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W. Thomas T. Ruppert M. Van Roozendael J. Verdebout D. Balis C. Meleti C. Zerefos 《Journal of Atmospheric Chemistry》2005,50(3):295-320
We focus on the retrieval of volcanic sulfur dioxide (SO2) emissions from an analysis of atmospheric UV backscatter spectra obtained by the Global Ozone Monitoring Experiment (GOME) spectrometer on board the ESA European Remote Sensing Satellite (ERS-2). Here, the last major eruptions of Mt. Etna on Sicily (Italy) in July/August 2001 and October/November 2002 provided an excellent opportunity to study the retrieval of SO2 columnar amounts from ground-based, LIDAR and satellite measurements. Our study shows that the bulk of emitted SO2 was confined in the troposphere, mainly between 700 hPa and 400 hPa which is confirmed by trajectory analysis, by LIDAR observations and AVHRR observations. The area of influence of Mt. Etna eruptions ranges from the Western Saharan Desert to Greece and the near east states and even down to the basin of Tschad, Africa. Our analysis revealed that information about the plume height of volcanic eruptions and aerosol parameters is necessary for a reliable quantitative retrieval of SO2 from space-borne sensor data at periods perturbed by volcanic eruptions. 相似文献
2.
Marcel Dobber Robert Voors Ruud Dirksen Quintus Kleipool Pieternel Levelt 《Solar physics》2008,249(2):281-291
We have constructed a new high resolution solar reference spectrum in the spectral range between 250 and 550 nm. The primary
use of this spectrum is for the calibration of the Dutch – Finnish Ozone Monitoring Instrument (OMI), but other applications
are mentioned. The incentive for deriving a new high resolution solar reference spectrum is that available spectra do not
meet our requirements on radiometric accuracy or spectral resolution. In this paper we explain the steps involved in constructing
the new spectrum, based on available low and high resolution spectra and discuss the main sources of uncertainty. We compare
the result with solar measurements obtained with the OMI as well as with other UV-VIS space-borne spectrometers with a similar
spectral resolution. We obtain excellent agreement with the OMI measurements, which indicates that both the newly derived
solar reference spectrum and our characterization of the OMI instrument are well understood. We also find good agreement with
previously published low resolution spectra. The absolute intensity scale, wavelength calibration and representation of the
strength of the Fraunhofer lines have been investigated and optimized to obtain the resulting high resolution solar reference
spectrum. 相似文献
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We present comparisons of the NO2 regional Chemical Transport Model (CTM) simulations over North-eastern North America during the time period from May to September, 1998 with hourly surface NO2 observations and the NO2 columns retrieved from the GOME (Global Ozone Monitoring Experiment) satellite instrument. The model calculations were performed using the Mesoscale Meteorological Model 5 (MM5), Sparse Matrix Operator Kernal Emissions (SMOKE), and Community Multiscale Air Quality (CMAQ) modeling systems, using the emission data from the National Emissions Inventory (NEI) databases of 1996 (U.S.) and 1995 (Canada). The major objectives were to assess the performance of the CMAQ model and the accuracy of the emissions inventories as they affected the simulations of this important short-lived atmospheric species. The modeled (NcMAQ) and measured (NGOME) NO2 column amounts, as well as their temporal variations, agreed reasonably well. The absolute differences (NcMAQ-NGOME) across the domain were between ±3.0×10^15 molecules cm^-2, but they were less than ±1.0×10^15 molecules cm^-2 over the majority (80%) of the domain studied. The overall correlation coefficient between the measurements and the simulations was 0.75. The differences were mainly ascribed to a combination of inaccurate emission data for the CTM and the uncertainties in the GOME retrievals. Of these, the former were the more easily identifiable. 相似文献
4.
X. Tie S. Chandra J. R. Ziemke C. Granier G. P. Brasseur 《Journal of Atmospheric Chemistry》2007,56(2):105-125
Satellite measurements of tropospheric column O3 and NO2 in eastern and southeastern Asia are analyzed to study the spatial and seasonal characteristics of pollution in these regions.
