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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff
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We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
对于改进的Encke方法,选择适当的参考轨道是一个关键.然而,对于人造地球卫星长弧轨道计算,目前所给出的几种参考轨道均需要逐段校正,这将给定轨问题带来附加的复杂性.本文将仔细探讨如何选择参考轨道和减少校正次数. 相似文献
3.
The actual penetration depth of the Shoemaker-Levy 9 fragments into the Jovian atmosphere is still an open question. From fundamental equations of meteoric physics with variable cross-section, a new analytic model of energy release of the fragments is presented. In use of reasonable parameters, a series of results are calculated for different initial mass of the fragments. The results show that the largest fragment explodes above pressure levels of 3 bars and does not penetrate into the H2O cloud layer of the Jovian atmosphere, and that airburst of smaller fragments occur even above the upper cloud layer. 相似文献
4.
为建立社会主义市场经济的地矿工作新秩序,本文对国有地矿企业的经营者(厂长、经理)这一特殊群体进行了分析。着重研究了新形势下企业经营者实行年薪制的问题。指出年薪制就是以企业一个生产经营周期为单位确定经营者的报酬,这一周期通常为一年。进而阐述了为什么要实行企业经营者年薪制;企业经营者的收入应与职工工资完全脱钩;采用基础报酬加效益报酬的方法确定收入等等。并构想了实行经营者年薪制所需要的外部环境:建立经营者人才市场、经营者要能进能出、实行任职资格制度、建立风险机制、按劳动力市场经济规律办事。 相似文献
5.
Based on the CN and C2 comae isophotes for two comets (1961 IX and 1970 16) given by Rahe et al. and the relevant theory of physical chemistry, we have deduced the distributions of the CN and C2 modecules in the coma, their scale heights and mean lifetimes. The results favour the viewpoint that HCN is the parent of CN, and that C2H2 is the parent of C2. 相似文献
6.
THE SIMULATED STORAGE CAPACITY OF FLOOD AND WATERLOGGING IN THE TYPICAL AGRICULTURAL REGION IN JIANGHAN PLAIN 总被引:2,自引:0,他引:2
1INTRODUCTIONJianghanPlainisoneoftheimportantbasesofChina′sagriculturalproductivitylocatedinthemiddleChangjiangRivervalleyofcentralChina.TheJianghanplainapproximately6.6×104km2inareaandover30millioninpopulationistherenowned“countryoffishandrice"in… 相似文献
7.
Zhang Qing Wang Li-fan Hu Jing-yao P. A. Mazzali Wang Zhen-ru 《Chinese Astronomy and Astrophysics》1995,19(4):426-431
We present the modeling of the ultraviolet and optical spectra obtained simultaneously on 1993 April 15 with the HST and at Lick Observatory. A Monte Carlo code is employed in the modeling and a comparison is made between models reported by different groups. With an atmosphere similar to the Sun in chemical composition, the observed spectral lines are well reproduced by a power law density structure of index around 20 except the strong H and HeI λ5876 lines which have peculiar absorption profiles. The photospheric velocity is found to be 9500 km/s and the blackbody temperature of the spectrum is 7990 K. For H and HeI λ5876, we suggest a two-component density structure which has a smoother layer located immediately outside the steeply decreasing inner envelope. The power law indices are most probably 20 and 3, respectively, with the transition point at about 13 000 km/s. In addition, this outer smooth layer serves to flatten the far UV spectrum as observed. 相似文献
8.
A THREE-DIMENSIONAL ELASTIC NESTED-GRID MESO-(β-γ)SCALE ATMOSPHERIC MODEL——PARTI:MODEL DESCRIPTION
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A three-dimensional elastic nonhydrostatic mesoscale(β-γ)model with nested-grid is presented.It uses a set of fullequations in terrain-following coordinates as its basic dynamic frame,which is solved with a time-splitting algorithmfor acoustic and gravity waves.The model physical parameterization includes a K-theory subgrid eddy mixing for cloudand free atmosphere,a bulk planetary boundary layer parameterization,and three types of sofisticated cloudmicrophysics schemes with double-parameters for hail-bearing clouds,warm clouds and snowing clouds respectively.The model is designed to be used flexibly for simulations of a variety of meso-and small-scale atmospheric processes,and can be improved as a regional and local operational NWP system in future. 相似文献
9.
这里叙述的新发现仅指某一特殊类型的发现(如新星,超新星和小行星等)及某一特殊类型天体的认证(如X射线源证认为类星体等),而不包括某一类天体的某种天象及未知性质源的列表(如深度成像观测得到的前人没有纪录过的一般天体,如恒星,但一些特殊天体亦列入),由于收集不全面和所谓“发现”定义的困难,向有发向而未列入者先歉意。从80年代后期开始,我国的观测设备有了很大垢发展,所以有一批重的的天文发现,为天文提供了很好的机会,它包括下面几方面,层系层次天体:(1)用X射线源和射电源证认了一批包括类星体,BL Lac天体,赛弗特天体在内的活动星系核;(2)用IRAS源证认了一批W-R星系;(3)BATC巡天在一个星系周围发现了一个“环”。恒星层次天体:(1)河外星系中发现了一批超新星的一个新星,(2)发现了和用ROSAT源证认了一批激变变星,(4)BATC和超新星巡天发现了一批变星,(4)发现了若干新的δSct变星,(5)发现了一批Herbig-Haro天体,(6)发现了一批水脉泽。行星层次天体:(1)发现了大批小行星,特别是有些是近地不行星,(20发现若干彗星。 相似文献
10.
作者用透射电子显微镜研究了沉积钙质白云石中的带状面缺陷。在衍衬象中面缺陷呈现出特有的条纹衬度,并具有一定的择优取向,它们沿着{018}面排列。面缺陷也可分叉,分枝部分平等于{2-/10}面。根据白云石面缺陷的取向,本文提出了鞍状白云石宏观弯曲面和微观面缺陷的取向关系。 相似文献