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1.
2.
Multiple sulfur isotope system is a powerful new tracer for atmospheric, volcanic, and biological influences on sulfur cycles in the anoxic early Earth. Here, we report high-precision quadruple sulfur isotope analyses (32S/33S/34S/36S) of barite, pyrite in barite, and sulfides in related hydrothermal and igneous rocks occurring in the ca. 3.5 Ga Dresser Formation, Western Australia. Our results indicate that observed isotopic variations are mainly controlled by mixing of mass-dependently (MD) and non-mass-dependently fractionated (non-MD) sulfur reservoirs. Based on the quadruple sulfur isotope systematics (δ34S-Δ33S-Δ36S) for these minerals, four end-member sulfur reservoirs have been recognized: (1) non-MD sulfate (δ34S = −5 ± 2‰; Δ33S = −3 ± 1‰); (2) MD sulfate (δ34S = +10 ± 3‰); (3) non-MD sulfur (δ34S > +6‰; Δ33S > +4‰); and (4) igneous MD sulfur (δ34S = Δ33S = 0‰). The first and third components show a clear non-MD signatures, thus probably represent sulfate and sulfur aerosol inputs. The MD sulfate component (2) is enriched in 34S (+10 ± 3‰) and may have originated from microbial and/or abiotic disproportionation of volcanic S or SO2. Our results reconfirm that the Dresser barites contain small amounts of pyrite depleted in 34S by 15-22‰ relative to the host barite. These barite-pyrite pairs exhibit a mass-dependent relationship of δ33S/δ34S with slope less than 0.512, which is consistent with that expected for microbial sulfate reduction and is significantly different from that of equilibrium fractionation (0.515). The barite-pyrite pairs also show up to 1‰ difference in Δ36S values and steep Δ36S/Δ33S slopes, which deviate from the main Archean array (Δ36S/Δ33S = −0.9) and are comparable to isotope effects exhibited by sulfate reducing microbes (Δ36S/Δ33S = −5 to −11). These new lines of evidence support the existence of sulfate reducers at ca. 3.5 Ga, whereas microbial sulfur disproportionation may have been more limited than recently suggested. 相似文献
3.
The Lagrangian diffusion equation appropriate for the dispersion of current followers (e. g., floats, drogues, drifters) is proposed. The analytical solution to the equation is obtained for a uniform deformation field, characterized by Lagrangian deformations and anisotropic eddy diffusivities both varying with time. Expressions are derived for the patch area and its elongation and rotation. For small values of elapsed time after the initial release the patch area can be accounted for by the exponential of the cumulative value of the horizontal divergence; the relative rate of change of the patch area can be accounted for by the horizontal divergence. 相似文献
4.
Yoshio Takasugi Akira Hoshika Hideaki Noguchi Terumi Tanimoto 《Journal of Oceanography》1994,50(1):65-80
The strong tidal current (tidal jet) in straits generates tidal vortices with a scale of several kilometers. The role of the vortices in material transport was investigated in the Neko Seto Sea, located in the western part of the Seto Inland Sea of Japan. A clockwise vortex with a diameter of about 0.8 km was observed in Nigata Bay (lying between two straits, the Neko Seto Strait and the Meneko Seto Strait). It was concluded that the clockwise vortex was the tidal vortex which was generated by the tidal jet in the Meneko Seto Strait. The vortex moved into the bay with the tide, but tended to stay on the sand bank in the bay. It was confirmed by current measurement with an ADCP and turbidity measurement that the secondary convergent flow was generated in the bottom layer of the vortex. This secondary flow seemed to contribute to the formation of the sand bank. It was suggested that tidal vortices may play an important role in the sediment transport and formation of topography in and around straits. 相似文献
5.
Tetsuo Yanagi Satoru Takahashi Akira Hoshika Terumi Tanimoto 《Journal of Oceanography》1996,52(5):539-552
Seasonal variation in the transport of suspended matter across the East China Sea is investigated with the use of results of field observations and diagnostic numerical experiments. Suspended matter is transported from the shelf edge to the inner shelf in summer and from the inner shelf to the shelf edge in autumn and winter due to the vertical circulation mainly induced by the monsoon wind. The maximum transport of suspended matter from the inner shelf to the shelf edge occurs in autumn. 相似文献
6.
