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1.
Titan's haze consists of long chain polymers of pure and N-mixed hydrocarbons (Coustenis et al., 1989, Icarus 80, 54-76, 1991, Icarus 89, 152-167). These polymers have regularly alternating (i.e., conjugated) double/single and triple/single bonds, which open either spontaneously (free aging) or under the action of some external factors (forced aging), the latter being very diverse, e.g., charging, photolysis, radiolysis, thermolysis, chemical effect of environment, etc. An essential of free aging was examined previously (Dimitrov and Bar-Nun, 2002, Icarus 156, 530-538). The main distinction between free and any forced aging is that both of them possess the same thermodynamics while different kinetics, the forced aging in any case being faster, proceeding in different pathways than the free aging. The more extensive is the list of the external effects and the more intensive they are, the faster and more variably the forced aging proceeds. In this paper we quantified the kinetics of forced aging, considering charging of Titan's aerosol population. It was found that forced aging proceeds approximately hundred times faster as compared to the free aging. Various physico-chemical properties of Titan's aerosol material, including coagulation coefficients, depending on particle size and medium conditions, were defined. The comparison of the aging rate, rate of sedimentation and rate of the particle increase proves that Titan's aerosol domain can be subdivided conditionally into two big subdomains. The upper one contains minor portion (<5%) of the total aerosol bulk, unannealed aerosol particles being fine and sticky. The lower subdomain contains the major portion (>95%) of aerosol bulk, which is completely aged, coarsely dispersed particles. We established the border between these subdomains at the altitude Z∼620 km. 相似文献
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Evolution of sedimentary systems at large temporal and spatial scales cannot be scaled down to laboratory dimensions by conventional hydraulic Froude scaling. Therefore, many researchers question the validity of experiments aiming to simulate this evolution. Yet, it has been shown that laboratory experiments yield stratigraphic responses to allocyclic forcing that are remarkably similar to those in real‐world prototypes, hinting at scale independency with strong dependence on boundary conditions but weak dependence on the actual sediment transport dynamics. This paper addresses the dilemma by contrasting sediment transport rules that apply in the laboratory with those that apply in real‐world geological systems. It is demonstrated that the generation of two‐dimensional stratigraphy in a flume can be simulated numerically by the non‐linear diffusion equation. Sediment transport theory is used to demonstrate that only suspension‐dominated meandering rivers should be simulated with linear diffusion. With increasing grain‐size (coarse sand to gravel) and shallowness of river systems, the prediction of long‐term transport must be simulated by non‐linear, slope‐dependent diffusion to allow for increasing transport rates and thus change in stratigraphic style. To point out these differences in stratigraphic style, three stages in infill of accommodation have been defined here: (i) a start‐up stage, when the system is prograding to base level (e.g. the shelf edge) with no sediment flux beyond the base‐level point; (ii) a fill‐up stage, when the system is further aggrading while progressively more sediment is bypassing base level with the progression of the infill; and (iii) a keep‐up stage, when more than 90% of the input is bypassing the base level and less than 10% is used for filling the accommodation. By plotting the rate of change in flux for various degrees of non‐linearity (varying the exponent in the diffusion equation) it was found that the error between model and real‐world prototype is largest for the suspension‐dominated prototypes, although never more than 30% and only at the beginning of the fill‐up stage. The error reduces to only 10% for the non‐linear sandy‐gravelly and gravelly systems. These results are very encouraging and open up ways to calibrate numerical models of sedimentary system evolution by such experiments. 相似文献
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Rajasekhar Balasubramanian Chanbasha Basheer Kang Lisa Siao Wei See 《中国地球化学学报》2006,25(B08):183-183
Microorganic pollutants such as polycylic aromatic hydrocarbons (PAHs), organochlorine pesticides (OCPs), polychlorinated biphenyls (PCBs) and total petroleum hydrocarbons (TPHs) are known to be present in urban ambient air. These organic compounds are prone to atmospheric transport and deposition over long distances, thus enabling them to accumulate even in regions remote from their sources. Deposition from the atmosphere can be via direct deposition and exchange with crops that may be directly or indirectly ingested by humans. It can also take place via wet and dry deposition and air-water exchange. Following their deposition, these microorganic pollutants tend to accumulate in soils, sediments and in human and ecological food chains. There are many reports in the literature on the atmospheric concentrations of microorganic pollutants, but there are few reports and data in Asia. This study was performed in Singapore to determine the relative amounts of persistent organic pollutants and TPHs in ambient aerosols. One of the important sources of these organic compounds in Southeast Asia is thought to be biomass burning (vegetation fires). Hence, air sampling was conducted during both smoke haze and non-haze periods. The data obtained from this study will be presented and discussed. 相似文献
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提出一个对多元判据综合评估的中期天气客观相似预报模式。模式应用同中期天气过程的时间—空间尺度相适应的经过时间滤波的大气环流背景为客观判据,比较全面地评估了预报时刻前后多层次、多要素的大气环流动态变化的相似,通过定义相似指数综合评估在多元判据下样本的相似程度,从相似时域的历史样本中找到较佳相似的中期过程,预测未来l~10天的中期天气过程。模式检验和预报试验表明该模式具有预报技巧。 相似文献
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最优气候相似法及其在降水预报中的应用 总被引:2,自引:0,他引:2
介绍了一种短期气候预测方法———最优气候相似法 ,并应用于张家界地区 1 999~ 2 0 0 2年 5~ 7月总降水预报中 ,结果显示最优气候相似法能够有效地提高短期气候的预测能力 ,特别对气候异常具有良好的反应能力 ,适合于短期气候业务预报。 相似文献
10.
Experiments were carried out on granular flows generated by instantaneous release of gas-fluidised, bidisperse mixtures and propagating into a horizontal channel. The mixture consists of fine (< 100 μm) and coarse (> 100 μm) particles of same density, with corresponding grain size ratios of ∼ 2 to 9. Initial fluidisation of the mixture destroys the interparticle frictional contacts, and the flow behaviour then depends on the initial bed packing and on the timescale required to re-establish strong frictional contacts. At a fines mass fraction (α) below that of optimal packing (∼ 40%), the initial mixtures consist of a continuous network of coarse particles with fines in interstitial voids. Strong frictional contacts between the coarse particles are probably rapidly re-established and the flows steadily decelerate. Some internal friction reduction appears to occur as α and the grain size ratio increases, possibly due to particle rolling and the lower roughness of internal shear surfaces. Segregation only occurs at large grain size ratio due to dynamical sieving with fines concentrated at the flow base. In contrast, at α above that for optimal packing, the initial mixtures consist of coarse particles embedded in a matrix of fines. Flow velocities and run-outs are similar to that of the monodisperse fine end-member, thus showing that the coarse particles are transported passively within the matrix whatever their amount and grain size are. These flows propagate at constant height and velocity as inviscid fluid gravity currents, thus suggesting negligible interparticle friction. We have determined a Froude number of 2.61 ± 0.08 consistent with the dam-break model for fluid flows, and with no significant variation as a function of α, the grain size ratio, and the initial bed expansion. Very little segregation occurs, which suggests low intensity particle interactions during flow propagation and that active fluidisation is not taking place. Strong frictional contacts are only re-established in the final stages of emplacement and stop the flow motion. We infer that fines-rich (i.e. matrix-supported) pyroclastic flows propagate as inviscid fluid gravity currents for most of their emplacement, and this is consistent with some field data. 相似文献