Cosmic‐ray exposure history of two Frontier Mountain H‐chondrite showers from spallation and neutron‐capture products

Abstract— We measured the concentrations of ¹⁰Be, ²⁶Al, ³⁶Cl, ⁴¹Ca and ¹⁴C in the metal and/or stone fractions of 27 Antarctic chondrites from Frontier Mountain (FRO), including two large H‐chondrite showers. To estimate the pre‐atmospheric size of the two showers, we determined the contribution of neutron‐capture produced ³⁶Cl (half‐life = 3.01 times 10⁵ years) and ⁴¹Ca (1.04 times 10⁵ years) in the stone fraction. The measured activities of neutron‐capture ³⁶Cl and ⁴¹Ca, as well as spallation produced ¹⁰Be and ²⁶Al, were compared with Monte Carlo‐based model calculations. The largest shower, FRO 90174, includes eight fragments with an average terrestrial age of (100 ± 30) × 10³ years; the neutron‐capture saturation activities extend to 27 dpm/kg stone for ³⁶Cl and 19 dpm/kg stone for ⁴¹Ca. The concentrations of spallation produced ¹⁰Be, ²⁶Al and ³⁶Cl constrain the radius (R) to 80–100 cm, while the neutron‐capture ⁴¹Ca activities indicate that the samples originated from the outer 25 cm. With a pre‐atmospheric radius of 80–100 cm, FRO 90174 is among the largest of the Antarctic stony meteorites. The large pre‐atmospheric size supports our hypothesis that at least 50 of the ～150 classified H5/H6‐chondrites from the Frontier Mountain stranding area belong to this single fall; this hypothesis does not entirely account for the high H/L ratio at Frontier Mountain. The smaller shower, FRO 90001, includes four fragments with an average terrestrial age of (40 ± 10) × 10³ years; they contain small contributions of neutron‐capture ³⁶Cl, but no excess of ⁴¹Ca. FRO 90001 experienced a complex exposure history with high shielding conditions in the first stage (150 < R < 300 cm) and much lower shielding in the second stage (R < 30 cm), the latter starting ～1.0 million years (Ma) ago. Based on the measured ¹⁰Be/²¹Ne and ²⁶Al/²¹Ne ratios, the cosmic‐ray exposure ages of the two showers are 7.2 ± 0.5 Ma for FRO 90174 and 8 ± 1 Ma for FRO 90001. These ages coincide with the well‐established H‐chondrite peak and corroborate the observation that the exposure age distribution of FRO H‐chondrites is similar to that of non‐Antarctic falls. In addition, we found that corrections for neutron‐capture ³⁶Ar (from decay of ³⁶Cl) result in concordant ²¹Ne and ³⁸Ar exposure ages.