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A New Index Developed for Fast Diagnosis of Meteorological Roles in Ground-Level Ozone Variations
Authors:Weihua CHEN  Weiwen WANG  Shiguo JIA  Jingying MAO  Fenghua YAN  Lianming ZHENG  Yongkang WU  Xingteng ZHANG  Yutong DONG  Lingbin KONG  Buqing ZHONG  Ming CHANG  Min SHAO  Xuemei WANG
Abstract:China experienced worsening ground-level ozone (O3) pollution from 2013 to 2019. In this study, meteorological parameters, including surface temperature (T2), solar radiation (SW), and wind speed (WS), were classified into two aspects, (1) Photochemical Reaction Condition (PRC = T2 × SW) and (2) Physical Dispersion Capacity (PDC = WS). In this way, a Meteorology Synthetic Index (MSI = PRC/PDC) was developed for the quantification of meteorology-induced ground-level O3 pollution. The positive linear relationship between the 90th percentile of MDA8 (maximum daily 8-h average) O3 concentration and MSI determined that the contribution of meteorological changes to ground-level O-3 varied on a latitudinal gradient, decreasing from ~40% in southern China to 10%–20% in northern China. Favorable photochemical reaction conditions were more important for ground-level O3 pollution. This study proposes a universally applicable index for fast diagnosis of meteorological roles in ground-level O3 variability, which enables the assessment of the observed effects of precursor emissions reductions that can be used for designing future control policies.
Keywords:ground-level ozone  meteorology synthetic index  photochemical reaction condition  physical dispersion capacity
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