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1.
Experiments were conducted in the field to determine the non-chemical loss rate of methyl iodide in seawater and to examine production rates of methyl halides. The loss rate of added C13 labelled methyl iodide, present at concentrations similar to those found in seawater, corrected for chemical loss due to reaction with Cl− varied from < 1 to 18% day− 1, with a mean value of 7%. This rate of loss is much lower than that which was proposed by Bell et al. [Bell, N., Hsu, L., Jacob, D. J., Schultz, M. G., Blake, D. R., Butler, J. H., King, D. B., Lobert, J. M., Maier-Reimer, E., 2002. Methyl iodide: Atmospheric budget and use as a tracer of marine convection in global models, Journal of Geophysical Research-Atmospheres 107(D17), 4340-4351.] to account for the large discrepancies between observed and predicted mid-latitude concentrations of CH3I based on their global photochemical source model. The suitability of several types of container for seawater incubations was studied and only quartz tubes appeared to be free of experimental artifact. Collapsible polyvinyl fluoride containers showed major production of methyl halides on irradiation with simulated sunlight. Polyethylene containers caused spurious production of methyl iodide at lower rates. 相似文献
2.
The Eastern Flank Hydrocarbon Province borders the southeastern edge of the South Oman Salt Basin in the southern part of Oman. An intensive exploration programme by PDO over the past seven years has led to the discovery of almost 2 × 109 m3 of oil with current production of some 15000 m3/d from six fields.In stark contrast to other oil habitats of the Arabian Peninsula, the main play involves rock units and geological events ranging in age from Late Precambrian to Quaternary Times, while trap development and charging are closely related to syn-tectonic salt dissolution.The principal reservoirs and seals are poorly consolidated, Palaeozoic clastics which drape, due to salt dissolution, over residual ‘cores’ principally composed of either Lower Palaeozoic sandstones (Haima Group), or Late Proterozoic carbonates (Huqf Group), or some combination of these. Oils have been geochemically correlated with algal source rocks of the Huqf Eastern Flank. Structures are considered to have been ‘charged’ from Late Mesozoic times onwards in conjunction with progressive subsurface salt removal and the onset of maturation of local source rocks. The effectiveness of ‘charging’ along the retreating salt edge is indicated by the small percentage of dry wells.Major oil zones are found in both anticlinal and truncation traps which are commonly developed around sandstone (Haima Group) cores. Oils show a wide range of characteristics but are typically heavy, early expulsion crudes, high sulphur with little associated gas. Bacterial transformation is not uncommon.Producing reservoirs mainly occur at relatively shallow depths (600–1200 m). Primary recovery factors of around 7% reflect the high density and viscosity of the Eastern Flank crudes and have initiated interest in Enhanced Oil Recovery (EOR) techniques. Two such pilot projects, involving steam and polymer flooding, are due to commence in 1984 and, if successful, will substantially increase the reserve base of these fields. 相似文献
3.
Deep sea drilling in the Central Gulf of California, a young and active spreading centre, shows that the high heat flow typical of these regions causes extensive alteration of sediment organic matter, especially near sills and above magma chambers where hydrothermal activity is concentrated. Even on the nearby passive margin, where there are no sills, heat flow is moderately high and hydrocarbon generation has begun in immature sequences. Migrating light hydrocarbons are detected especially where hydrothermal activity is concentrated. Thermogenic methane is more widespread, though not in the passive margin bordering the spreading centre. Despite the incidence of hydrocarbon generation and migration, the amounts of hydrocarbons involved are relatively small and apparently do not lead to commercially significant accumulations of petroleum.The organic matter in these sediments is mostly marine because the Gulf of California generally has low runoff from land and highly productive surface waters. Turbidites rich in terrigenous organic material are locally abundant in the mainly pelagic section in the Guaymas Basin. The highest concentrations of organic matter are found in laminated diatomites deposited on the Guaymas passive margin within the oxygen minimum zone. 相似文献
4.
Based on the determination of composition of volcanic volatiles and petrologic estimation of the total mass of volatiles erupted,
we showed important advances in the study of the impact of Mesozoic and Cenozoic volcanic activities on paleo-environmental
changes in China. The volcanic activities include western Liaoning and Zhangjiakou Mesozoic intermediate-acidic explosive
eruptions, southern Tibet and Shanwang Cenozoic volcanism, and Mt. Changbai volcanic eruption around one thousand years ago.
