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1.
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An overview is presented on possible mechanisms that control the leaching behaviour of the oxyanion forming elements As, Cr, Mo, Sb, Se, V and W in cementituous systems and alkaline solid wastes, such as municipal solid waste incinerator bottom ash, fly ash and air pollution control residues, coal fly ash and metallurgical slags. Although the leachability of these elements generally depends on their redox state, speciation measurements are not common. Therefore, experimental observations available in the literature are combined with a summary of the thermal behaviour of these elements to assess possible redox states in freshly produced alkaline wastes, given their origin at high temperature. Possible redox reactions occurring at room temperature, on the other hand, are reviewed because these may alter the initial redox state in alkaline wastes and their leachates. In many cases, precipitation of oxyanions as a pure metalate cannot provide a satisfactory explanation for their leaching behaviour. It is therefore highly likely that adsorption and solid solution formation with common minerals in alkaline waste and cement reduce the leachate concentration of oxyanions below pure-phase solubility. 相似文献
3.
Claude Boutron Kevin Rosman Carlo Barbante Michael Bolshov Freddy Adams Sungmin Hong Christophe Ferrari 《Comptes Rendus Geoscience》2004,336(10):847-867
The investigation of the occurrence of lead in dated snow and ice from Greenland and Antarctica has played a major role in our understanding of the history of the pollution of the atmosphere of our planet by this metal. Such studies have however proved to be very demanding, mainly because of the extreme purity of polar snow and ice. Reliable measurements can be obtained only if ultra-clean and highly sensitive procedures are used, as pioneered by Clair Patterson. The Greenland data show evidence of large-scale pollution of the atmosphere of the Northern Hemisphere for lead as early as two millennia ago during Greco–Roman times, especially because of mining and smelting activities in southern Spain. It peaked at the end of the 1960s, with lead concentrations in snow about 200 times higher than natural values, before declining during recent times because of the fall in the use of leaded gasoline. Lead pollution in Antarctica was already significant at the end of the 19th century as a consequence of whaling activities, the traffic of coal-powered ships crossing the Cape Horn, and mining activities in South America, South Africa and Australia. After declining because of the opening of the Panama Canal, the great economic depression and World War II, it reached a maximum during the 1980s, with lead concentrations 20 times higher than natural values. Other studies focus on past natural variations of lead in ancient ice dated from the last climatic cycles. To cite this article: C. Boutron et al., C. R. Geoscience 336 (2004). 相似文献
4.
Tommaso De Pippo Carlo Donadio Micla Pennetta Francesco Terlizzi Carlo Vecchione Margherita Vegliante 《Marine Ecology》2002,23(S1):154-168
Abstract. The interaction of coastal and submarine morphology with the hydrodynamic regimes exerts a control on coastal dynamic processes, conditioning the dispersion of sediments and potential pollutants existing in the area. Thus, the study of such parameters is useful in order to define environmental threats. Within the submerged sector of the Bagnoli coast and particularly in the southern part of the investigated area, there are sediment groups composed of very fine sands located in low-energy zones due to wave refraction and diffraction; they can also be found on the sea bottom and on the man-made structures typical of this zone. These areas show high pollutant levels of N, P, Cu, Fe, Mn, Ni, Pb, Zn, Cd, polyaromatic hydrocarbons (PAHs) and polychlorinated bi-phenyls (PCBs). The northern area, a place of high-energy hydrodynamic processes, also shows high concentration levels of pollutants due to the presence of secondary cell circulation.
Morphological research and analysis of textural characteristics of bottom sediments along the Bagnoli coast allowed the actual processes and their evolution in space and time to be defined. It has also been possible to correlate such processes to the seabed morphology system, the wave formations which affect the coast, the complex system of sediment transport, as well as to the man-made interventions in the area. The results of recent chemical analyses of beach sediments and bottom sediments off the Bagnoli coast were also incorporated. They prove the presence of heavy metals, PAHs and PCBs in high and sometimes very high concentrations. Finally, based on the results of research and analyses, a hypothesis for an intervention for environmental restoration has been formulated in order to renaturalise the coast through dredging and treatment of the sand, both on the seabed and on the emerged beach. 相似文献
Morphological research and analysis of textural characteristics of bottom sediments along the Bagnoli coast allowed the actual processes and their evolution in space and time to be defined. It has also been possible to correlate such processes to the seabed morphology system, the wave formations which affect the coast, the complex system of sediment transport, as well as to the man-made interventions in the area. The results of recent chemical analyses of beach sediments and bottom sediments off the Bagnoli coast were also incorporated. They prove the presence of heavy metals, PAHs and PCBs in high and sometimes very high concentrations. Finally, based on the results of research and analyses, a hypothesis for an intervention for environmental restoration has been formulated in order to renaturalise the coast through dredging and treatment of the sand, both on the seabed and on the emerged beach. 相似文献
5.
