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1.
Th sorption and export models in the water column: A review 总被引:2,自引:3,他引:2
Nicolas Savoye Claudia Benitez-Nelson Adrian B. Burd J. Kirk Cochran Matthew Charette Ken O. Buesseler George A. Jackson Matthieu Roy-Barman Sabine Schmidt Marc Elskens 《Marine Chemistry》2006,100(3-4):234
Over the past few decades, the radioisotope pair of 238U / 234Th has been widely and increasingly used to describe particle dynamics and particle export fluxes in a variety of aquatic systems. The present paper is one of five review articles dedicated to 234Th. It is focused on the models associated with 234Th whereas the companion papers (same issue) are focused on present and future methodologies and techniques (Rutgers van der Loeff et al.), C / 234Th ratios (Buesseler et al.), 234Th speciation (Santschi et al.) and present and future applications of 234Th [Waples, J.T., Benitez-Nelson, C.R., Savoye, N., Rutgers van der Loeff, M., Baskaran, M., Gustafsson, Ö., this issue. An Introduction to the application and future use of 234Th in aquatic systems. Marine Chemistry, FATE special issue]. In this paper, we review current 234Th scavenging models and discuss the relative importance of the non-steady state and physical terms associated with the most commonly used model to estimate 234Th flux. Based on this discussion we recommend that for future work the use of models should be accompanied by a discussion of the effect that model and data uncertainty have on the model results. We also suggest that future field work incorporate repeat occupations of sample sites on time scales of 1–4 weeks in order to evaluate steady state versus non-steady state estimates of 234Th export, especially during high flux events (> ca. 800 dpm m− 2 d− 1). Finally, knowledge of the physical oceanography of the study area is essential, particularly in ocean margins and in areas of established upwelling (e.g., Equatorial Pacific). These suggestions will greatly enhance the application of 234Th as a tracer of particle dynamics and flux in more complicated regimes. 相似文献
2.
Re-Os Isotopic Measurements at the Femtomole Level in Natural Samples 总被引:17,自引:0,他引:17
Jean Louis Birck Matthieu Roy Barman Françoise Capmas 《Geostandards and Geoanalytical Research》1997,21(1):19-27
Here we describe a new chemical separation method for Os and an improved mass spectrometric procedure for Re and Os. This technique is based on the selective extraction of OsO4 from aqueous solution in liquid bromine. Among other advantages, this procedure avoids the cumbersome distillation procedure for Os and uses only commercial "off the shelf" PFA teflon labware. Blank levels for 0.5 g sample sizes are: 0.06 pg and 0.5 pg for Os and Re respectively. Samples containing as little as 1 pg g−1 Os can be analysed reliably with this method. Adaptation to other dissolution methods is also discussed. 相似文献
3.
Michel Magny Matthieu Honegger et Laurent Chalumeau 《Eclogae Geologicae Helvetiae》2005,98(2):249-259
Resume. Les fouilles archéologiques réalisées de 1998 à 2002 sur le site néolithique de Marin-Les Piécettes sur la rive nord-ouest
du lac de Neuchatel ont offert l’opportunité d’observer deux séquences sédimentaires intéressantes pour la reconstitution
des variations holocènes du niveau du lac, en particulier au cours de la période correspondant au changement de cours de l’Aar
en direction du nord-est, vers 5650–5500 cal BP. La géométrie des corps sédimentaires et les changements lithologiques permettent
de reconna?tre plusieurs phases majeures de bas niveaux relatifs du plan d’eau vers 6870, 5660, 5060–3990, 3580, 2280, 1640
et 1170 cal BP. Le site néolithique de Marin-Les Piécettes s’est développé vers 5454–5433 cal BP à la faveur d’un court épisode
de bas niveau du lac qui a interrompu une importante phase de haut niveau au début du Subboréal. Les événements paléohydrologiques
identifiés à Marin-Les Piécettes apparaissent cohérents avec ceux reconstitués sur le site de Montilier au bord du lac de
Morat, ainsi qu’avec les variations paléohydrologiques reconstituées à partir des lacs du Jura, du Plateau suisse et des Préalpes
du Nord fran?aises. Ceci suggère qu’ils témoignent d’un signal climatique. La séquence sédimentaire de Marin-Les Piécettes
met enfin en évidence la formation d’un cordon littoral sur la rive nord-ouest du lac juste après 5660 cal BP.
Manuscrit re?u le 22 septembre 2004 Révision acceptée le 11 mars 2005 相似文献
4.
