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Prediction of solid/liquid distribution coefficients of radiocaesium in soils and sediments. Part one: a simplified procedure for the solid phase characterisation
Institution:1. Moscow Lomonosov State University, Soil Science Department, Moscow, Russia, 119991;2. Saskatchewan Research Council, Saskatoon, Canada, S7N 2X8;1. Institut de Radioprotection et de Sûreté Nucléaire (IRSN), Laboratoire de Modélisation pour l’Expertise Environnementale (LM2E), Cadarache, Bâtiment 159, St Paul-lez-Durance, 13115, France;2. Institut de Radioprotection et de Sûreté Nucléaire (IRSN), PRP-HOM, SRBE, Laboratoire d’Epidémiologie (LEPID) Fontenay-aux-Roses, 92262, France;3. Institut de Radioprotection et de Sûreté Nucléaire (IRSN), Laboratoire de Biogéochimie, Biodisponibilité et Transferts des radionucléides (L2BT), Cadarache, Bâtiment 183, St Paul-lez-Durance, 13115, France;1. National Institute of Advanced Industrial Science and Technology, 1-1-1 Higashi, Tsukuba, Ibaraki 305-8567, Japan;2. Center for Research in Isotopes and Environmental Dynamics, University of Tsukuba, 305-8577, Japan;3. Graduate School of Pharmaceutical Sciences (Radioisotope Research Center), Chiba University, 1-33 Yayoichou, Inage-ku, Chiba 263-8522, Japan
Abstract:A comparative study is presented on the quantitative characterisation procedures of soils and sediments in terms of specific radiocaesium sorption potentials obtained during elaborate procedures, which include masking techniques, and a simplified protocol relying on a single KD137Csmeasurement. The elaborate and simple procedures were compared for some 120 soils and sediments of widely different origin, covering some three orders of magnitude in specific sorption capacities. The excellent agreement between both procedures provides the basis for a new and simple characterisation procedure which can be used in routine application.
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