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中国湖泊柱样沉积物中239+240Pu的来源与分布特征
引用本文:黄亚楠,潘少明,刘志勇. 中国湖泊柱样沉积物中239+240Pu的来源与分布特征[J]. 地理科学, 2018, 38(3): 437-447. DOI: 10.13249/j.cnki.sgs.2018.03.014
作者姓名:黄亚楠  潘少明  刘志勇
作者单位:1.南京大学海岸与海岛开发教育部重点实验室,江苏 南京 210023
2.苏州大学放射医学与防护学院,江苏 苏州 215123
基金项目:国家重点研发计划项目(2016YFA0600502)、国家自然科学基金项目(41671466)资助
摘    要:针对当前中国湖泊柱样沉积物中239+240Pu的研究现状,对中国湖泊239+240Pu的来源、239+240Pu最大蓄积峰的年代以及239+240Pu在湖泊沉积物中的迁移行为进行了研究总结。结果表明:中国湖泊239+240Pu的主要来源于全球大气核试验沉降,湖泊沉积柱样中表层沉积物240Pu/239Pu均值为0.177±0.019;柱样240Pu/239Pu均值为0.177±0.008;柱样239+240Pu的沉积通量范围在7.45~240.6 MBq/km2之间,因湖泊所处沉积环境及纬度的差异而变化。湖泊柱样剖面中的239+240Pu的分布多呈单峰分布,湖泊沉积物中239+240Pu的最大蓄积峰位置改变可以忽略不计,239+240Pu最大蓄积峰具有时标价值。

关 键 词:湖泊  柱样沉积物  239+240Pu  240Pu/239Pu  沉积通量  
收稿时间:2017-07-09
修稿时间:2017-10-08

The Source and Distribution Characteristic of 239+240Pu in Sediment Cores of Chinese Lakes
Yanan Huang,Shaoming Pan,Zhiyong Liu. The Source and Distribution Characteristic of 239+240Pu in Sediment Cores of Chinese Lakes[J]. Scientia Geographica Sinica, 2018, 38(3): 437-447. DOI: 10.13249/j.cnki.sgs.2018.03.014
Authors:Yanan Huang  Shaoming Pan  Zhiyong Liu
Affiliation:1.The Key Laboratory of Ministry Education of Coastal and Island Development, Nanjing University, Nanjing 210023, Jiangsu, China
2. School for Radiological and Interdisciplinary Sciences, Soochow University, Suzhou 215123, Jiangsu, China
Abstract:China is a nation with numerous lakes; tracer studies of 239+240Pu have been carried out in 14 lakes. According to the research status of 239+240Pu in Chinese lakes, this article summarizes the source, the migration behavior of 239+240Pu and the age of the maximum accumulation peaks of 239+240Pu. The results show that 239+240Pu in lacustrine sediment cores of Chinese lakes are mainly derived from the global atmospheric nuclear tests, the mean value of 240Pu/239Pu was 0.177±0.019 in the surface sediments, the mean value 240Pu/239Pu was 0.177±0.008 in the all sediment cores. Because of the difference of lake sedimentary environment and latitude changes, the range of the 239+240Pu inventories of was 7.45-240.6 MBq/km2. The distribution characteristic of 239+240Pu in lacustrine sediment cores of Chinese lakes are mostly unimodal, and the migration of 239+240Pu in sediment cores can be neglected and the maximum accumulation peak of 239+240Pu has time scale value.
Keywords:lake  sediment cores  239+240Pu activity   240Pu/239Pu  239+240Pu inventory  
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