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Distribution of222Rn over the north Pacific: Implications for continental influences
Authors:Yves J Balkanski  Daniel J Jacob  Richard Arimoto  Mark A Kritz
Institution:(1) Dept. of Earth & Planetary Sciences, Harvard University, Pierce Hall, 29 Oxford St., 02138 Cambridge, Massachusetts, U.S.A.;(2) Division of Applied Sciences, Harvard University, Pierce Hall, 29 Oxford St., 02138 Cambridge, Massachusetts, U.S.A.;(3) Graduate School of Oceanography, University of Rhode Island, 02882 Narragansett, RI, U.S.A.;(4) Atmospheric Sciences Research Center, State University of New York, 12222 Albany, NY, U.S.A.
Abstract:The atmospheric distribution of222Rn over the north Pacific is simulated with a three-dimensional chemical tracer model using meteorological input from the NASA-GISS general circulation model (4°×5° resolution). Radon-222 (half-life 3.8 days) is a tracer of continental air. Model results are in good agreement with measurements from ships and aircraft. Strong Asian influence is found throughout the tropospheric column over the north Pacific in spring, reflecting a combination of frequent convection over the continent, strong westerly winds at altitude, and subsidence over the ocean. In summer, the upper troposphere over the north Pacific is heavily affected by deep convection over China; however, Asian influences at the surface are then at their yearly minimum. In winter, strong Asian influence is found near the surface but not at high altitudes. Transport of American air over the Pacific is important only at low latitudes. American sources account for 11% of total222Rn in the model at Midway, 30% at Mauna Loa and 59% at Oahu. Results for Hawaii indicate two seasonal peaks of American influence, one in summer and one in winter. The tropical western Pacific is particularly remote from continental influences year round.
Keywords:North Pacific  global atmospheric chemistry  modeling  radon
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