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François M. Costard 《Earth, Moon, and Planets》1989,45(3):265-290
In order to quantify the spatial distribution of volatiles on Mars, 2600 fluidized ejecta craters have been systematically measured, classified and mapped over the planet Mars, using 1 : 2 M scale USGS photomosaics. The latitudinal distribution of ejecta craters reveals that flower ejecta deposits (Type 1), together with low mobility ejecta, are frequently observed in the equatorial region and on ridged plains. Rampart craters (Type 2), with high mobility ejecta, occur at mid latitudes and exhibit a spatial relationship with polygonal patterns and pseudocrater areas. The increase of ejecta mobility with latitude attests for a concentration of volatiles at high latitudes. Statistical analysis shows that cratered uplands and ridged plains contain less volatile material near the surface than the underlying materials. In Chryse Planitia and Utopia Planitia the statistical study and the spatial relationships between polygonally fractured patterns, pseudocraters and the great number of high mobility ejecta deposits suggest the presence of a water-rich alluvial deposit close to the surface near the mouth of Chryse and Elysium channels. This result explains, on a more quantitative basis, the idea that fractured patterns were preferentially developed in a volatile-rich sedimentary deposits. The behaviour of volatiles, at 41 S, 257 W near Reull Vallis, exhibits a strong anomaly, with the presence of an abnormally volatile rich layer close to the surface. 相似文献
4.
Yves Goddéris Louis M. François Jacques Schott David Labat 《Geochimica et cosmochimica acta》2006,70(5):1128-1147
A numerical model of chemical weathering in soil horizons and underlying bedrock (WITCH) has been coupled to a numerical model of water and carbon cycles in forest ecosystems (ASPECTS) to simulate the concentration of major species within the soil horizons and the stream of the Strengbach granitic watershed, located in the Vosges Mountains (France). For the first time, simulations of solute concentrations in soil layers and in the catchment river have been performed on a seasonal basis. The model is able to reproduce the concentrations of most major species within the soil horizons, as well as catching the first-order seasonal fluctuations of aqueous calcium, magnesium and silica concentrations. However, the WITCH model underestimates concentrations of Mg2+ and silica at the spring of the catchment stream, and significantly underestimates Ca2+ concentration. The deficit in calculated calcium can be compensated for by dissolution of trace apatite disseminated in the bedrock. However, the resulting increased Ca2+ release yields important smectite precipitation in the deepest model layer (in contact with the bedrock) and subsequent removal of large amount of silica and magnesium from solution. In contrast, the model accurately accounts for the concentrations of major species (Ca, Mg and silica) measured in the catchment stream when precipitation of clay minerals is not allowed. The model underestimation of Mg2+ and H4SiO4 concentrations when precipitation of well crystallized smectites is allowed strongly suggests that precipitation of well crystallized clay minerals is overestimated and that more soluble poorly crystallized and amorphous materials may be forming. In agreement with observations on other watersheds draining granitic rocks, this study indicates that highly soluble trace calcic phases control the aqueous calcium budget in the Strengbach watershed. 相似文献
5.
Dominique AubertPeter Stille Anne ProbstFrançois Gauthier-lafaye Laurent PourcelotMireille Del nero 《Geochimica et cosmochimica acta》2002,66(19):3339-3350
Rainwater and snow collected from three different sites in France (Vosges Mountains, French Alps and Strasbourg) show more or less similar shapes of their REE distribution patterns. Rainwater from Strasbourg is the most REE enriched sample, whereas precipitations from the two mountainous, less polluted catchments are less REE enriched and have concentrations close to seawater. They are all strongly LREE depleted.Different water samples from an Alpine watershed comprising snow, interstitial, puddle and streamwater show similar REE distributions with LREE enrichment (rainwater normalized) but MREE and HREE depletion. In this environment, where water transfer from the soil to the river is very quick due to the low thickness of the soils, it appears that REE in streamwater mainly originate from atmospheric inputs. Different is the behaviour of the REE in the spring- and streamwaters from the Vosges Mountains. These waters of long residence time in the deep soil horizons react with soil and bedrock REE carrying minerals and show especially significant negative Eu anomalies compared to atmospheric inputs. Their Sr and Nd isotopic data suggest that most of the Sr and Nd originate from apatite leaching or dissolution. Soil solutions and soil leachates from the upper soil horizons due to alteration processes strongly depleted in REE carrying minerals, have REE distribution patterns close to those of lichens and throughfall. Throughfall is slightly more enriched especially in light REE than filtered rainwater probably due to leaching of atmospheric particles deposited on the foliage and also to leaf excretion.Data suggest that Sr and Nd isotopes of the soil solutions in the upper soil horizons originate from two different sources: 1) An atmospheric source with fertilizer, dust and seawater components and 2) A source mainly determined by mineral dissolution in the soil. These two different sources are also recognizable in the Sr and Nd isotopic composition of the tree’s throughfall solution. The atmospheric contributions of Sr and Nd to throughfall and soil solution are of 20 to 70 and 20%, respectively. In springwater, however, the atmospheric Sr and REE contribution is not detectable. 相似文献
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Isotope fractionation of electroplated Fe was measured as a function of applied electrochemical potential. As plating voltage was varied from −0.9 V to 2.0 V, the isotopic signature of the electroplated iron became depleted in heavy Fe, with δ56Fe values (relative to IRMM-14) ranging from −0.18(±0.02) to −2.290(±0.006) ‰, and corresponding δ57Fe values of −0.247(±0.014) and −3.354(±0.019) ‰. This study demonstrates that there is a voltage-dependent isotope fractionation associated with the reduction of iron. We show that Marcus’s theory for the kinetics of electron transfer can be extended to include the isotope effects of electron transfer, and that the extended theory accounts for the voltage dependence of Fe isotope fractionation. The magnitude of the electrochemically-induced fractionation is similar to that of Fe reduction by certain bacteria, suggesting that similar electrochemical processes may be responsible for biogeochemical Fe isotope effects. Charge transfer is a fundamental physicochemical process involving Fe as well as other transition metals with multiple isotopes. Partitioning of isotopes among elements with varying redox states holds promise as a tool in a wide range of the Earth and environmental sciences, biology, and industry. 相似文献
8.
