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Chemistry of Aerosols over Chukchi Sea and Bering Sea
作者姓名:朱赖民  陈立奇  杨绪林  杜俊民  张远辉
作者单位:TheThirdInstituteofOceanography,KeyLaboratoryofGlobalChangeandMarine-AtmosphericChemistry,SOA,Xiamen361005,China
基金项目:国家自然科学基金,First Arctic Research Expedition Program,State Ocean Adminis-tration
摘    要:The contents of elements in aerosols sampled during the First Chinese Arctic Research Expedition (CHINARE-1) show great differences from one element to another. Na, K,Ca, Mg, A1, F, and Cl are the major components in the aerosols, whose contents are larger than 30 ng/m^3. The chemical elements whose contents vary between 0.1 - 30 ng/m^3 are Br,Sr, Cr, Ni, and Zn. The chemical elements whose contents are close to or slightly higher than 0.1 ng/m^3 are Rb, Ba, Zr, Th, and Pb. The contents of As, Sb, W, Mo, Au, La, Ce, Nd,Sin, Eu, Tb, Yb, Lu, Sc, Co, Hf, Ta, and Cd are less than 0.1 ng/m^3. The mass concentration data for the same element, as observed during CHINARE-1, are almost accordant, but much lower than what is observed in the China‘ s seas or the coasts of China. The enrichment factor and electron microscopic analyses and lead isotope tracing were used to distinguish their sources.Four groups of sources can be classified as follows: anthropogenic: As, Sb, W, F, Mo, Au,Cu, Pb, Cd, V; crustal: La, Ce, Nd, Sm, Eu, Tb, Yb, Lu, Fe, Sc, Cr, Co, Ba, Zr, Hf,Ta, Cs, Mn, Th, U; oceanic:Na, K, Ca, and Mg; and mixing: Rb, Sr, Ca, and Mg.

关 键 词:气溶胶  化学元素  化合作用  楚克其海

Chemistry of aerosols over Chukchi Sea and Bering Sea
Zhu?Laimin,Chen?Liqi,Yang?Xuling,Du?Junmin,Zhang?Yuanhui.Chemistry of Aerosols over Chukchi Sea and Bering Sea[J].Chinese Journal of Geochemistry,2004,23(1):26-36.
Authors:Zhu Laimin  Chen Liqi  Yang Xuling  Du Junmin  Zhang Yuanhui
Institution:(1) The Third Institute of Oceanography, Key Laboratory of Global Change and Marine-Atmospheric Chemistry, SOA, 361005 Xiamen, China
Abstract:The contents of elements in aerosols sampled during the First Chinese Arctic Research Expedition (CHINARE-1) show great differences from one element to another. Na, K,Ca, Mg, Al, F, and Cl are the major components in the aerosols, whose contents are larger than 30 ng/m3. The chemical elements whose contents vary between 0.1-30 ng/m3 are Br,Sr, Cr, Ni, and Zn. The chemical elements whose contents are close to or slightly higher than 0. 1 ng/m3 are Rb, Ba, Zr, Th, and Pb. The contents of As, Sb, W, Mo, Au, La, Ce, Nd,Sm, Eu, Tb, Yb, Lu, Sc, Co, Hf, Ta, and Cd are less than 0.1 ng/m3. The mass concentration data for the same element, as observed during CHINARE-1, are almost accordant, but much lower than what is observed in the China' s seas or the coasts of China. The enrichment factor and electron microscopic analyses and lead isotope tracing were used to distinguish their sources.Four groups of sources can be classified as follows: anthropogenic: As, Sb, W, F, Mo, Au,Cu, Pb, Cd, V; crustal: La, Ce, Nd, Sm, Eu, Tb, Yb, Lu, Fe, Sc, Cr, Co, Ba, Zr, Hf,Ta, Cs, Mn, Th, U; oceanic:Na, K, Ca, and Mg; and mixing: Rb, Sr, Ca, and Mg.
Keywords:marine aerosol  global change  Arctic  CHINARE-1
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