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Radium in the near-surface Caribbean Sea
Authors:David F. Reid  William M. Sackett
Affiliation:Oceanography Division, Code 334, Naval Ocean Research and Development Activity, NSTL Station, MS, 39529, U.S.A.;Department of Oceanography, Texas A & M University, College Station, TX77843, U.S.A.
Abstract:Recent radium measurements from the near-surface Caribbean Sea are presented. The surface horizontal and vertical distributions of226Ra are essentially the same as reported by Szabo et al. (1967) for the early 1960's. The226Ra activity at the surface is relatively uniform across the Caribbean, with an average of8.2±0.4dpm/100kg. The subsurface distribution to ~200 m averages7.8±0.4dpm/100kg and increases slowly below 200 m. reaching ~9.5 dpm/100 kg at 560 m. In contrast to226Ra, the surface concentration of228Ra was much more variable in both time and space. An average increase of 33% was found between 1968 and 1976 in the western Caribbean and during both years an anomalously high228Ra activity was found in the eastern Caribbean. These data support previous hypotheses that water entering the eastern Caribbean has been enriched in228Ra prior to entry and that variable mixing of the Atlantic water masses found to the northeast and southeast of the Lesser Antilles may produce temporal variations in the near-surface228Ra activity. Scatter plots of228Ra vs. salinity and sigma-t indicate that the near-surface vertical distribution of228Ra in the Caribbean Sea is predominantly influenced by advection. Thus228Ra cannot be used to study near-surface vertical mixing rates in this region.
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