François Farges 《Physics and Chemistry of Minerals》2009,36(8):463-481
Cr K-edge XANES spectra were obtained for a variety of Cr-bearing model compounds containing Cr(II), Cr(III), Cr(IV), Cr(V) and Cr(VI), in which the Cr-site symmetry is D4h, Oh and Td. The centroid position of the pre-edge feature is a better indicator of the Cr valence than the edge position. In Cr-rich oxides, higher-energy transitions must be excluded in order to refine a robust valence for Cr. The pre-edge for chromates is not unique and varies as a function of the CrO4 2? moiety distortion, which is often related to Cr-polymerization (monochromate vs. dichromate). Both the analogy with the Mn K-pre-edge information and ab initio FEFF calculations of the pre-edge feature for Cr(III) and Cr(VI) confirm the experimental trends. This methodology is applied to the Cr K-edge pre-edge feature collected in gems (emerald, spinel and ruby), the layered minerals fuchsite and kämmererite, two Cr-bearing aqueous solutions and a set of sodo-calcic silicate glasses used for bottling sparkling white wine. In emerald and fuchsite, the Cr-site is differently distorted than its ruby or spinel counterpart. In a Cr(III)-bearing aqueous solution and sodo-calcic glass, no evidence for Cr(III) with Td and C3v symmetry is detected. However, minor amounts of chromate moieties (most likely monomeric) are detected in a glass synthesized in air. Preliminary spectra for the wine bottle glass suggest that only trace amounts of chromates might possibly be present in these glasses. 相似文献
9.
Surface rupture and source fault of the 20 February 1956 Eskişehir earthquake have been a matter of debate that potentially
contributes towards the understanding of the active deformation and seismic risk in the highly populated NW Anatolia. Field
observations on the two fault segments (namely Kavacık and Uludere faults) in the north of the Eskişehir graben revealed evidences
of co-seismic surface rupture and mass movements during the Eskişehir earthquake. Surface rupture was observed as a 2.5m wide,
a 100m long and ca. 20 cm deep asymmetric depression in the Gümüşlü valley, 2 km east of the Uludere village. A trench dug
on this depression confirms a prominent high-angle south dipping fault (dominantly left lateral strike slip) and two faint
north-dipping antithetics as clear noticeable shear zones in organic-rich thick soil. Mass failures are particularly observed
in spring depressions filled with loose torrent and carbonaceous material in front of the fault scarp. Some rock slides of
several tens of meters in size that obviously require significantly high ground shaking were also developed on steep fault
scarps. The orientation of the principal stress tensor as deduced from the surface rupture of the Eskişehir earthquake displays
clear inconsistency with the geometry of prominent faults in the area. We concluded that this disagreement may be explained
by a curved surface rupture. The western and eastern tips of this rupture are EW trending and the probable NW-running part
in the middle would correspond to the bounding zone between two right-stepping faults. 相似文献
10.
Marie-Françoise Bonifay 《Quaternary Research》1980,14(2):251-262
This study is the first test of correlation between the results obtained on the large Plio-Pleistocene European faunas and the main climatic stages (cold as well as temperate) demonstrated in marine isotopic records. In particular, there are cold stages which often explain the disappearance of some species, as well as climatic events that promote the substitution of some species by other groups. A rather evident parallelism appears between the European succession of large faunal associations and paleoclimatic stages revealed in oceanic areas, but some discordance occurs in the later periods. Faced with the great diversification of the Quaternary faunas, probably due to the multiplicity of climatic environments, and with global information from oceanic records, only local biostratigraphic studies will allow precise reconstruction of the different biotopes. 相似文献