Mariano Angelo Zanini Carlo Pellegrino Riccardo Morbin Claudio Modena 《Bulletin of Earthquake Engineering》2013,11(2):561-579
This paper investigates the problem of management, maintenance and planning of interventions in transport networks located in seismic zones, in relation to the actual state of degradation of their most vulnerable elements, as bridges. The study consists in two phases: the first phase is concerned with definition of the seismic vulnerability of a typical bridge in the network, through the construction of fragility curves calculated taking into account the corrosion of the reinforcing steel as the main cause of environmental deterioration. Once the fragility curves of the deteriorated bridges are computed, the second phase consists in the analysis of the vulnerability of the transport network in which the bridges are included taking into account the modification of the traffic flows when bridge infrastructures are damaged. The results of this pilot study can be used as a first step for a proper allocation of economic resources in the planning of seismic retrofit interventions to minimize the overall risk and manage the immediate post-earthquake emergency phase and guide rescuers in reaching the affected and critical areas. 相似文献
6.
Posidonia oceanica meadows can be severely damaged by dredge-fill operations. We report on the construction of gas pipelines that occurred between 1981 and 1993 in SW Sicily, Italy. A large portion of the meadow was mechanically removed, and the excavated trench was filled with a mosaic of substrates, ranging from sand to consolidated rock debris. Meadow loss and recovery were quantified over 7 years after the end of operations. We recorded an overall loss of 81.20 ha of meadow. Substrate strongly affected recovery as the percent cover by P. oceanica consistently increased on calcareous rubble, reaching values of 44.37 ± 3.05% in shallow sites after 7 years, whereas no significant increase occurred on other substrates. As in the Mediterranean Sea exploitation of coastal areas continues to grow with consequent impacts on P. oceanica meadows, this case study illustrates how artificial rubble-like materials could be employed to support the restoration of damaged meadows. 相似文献
7.
8.
Hydrologic changes have a great impact on the long-term river morphology. The most common anthropic cause is the construction of dams, which often reduces both the discharge regime and sediment transport, producing a narrowing and degradation of the river bed. In this study we propose a simple, lumped morphodynamic model that describes fluvial cross-section dynamics consequent to changes in discharge and sediment transport induced by external factors. The model provides the temporal dynamics of the river width and bed quote. These dynamics result not to be trivial and can exhibit non monotonic behavior, with aggradations and degradations, and narrowing and widening. The model has been tested on real rivers using data obtained from field studies. The agreement between the outcomes and the data measured in the field works is always satisfactory. 相似文献
9.
A temporary accelerometer network has been installed in Tarcento (Friuli, NE Italy), a small town heavily hit by the 1976–1977
Friuli earthquake sequence, as a part of an ongoing research project aimed at ground motion simulation and generation of shakemaps
in the near-field of an earthquake. The network operated from October 2008 to April 2010 and consisted of three K2 accelerographs
with internal Episensor, distributed over a linear array of about 1.5 km length. Tarcento town had been chosen, at the end
of the 1970s, as the ideal site for a pilot microzonation study, the first of this kind in Italy, in which a substantial number
of field (and laboratory) tests were carried out in order to assess the mechanical properties of local alluvium deposits and
their complex (3D) geometrical configuration. The data from the temporary network, illustrated herein, allow for proper verification
and review of some of the quantitative predictions formulated in the 1980 study. As argued in the discussion section, we also
believe that the data are apt to provide valuable information of more general interest on the complex seismic response of
alluvium-filled valleys, and we show therein how the observations can be interpreted in the light of presently available parametric
simulation studies and simplified criteria for handling basin amplification effects. 相似文献
10.
Thomas A. Vogel Timothy P. Flood Lina C. Patino Melissa S. Wilmot Raymond Patrick R. Maximo Carmencita B. Arpa Carlo A. Arcilla James A. Stimac 《Contributions to Mineralogy and Petrology》2006,151(3):267-281
Silicic volcanic deposits (>65 wt% SiO2), which occur as domes, lavas and pyroclastic deposits, are relatively abundant in the Macolod Corridor, SW Luzon, Philippines.
At Makiling stratovolcano, silicic domes occur along the margins of the volcano and are chemically similar to the silicic
lavas that comprise part of the volcano. Pyroclastic flows are associated with the Laguna de Bay Caldera and these are chemically
distinct from the domes and lavas at Makiling stratovolcano. As a whole, samples from the Laguna de Bay Caldera contain lower
concentrations of MgO and higher concentrations of Fe2O3(t) than the samples from domes and lavas. The Laguna de Bay samples are more enriched in incompatible trace elements. The silicic
rocks from the domes, Makiling Volcano and Laguna de Bay Caldera all contain high alkalis and high K2O/Na2O ratios. Melting experiments of primitive basalts and andesites demonstrate that it is difficult to produce high K2O/Na2O silicic magmas by fractional crystallization or partial melting of a low K2O/Na2O source. However, recent melting experiments (Sisson et al., Contrib Mineral Petrol 148:635–661, 2005) demonstrate that extreme
fractional crystallization or partial melting of K-rich basalts can produce these silicic magmas. Our model for the generation
of the silicic magmas in the Macolod Corridor requires partial melting of mantle-derived, evolved, moderate to K-rich, crystallized
calc-alkaline magmas that ponded and crystallized in the mid-crust. Major and trace element variations, along with oxygen
isotopes and ages of the deposits, are consistent with this model.
Electronic Supplementary Material Supplementary material is available for this article at 相似文献