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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
对青藏东北缘现今块体划分、运动及变形的初步研究 总被引:19,自引:9,他引:10
利用2维非连续变形分析方法(DDA),以位移代替围压作为边界约束力,研究青藏东北缘现今块体划分及其运动变形。根据该地区地质构造及地震活动,以GPS点测量位移作为模拟结果约束点,得出了较合理的块体划分模型和随时间演化的主应变分布图,并把应变高值区与近几年来发生的5级以上地震作对比,得出了研究区内地震危险性可能较大的区域。另外,对模拟的甘青块体与阿拉善块体的边缘带断裂左旋运动做了大概计算。 相似文献
3.
C. Beaugé 《Celestial Mechanics and Dynamical Astronomy》1996,64(4):313-350
Starting with a simple Taylor-based expansion of the inverse of the distance between two bodies, we are able to obtain a series expansion of the disturbing function of the three-body problem (planar elliptic case) which is valid for all points of the phase space outside the immediate vicinity of the collision points. In particular, the expansion is valid for very high values of the eccentricity of the perturbed body. Furthermore, in the case of an interior mean-motion resonant configuration, the above-mentioned expression is easily averaged with respect to the synodic period, yielding once again a global expansion of (R) valid for very high eccentricities.Comparisons between these results and the numerically computed exact function are presented for various resonances and values of the eccentricity. Maximum errors are determined in each case and their origin is established. Lastly, we discuss the applicability of the present expansion to practical problems. 相似文献
4.
A recently developed near infrared high speed photometer intended for lunar oc-cultation studies is described. The primary scientific objective is to reach milli arc second levels of angular resolution so that circumstellar structure of the occulted sources can be resolved. Near infrared sky brightness close to the lunar limb is also studied. Angular diameter derived from the observed occultation of IRC +20169 is presented and system performance discussed. 相似文献
5.
We have analysed short-exposure high-resolution images obtained on the William Herschel Telescope (WHT), Big Telescope Azimuthal (BTA) and CanadaFranceHawaii Telescope (CFHT) in order to investigate mechanical vibrations that are capable of reducing the high angular resolution allowed by speckle-interferometric methods. After filtering the photon noise we have computed power spectra of the image centres of gravity. In these spectra we have found vibration features that differ from one telescope to another and that vary in particular with the zenith angle. In the case of the WHT we discuss these results in terms of possible causes and in terms of degradation of the transfer function. We present some means to improve the data. 相似文献
6.
基于可靠度理论的黄土高边坡优化设计 总被引:11,自引:2,他引:9
对黄土高边坡进行可靠性分析,应用数学原理和优化原理,建立了黄土高边坡的优化模型,对铜黄一级公路黄土高边坡进行分析验证。结果表明,该方法计算的结果与实际较接近.应用中易操作。 相似文献
7.
A coupled deterministic hydrological and water temperature model, CEQUEAU, was modified to include soil temperature and crown closure in its calculation of local advective terms in the heat budget. The modified model was than tested to verify its sensitivity to these modifications. An analysis of the heat budget of a small forested catchment in eastern Canada revealed that the advective term related to interflow plays a significant role in the daily water heat budget, providing on average 28% of the local advective budget (which also includes advective heat terms from surface runoff and groundwater) and nearly 14% of the total heat budget (which includes all radiative terms at the water surface, convection and evaporation, as well as the local advective terms). Relative sensitivity indices (RSIs) were used to verify the impact of the newly introduced parameters and variables. Among them, parameters related to the forest cover (crown closure and leaf area index) have a maximum RSI of ?0·6; i.e. a 100% increase in value produces a 60% decrease in the local advective term. Parameters with the greatest influence are the volume of water contributing to interflow and the amplitude of the net radiative flux at the soil surface, which, if doubled, would double the contribution of the local interflow advective term to the heat budget. Copyright © 2003 John Wiley & Sons, Ltd. 相似文献
8.
1IntroductionOne of the key factors related to basin geody-namics is deep process controlling formation and evolution of sedimentary basin. Depth and tempera-ture of asthenosphere,existence of mantle plume,occurrence of mantle melting,and amounts of melts under depressurization during thinning of lithosphere are controlling factors influenced formation and characteristics of extensional basin directly (Li,1994). Rifting is probably governed by frictional forces exerted on the base of litho… 相似文献
9.
鱼卡煤田大煤沟组高分辨率层序地层特征及聚煤规律 总被引:1,自引:0,他引:1
利用高分辨率层序地层学理论和技术方法,综合地震、测井、岩芯和煤质资料对柴达木盆地北缘鱼卡煤田中下侏罗统大煤沟组地层河湖三角洲沉积体系进行高分辨率层序地层学分析,从中识别出短期、中期、长期3个级别的基准面旋回层序,划分出向上"变深"非对称型、向上"变浅"非对称型及对称型3种短期基准面旋回基本结构类型。依据等时地层对比法则进行不同级次基准面旋回层序的联井对比,建立了大煤沟组的等时地层格架,在等时地层格架内进行了煤层对比,并在等时地层格架内分析了聚煤规律。 相似文献
10.
碱消解-高效液相色谱-电感耦合等离子体质谱法测定生物样品中的甲基汞和乙基汞 总被引:7,自引:2,他引:5
建立了碱消解-高效液相色谱-电感耦合等离子体质谱联用系统测定生物样品中甲基汞(MeHg)与乙基汞(EtHg)的分析方法。为提高灵敏度,选用微流量的PFA雾化器,在优化的检测条件下,MeHg及EtHg检出限可达到0.036μg/L和0.03μg/L;线性范围达到4个数量级,两条工作曲线线性相关系数为1。对1.78μg/L MeHg、1.65μg/L EtHg的混合标准溶液重复测定7次,色谱峰面积的相对标准偏差(RSD)分别为1.79%和1.44%。对标准物质BCR 464(金枪鱼)的分析结果表明,测定值与标准值基本吻合,但略低于标准值;甲基汞和乙基汞的加标回收率分别为85.9%和84.5%。高效液相色谱与质谱联用技术的高灵敏度和低检出限能够满足生物样品中汞形态定量分析的要求。 相似文献