Radiocarbon and total carbonate data were obtained near the 1973 GEOSECS stations in the North Pacific along 30°N and along 175°E between 1993 and 1994. In these stations, we estimated radiocarbon originating from atomic bomb tests using tritium, trichlorofluoromethane and silicate contents. The average penetration depth of bomb radiocarbon during the two decades has deepened from 900 m to 1300 m. Bomb radiocarbon inventories above the average value for the whole North Pacific were found widely in the western subtropical region around 30°N both in the 1970s and 1990s, and its area in the 1990s was broader than that in the 1970s. In most of the North Pacific, while the bomb radiocarbon has decreased above 25.4, the bomb radiocarbon flux below 25.4 was over 1 × 1012 atom m-2yr-1 in the subtropical region around 30°N. In the tropical area south of 20°N, the bomb radiocarbon inventory below 25.4 increased from zero to over 10 × 1012 atom m-2 during the last three decades. These distributions suggest that the bomb radiocarbon removed from the surface is currently accumulated with bomb 14C flux of over 1 × 1012 atom m-2yr-1 below 25.4 in the subtropical region, mainly by advection from the higher latitude, and that part of the accumulated bomb 14C gradually spread southward with about 30 years. 相似文献
7.
Carbon and nitrogen stable isotope ratios (13C and 15N) of surface sediments were measured within Osaka Bay, in the Seto Inland Sea in Japan, in order to better understand the sedimentation processes operating on both terrestrial and marine organic matter in the Bay. The 13C and 15N of surface sediments in the estuary of the Yodo River were less than –23 and 5 respectively, but increased in the area up to about 10 km from the river mouth. At greater distances they became constant (giving 13C of about –20 and 15N about 6). It can be concluded that large amounts of terrestrial organic matter exist near the mouth of the Yodo River. Stable isotope ratios in the estuary of the Yodo River within 10 km of the river mouth were useful indicators allowing study of the movement of terrestrial organic matter. Deposition rates for total organic carbon (TOC) and total nitrogen (TN) over the whole of the Bay were estimated to be 63,100 ton C/year and 7,590 ton N/year, respectively. The deposition rate of terrestrial organic carbon was estimated to be 13,200 (range 2,000–21,500) ton C/year for the whole of Osaka Bay, and terrestrial organic carbon was estimated to be about 21% (range 3–34) of the TOC deposition rate. The ratio of the deposition rate of terrestrial organic carbon to the rate inflow of riverine TOC and particulate organic carbon (POC) were estimated to be 19% (range 3–31) and 76% (range 12–100), respectively. 相似文献
8.
Akira Shibata Kouichi Ohwada Masakazu Tsuchiya Kazuhiro Kogure 《Journal of Oceanography》2006,62(1):91-97
Peptidoglycan (PG) is a biopolymer found exclusively in the cell wall of bacteria. Recent chemical analysis of particulate
organic matter suggests that a major amount of the muramic acid, an amino sugar present only in PG, could not be accounted
for in terms of bacterial cells (Benner and Kaiser, 2003); however, data on particulate PG is quite sparse. In the present
study, conducted in 1996, the PG was examined at 5 sampling sites in the northwestern Pacific Ocean, and in natural seawater
cultures. Particulate PG, which was concentrated using a 96-well filtration plate equipped with Durapore filters (pore size,
0.22 μm), was measured by the silkworm larvae plasma (SLP) assay. The PG concentration generally decreased with depth and
correlated significantly with bacterial abundance throughout the entire water column. However, the ratio of particulate PG
to bacterial abundance varied with depth. The average ratio was 0.61 ± 0.53 (average ± SD, n = 40) between 50 and 2000 m,
which agreed with the bacterial cellular PG content from 0.63 to 1.1 fg cell−1 obtained in seawater cultures. On the other hand, the ratios of PG to bacteria from the surface to 50 m (3.7 ± 2.6, n = 29)
and below 2,000 m (2.1 ± 1.7, n = 7) were significantly higher than that between 50 and 2,000 m. These results may suggest
that, in the surface and deep layers, a significant fraction of particulate PG was present in bacterial detritus, whereas
this fraction was reduced in the middle layer. 相似文献
9.
10.
Sea water samples were collected from various depths in the North Pacific (40–21°N) along 165°E in 1991. Their total carbonate (total dissolved carbonate species) contents were determined with random errors less than 0.2% by a coulometric method. The preformed carbonate contents defined by Chen (1982) were calculated from the obtained data and other observed data including potential temperature, salinity, dissolved oxygen and total alkalinity. The same calculation was done for the GEOSECS data obtained in nearly the same region in 1973. The difference between the two data sets reveals that the preformed carbonate has increased by 180±41 gC/m2 during the last 18 years. This value is comparable or somewhat larger than 150 gC/m2 obtained in the case that the ocean uptakes 3 GtC/yr for 18 years and distributes it equally among the world oceans. Based on the results, a hypothesis on the missing sink for the anthropogenic carbon dioxide is presented, in that the missing sink is the intermediate waters formed in the northern North Pacific and the Southern Ocean besides the deep waters formed in the North Atlantic and the Southern Ocean. 相似文献