Tropospheric column O3 is derived from differential measurements of total column ozone from Total Ozone Mapping Spectrometer (TOMS), and stratospheric
column ozone from the Microwave Limb Sounder (MLS) instrument on the Upper Atmosphere Research Satellite (UARS). The tropospheric
column NO2 is measured by Global Ozone Monitoring Experiment (GOME). A global chemical and transport model (Model of Ozone and Related
Chemical Tracers, version 2; MOZART-2) is applied to analyze and interpret the satellite measurements. The study, which is
based on spring, summer, and fall months of 1997 shows generally good agreement between the model and satellite data with
respect to seasonal and spatial characteristics of O3 and NO2 fields. The analysis of the model results show that the industrial emission of NOx (NO + NO2) contributes about 50%–80% to tropospheric column NO2 in eastern Asia and about 20%–50% in southeastern Asia. The contribution of industrial emission of NOx to tropospheric column O3 ranges from 10% to 30% in eastern Asia. Biomass burning and lightning NOx emissions have a small effect on tropospheric O3 in central and eastern Asia, but they have a significant impact in southeastern Asia. The varying effects of NOx on tropospheric column ozone are attributed to differences in relative abundance of volatile organic compounds (VOCs) with
respect to total nitrogen in the two regions. 相似文献
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B. A. Ridley T. Zeng Y. Wang E. L. Atlas E. V. Browell P. G. Hess J. J. Orlando K. Chance A. Richter 《Journal of Atmospheric Chemistry》2007,57(3):255-280
During the Tropospheric Ozone Production about the Spring Equinox (TOPSE) program, aircraft flights during April 7–11, 2000
revealed a large area air mass capped below ∼500 m altitude over Hudson Bay, Canada in which ozone was reduced from normal
levels of 30–40 ppbv to as low as 0.5 ppbv. From some of the in-situ aircraft measurements, back-trajectory calculations,
the tropospheric column of BrO derived from GOME satellite measurements, and results from a regional model, we conclude that
the event did not originate from triggering of reactive halogen release in the sub-Arctic region of Hudson Bay but resulted
from such an event occurring at higher latitudes over the islands of the northern Canada Archipelago and nearby Arctic Ocean
with subsequent transport over a distance of 1,000–1,500 km to Hudson Bay. BrO
x
remained active during this transport despite considerable changes in the conditions of the underlying surface suggesting
that chemical recycling during transport dominated any local halogen input from the surface. If all of the tropospheric column
density of BrO is distributed uniformly within the surface layer, then the mixing ratio of BrO derived from the satellite
measurements is at least a factor of 2–3 larger than derived indirectly from in situ aircraft measurements of the NO/NO2 ratio. 相似文献
6.
利用1996年3月-2003年6月部分时段拉萨、西宁、北京3个站的臭氧探空资料验证了GOME(Global Ozone Monitoring Experiment)卫星臭氧廓线及对流层臭氧柱总量。对比结果表明:在对流层中下层,拉萨和西宁两地GOME与探空的平均偏差小于5%,北京地区平均偏差小于10%;在对流层上层/平流层下层,拉萨和西宁平均偏差小于10%,北京小于20%;在平流层中上层3个站的平均偏差均小于5%。在对流层上层/平流层下层区域,GOME与臭氧探空的平均偏差在北京明显高于拉萨和西宁。3个地区对流层柱总量的平均偏差都在10%以内,表明该资料可用于研究我国对流层臭氧总量的变化规律。同时段的GOME最低层(0~2.5km)月平均臭氧浓度对比结果显示,GOME结果同地面臭氧观测值有很好的相关性,GOME臭氧浓度反映了拉萨、瓦里关、临安地面臭氧浓度的主要变化特征。 相似文献
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利用GOME (Global Ozone Monitoring Experiment, 全球臭氧监测实验) 1996年1月—2002年12月NO2对流层柱浓度月平均卫星遥感资料以及根据北京市2001年1月1日—2002年12月31日NO2污染指数数据计算出的地面NO2日均质量浓度值, 分析了北京市城市大气NO2污染变化的季节变化特征以及年际变化, 并将2001年1月—2002年12月北京上空GOME NO2对流层柱浓度月平均值变化与北京市地面NO2日均质量浓度月平均值变化进行了比较, 结果表明两者随时间的变化趋势具有较好的一致性, 据此可以利用GOME NO2对流层柱浓度月平均卫星遥感资料来分析特定区域大气NO2的季节变化和年际变化。 相似文献
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