER), Universität Stuttgart, D-70569 Stuttgart, Germany;(2) Fraunhofer-Institut für Atmosphäre Umweltforschung (IFU), D-82467 Garmisch-Partenkirchen, Germany;(3) Institut für Analytische Chemie, Universität Leipzig, D-04103 Leipzig, Germany;(4) Testzentrum Energietechnik, TÜV Rheinland Sicherheit und Umweltschutz GmbH, Am Grauen Stein, 51105 Köln, Germany;(5) Institut für Chemie der Belasteten Atmosphäre (ICG-2), Forschungszentrum Jülich, 52425 Jülich, Germany
Abstract:Measurements and model developments with the objective to improve the quality and resolution of estimations of anthropogenic emissions are described. Measurement results on a chassis dynamometer were used to determine VOC profiles for exhaust gas emissions of passenger cars for different vehicle and fuel types and different driving modes. Further measurements resulted in emission factors and VOC profiles for lignite burning in residential stoves. Using remote sensing techniques benzene emission factors of gas stations and the efficiency of gasoline vapour recovery systems were measured.To improve the quality and the spatial and temporal resolution of emission data, emission models were improved or modified. This was done by elaborating and applying new methods for important emission source categories (e.g., solvent use, road traffic, small combustion) as well as including new data sources in the calculation routines (e.g. emission statements, land use data, import/export indices of solvents). Simultaneously considerable progress was made improving temporal and spatial allocation functions and VOC profiles. With these improvements a large number of anthropogenic emission data sets for 14 different grid projections in Germany and Europe have been generated. An emission scenario for Germany for 2010 suggests that considering air quality directives from the EU and Germany which are in force or in pipeline, German emissions of VOC and NOx will decrease, but still exceed the national emission ceilings of the EU-NEC directive.
Keywords:emission model  emission factor  VOC profile  emission inventories  NOx  NMVOC
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