Sulfur in the precambrian metallogeny |
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Authors: | Priv-Doz Dr Manfred Schidlowski |
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Institution: | (1) Max-Planck-Institut für Chemie (Otto-Hahn-Institut), 65 Mainz;(2) Present address: Department of Geological Sciences, Harvard University, 02138 Cambridge, Mass. |
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Abstract: | The economically important sulfide deposits of Precambrian age can be subdivided into two principal groups. The first group is represented by Ni- and Cu-bearing differentiates within either layered intrusions of the Sudbury-Bushveld type or within smaller ultramafic bodies (sometimes of greenstone belt association). The relatively narrow spread around the meteorite standard of the 34S values of these deposits suggests a mantle provenance of the sulfide sulfur.The second group (which is quantitatively more important) is represented by stratiform concentrations of base metal sulfides in sedimentary sequences lacking normally any ties to potentially ore-bearing magmas (Copper Belt, Broken Hill, Mount Isa, etc.). Although the problems related to the origin of such strata-bound deposits are rather complex, the majority of the latter probably formed as syngenetic sulfide precipitates in reducing aqueous environments characterized by the presence of bacteriogenic H2S. Sulfur isotope data furnished by some of the principal deposits actually suggest that hydrogen sulfide produced by bacterial sulfate reduction was instrumental in bringing about a precipitation of the metal sulfides, thus underlining the decisive role played by the biosphere in processes of supergene metal concentration.
Zusammenfassung Die wirtschaftlich wichtigen sulfidischen Metallkonzentrationen in präkambrischen Gesteinen lassen sich im wesentlichen zwei Lagerstättengruppen zuordnen. Die erste Gruppe bilden Ni- und Cu-führende sulfidische Differentiate in geschichteten Intrusionen vom Typ Sudbury-Bushveld oder innerhalb kleinerer ultrabasischer Komplexe. Die nur geringe Streubreite der 34S-Werte um den Meteoriten-Standard legt eine abyssische Herkunft des sulfidischen Materials (Magnetkies, Pentlandit, Kupferkies u. a.) derartiger Lagerstätten nahe.Die zweite und quantitativ wichtigere Gruppe bilden schichtige Anreicherungen von Buntmetallsulfiden in Sedimenten, die in der Regel keinerlei Beziehungen zu potentiell erzbringenden Magmatiten erkennen lassen (Copper Belt, Broken Hill, Mount Isa u. a.). Obwohl die beträchtlichen Probleme dieser stratiformen Sulfidlagerstätten eine genetische Deutung schwierig machen (und insbesondere die oft enorme Streubreite der Schwefelisotopen auf eine polygene Herkunft der Sulfide schließen läßt), dürfte es sich bei der Mehrzahl der Vorkommen um primär synsedimentäre Metallausfällungen in einem H2S-führenden reduzierenden Milieu handeln, wobei spätere tektonischmetamorphe Stoffmobilisierungen möglicherweise eine weitere Konzentration der Lagerstättensubstanz bewirkt haben. Die starke Beteiligung von bakteriogenem Schwefelwasserstoff bei der Ausfällung der Sulfide wird durch die Schwefelisotopen-Verteilung in verschiedenen derartigen Lagerstätten gestützt. Dieser Befund unterstreicht gleichzeitig die entscheidende Rolle der Biosphäre bei der Bildung von Metallanreicherungen im exogenen Zyklus.
Résumé Les concentrations de sulfures métalliques économiquement importantes dans les terrains précambriens peuvent essentiellement être subdivisées en deux groupes de gisements. Le premier groupe comprend les différenciats de sulfures nickelifères et cuprifères dans les intrusions litées du type Sudbury-Bushveld ou dans l'intérieur de complexes ultrabasiques plus petits. La faible distribution des valeurs du soufre 34 des météorites standard suggère une provenance abyssale des matériaux sulfurés de ces gisements (pyrrhotine, pentlandite, sulfures de Cu, etc.). Le deuxième groupe quantitativement plus important comprend les enrichissements «stratiformes »de sulfures métalliques dans les sédiments qui, en règle générale, ne montrent aucune liaison avec des magmatites potentiellement minéralisantes (Copper Belt, Broken Hill, Mount Isa, etc.). Quoique les problèmes importants relatifs à ces gisements sulfurés stratiformes rendent difficile une interprétation génétique (et en particulier la dispersion souvent énorme des isotopes du soufre qui permet de conclure à une provenance polygène des sulfures), il doit s'agir dans la plupart des cas de précipitations de métaux synsédimentaires primaires dans un milieu réducteur contenant H2S; à la suite de quoi une mobilisation ultérieure tectonico-métamorphique pourrait avoir exercé une nouvelle concentration de la matière du gisement. La forte participation d'H2S bactériogène au cours de la précipitation des sulfures est confirmée par la distribution des isotopes du soufre dans différents de ces gisements. Ce fait souligne simultanément le rôle décisif de la biosphère au cours de la formation des enrichissements métalliques dans le cycle exogène.
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