The paper predominantly discusses the earth’s surface temperature changes, ozone depletion, acidic rain formation and mass
mortalities of vertebrate induced by the Mesozoic and Cenozoic volcanism in China.
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Translated from Bulletin of Mineralogy, Petrology and Geochemistry, 2007, 26(4): 319–322 [译自: 矿物岩石地球化学通报] 相似文献
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6.
Bruce A. Callander 《GeoJournal》1997,42(1):55-63
IPCCs statement in its 1995 report (IPCC 1996) that a human influence was discernible in global climate has been widely quoted but often misunderstood. The character of the evidence underpinning this detection statement is explained so that its strengths and weaknesses can be better understood and the subtleties of its message better appreciated. To demonstrate the close linkage between the government-approved summary and the underlying chapters of the IPCC report the detailed evolution of the detection statement from first draft through to the form finally approved by the IPCC is described. 相似文献
7.
As a legacy of the centrally planned economy, the economies in transition of Central and Eastern Europe (CEE) have a unique
potential to reduce their greenhouse gas emissions through the improvement in their high energy intensities. Since much of
this `low-hanging fruit' in energy-efficiency improvements can be highly cost-effective, many developed countries facing difficulties
in meeting their greenhouse gas (GHG) emission targets domestically are eager to find such opportunities in the CEE region.
Therefore, studies analysing the potentials and costs of carbon dioxide reduction through technology improvement in the region
have come into the limelight. While there are a few excellent studies in the region aimed at analysing climate change abatement
potentials, they all embark on different assumptions, methodologies and boundary conditions. It is hence difficult, if not
impossible, to compare and analyse the results of these studies across different authors, countries or time horizons. Consequently,
the purpose of this paper is to place four leading studies on GHG mitigation through technology improvement from the CEE region
into an internationally comparable framework. Four studies were selected from three countries, Poland, Hungary and Estonia,
which are all the results of major national and international efforts to assess costs and potentials of GHG reduction. The
paper places their assumptions, methods and final results into a framework which enables policy-makers and project designers
to compare these across geographical and technological boundaries. Since other studies from around the globe have been analysed
in this framework in the literature, this paper provides a vehicle for the findings of these four studies to be compared to
others worldwide. In addition, the paper highlights a few areas where similar studies to be completed in the future in the
region may be enhanced by incorporating features used in GHG mitigation research in other parts of the world.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
8.
9.
S. E. Beaubien G. Ciotoli S. Lombardi 《Journal of Volcanology and Geothermal Research》2003,123(1-2):63
The sudden and catastrophic, or slow and continuous, release at surface of naturally occurring toxic gases like CO2, H2S and Rn poses a serious health risk to people living in geologically active regions. In general this problem receives little attention from local governments, although public concern is raised periodically when anomalous toxic-gas concentrations suddenly kill humans or livestock. For example, elevated CO2 concentrations have been linked to the death of at least 10 people in the central Italian region of Lazio over the last 20 years, while it was the CO2 asphyxiation of 30 cows in a heavily populated area near Rome in 1999 which prompted the present soil-gas study into the distribution of the local health risk. A detailed geochemical survey was carried out in an area of about 4 km2 in the Ciampino and Marino districts, whereby a total of 274 soil-gas samples were collected and analysed for more than 10 major and trace gas species. Data were then processed using both statistical and geostatistical methods, and the resulting maps were examined in order to highlight areas of elevated risk. General trends of elevated CO2 and Rn concentrations imply the presence of preferential pathways (i.e. faults and fractures) along which deep gases are able to migrate towards the surface. The CO2 and Rn anomalous trends often correspond to and are usually elongated parallel to the Apennine mountain range, the controlling structural feature in central Italy. Because of this fundamental anisotropy in the factors controlling the soil-gas distribution, it was found that a geostatistical approach using variogram analysis allowed for a better interpretation of the data. With regard to the health risk to local inhabitants, it was found that although some high risk areas had been zoned as parkland, others had been heavily developed for residential purposes. For example, many new houses were found to have been built on ground which has soil-gas CO2 concentrations of more than 70% and radon values of more than 250 kBq m−3. It is recommended that land-use planners incorporate soil-gas and/or gas flux measurements in environmental assessments in areas of possible risk (i.e. volcanic or structurally active areas). 相似文献
10.