Matthieu Gounelle Cécile Engrand Philip A. Bland Michael E. Zolensky Jean Duprat 《Geochimica et cosmochimica acta》2005,69(13):3431-3443
We have measured the hydrogen isotopic composition (D/H ratios) of the water from 13 carbonaceous chondritic microclasts (CCMs, size <1 mm) trapped in two howardites (Kapoeta and Yamato-793497) early in the evolution of Solar System. The division into tochilinite-rich; magnetite-rich, olivine-poor; magnetite-rich, olivine-rich CCM types is corroborated by the hydrogen isotopic compositions. Both mineralogy and hydrogen isotopic compositions demonstrate that tochilinite-rich CCMs represent CM2 chondritic matter. In contrast, there is no good match between the isotopic and mineralogical properties of the magnetite-rich CCMs and the known groups of carbonaceous chondrites, suggesting that magnetite-rich CCMs represent a new kind of chondritic matter, not yet sampled in meteorite collections. This demonstrates that the view of the asteroid belt revealed by the collection of meteorites is incomplete. The study of (micro)clasts offers a unique opportunity to better decipher the nature and relative abundance of asteroids.The average hydrogen isotopic composition of water belonging to CCMs, D/H = (152.0 ± 4.8) × 10−6 (1σm), is similar to that of Antarctic micrometeorites (AMMs), D/H = (161.2 ± 3.8) × 10−6 (1σm). The similarity, in terms of mineralogy and hydrogen isotopic composition, between CCMs and AMMs demonstrates that the composition of the micrometeorites has not been modified over the whole history of the Solar System. It indicates that the composition of the micrometeorite flux onto Earth has been, and is, dominated by a mixture of CM2-like; magnetite-rich, olivine-poor; magnetite-rich, olivine-rich carbonaceous chondritic matter exemplified by CCMs found in howardites. Because CCMs have not suffered atmospheric entry, they provide an abundant source of pristine micrometeorites.The average D/H ratio of the whole population of CCMs is identical within errors to that of the Earth (149 ± 3 × 10−6). The match between the CCMs D/H ratio and that of the Earth is especially remarkable because 1) three different populations of CCMs are needed to make the D/H ratio of the Earth; 2) there is no single carbonaceous chondrite group for which a similar match exists. This observation suggests that CCMs population might be representative of the late veneer agent(s) that delivered water to the Earth. 相似文献
5.
6.
A new elastoplastic model called loading memory surface based on the critical state concept and the multi‐surface framework is proposed for geomaterials. The model uses a hypoelastic formulation and two plastic mechanisms. The formulations of the model are made in three‐dimensional stress–strain space and work under both monotonic and cyclic loadings. A newly introduced formalism makes it possible to obtain the cyclic response directly from the monotonic loading one. This formalism gives a three‐dimensional generalization of the well‐known Masing rule. The model has been validated against test results of Hostun sand under several conditions: monotonic and cyclic, drained and undrained, tests in compression and in extension, and at different confining pressures and different densities. Copyright © 2014 John Wiley & Sons, Ltd. 相似文献
7.
8.
Although meteorites are now considered as scientific objects, they still bear a strong and powerful symbolic meaning due to their extraterrestrial provenance. The present article focuses on their legal status, in other words the collection of rules, very diverse in nature, which are applicable to them. Despite a growing international market, the question of meteorites is often ignored or regarded as a detail in international relations and is rarely taken explicitly into account in negotiations and treaties. This relative neglect explains why a non‐State player, the Meteoritical Society, has taken methodological initiatives into meteoritic science and has effectively become a regulator of meteorite naming and acceptance, with a global scope. We show that to understand the legal status of meteorites, it is necessary to consider them under the prism of public international law, transnational law, and national law. We conclude that, despite the universality of meteorites as extraterrestrial objects, the variability of legal rules applicable to meteorites depending onto which territory they fall or where they are found. We note, however, that there is a trend toward regulatory uniformity in the scientific analysis of meteorites, which frames the practices of researchers and regulates traders’ activities. Finally, we contend that a meteorite remains a badly defined legal object, because it can be viewed under many angles: as an object susceptible to private appropriation, as a “common thing” (res communis), or as an element of national heritage. 相似文献
9.
Philipp R. Heck Christopher Herd Jeffrey N. Grossman Dmitry Badjukov Audrey Bouvier Emma Bullock Hasnaa Chennaoui‐Aoudjehane Vinciane Debaille Tasha L. Dunn Denton S. Ebel Ludovic Ferrire Laurence Garvie Jrme Gattacceca Matthieu Gounelle Richard Herd Trevor Ireland Emmanuel Jacquet Robert J. Macke Tim McCoy Francis M. McCubbin Takashi Mikouchi Knut Metzler Mathieu Roskosz Caroline Smith Meenakshi Wadhwa Linda Welzenbach‐Fries Toru Yada Akira Yamaguchi Ryan A. Zeigler Michael Zolensky 《Meteoritics & planetary science》2019,54(7):1397-1400
10.