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1.
We present a computer model calculation for the racemization of a possible excess of amino acids in the icy fraction of comet nuclei bring about by ionizing radiation released during the decay of26Al,40K,235U,238U and232Th. The model takes into account a total of 110 chemical reactions, of which 91 are needed to explain the radiation chemical processing of the major constituents of comet nuclei (Navarro-Gonzálezet al., 1992) and 19 are necessary to simulate the radiolysis of glycine/alanine mixtures in aqueous solutions (Navarro-Gonzálezet al., 1994 and 1996). It is predicted that an enantiomeric excess of alanine would not be destroyed by radioracemization during the decay of embedded radionuclides. Nevertheless, this enantiomeric excess could be attenuated by the formation of racemic amino acids in the interior of comet nuclei as a result of the radiation-induced polymerization of HCN. 相似文献
2.
Andrew J. L. Harris Anna L. Butterworth Richard W. Carlton Ian Downey Peter Miller Pedro Navarro David A. Rothery 《Bulletin of Volcanology》1997,59(1):49-64
Satellite data offer a means of supplementing ground-based monitoring during volcanic eruptions, especially at times or locations
where ground-based monitoring is difficult. Being directly and freely available several times a day, data from the advanced
very high resolution radiometer (AVHRR) offers great potential for near real-time monitoring of all volcanoes across large
(3000×3000 km) areas. Herein we describe techniques to detect and locate activity; estimate lava area, thermal flux, effusion
rates and cumulative volume; and distinguish types of activity. Application is demonstrated using data for active lavas at
Krafla, Etna, Fogo, Cerro Negro and Erebus; a pyroclastic flow at Lascar; and open vent systems at Etna and Stromboli. Automated
near real-time analysis of AVHRR data could be achieved at existing, or cheap to install, receiving stations, offering a supplement
to conventional monitoring methods.
Received: 21 January 1997 / Accepted: 3 April 1997 相似文献
3.
Trace elements contamination of agricultural soils affected by sulphide exploitation (Iberian Pyrite Belt,Sw Spain) 总被引:1,自引:0,他引:1
Agricultural soils of the Riotinto mining area (Iberian Pyrite Belt) have been studied to assess the degree of pollution by
trace elements as a consequence of the extraction and treatment of sulphides. Fifteen soil samples were collected and analysed
by ICP-OES and INAA for 51 elements. Chemical analyses showed an As–Cu–Pb–Zn association related with the mineralisation of
the Iberian Pyrite Belt. Concentrations were 19–994 mg kg−1 for As, 41–4,890 mg kg−1 for Pb, 95–897 mg kg−1 for Zn and of 27–1,160 mg kg−1 for Cu. Most of the samples displayed concentrations of these elements higher than the 90th percentile of the corresponding
geological dominium, which suggests an anthropogenic input besides the bedrock influence. Samples collected from sediments
were more contaminated than leptosols because they were polluted by leachates or by mining spills coming from the waste rock
piles. The weathering of the bedrock is responsible for high concentrations in Co, Cr and Ni, but an anthropogenic input,
such as wind-blown dust, seems to be indicative of the high content of As, Cu, Pb and Zn in leptosols. The metal partitioning
patterns show that most trace elements are associated with Fe amorphous oxy-hydroxides, or take part of the residual fraction.
According to the results obtained, the following mobility sequence is proposed for major and minor elements: Mn, Pb, Cd, > Zn,
Cu > Ni > As > Fe > Cr. The high mobility of Pb, Cu and Zn involve an environmental risk in this area, even in soils where
the concentrations are not so high. 相似文献
4.
Pedro J. Marenco Frank A. Corsetti Douglas E. Hammond Alan J. Kaufman David J. Bottjer 《Chemical Geology》2008,247(1-2):124-132
The sulfur isotopic composition of carbonate associated sulfate (CAS) has been used to investigate the geochemistry of ancient seawater sulfate. However, few studies have quantified the reliability of δ34S of CAS as a seawater sulfate proxy, especially with respect to later diagenetic overprinting. Pyrite, which typically has depleted δ34S values due to authigenic fractionation associated with bacterial sulfate reduction, is a common constituent of marine sedimentary rocks. The oxidation of pyrite, whether during diagenesis or sample preparation, could thus adversely influence the sulfur isotopic composition of CAS. Here, we report the results of CAS extractions using HCl and acetic acid with samples spiked with varying amounts of pyrite. The results show a very strong linear relationship between the abundance of fine-grained pyrite added to the sample and the resultant abundance and δ34S value of CAS. This data represents the first unequivocal evidence that pyrite is oxidized during the CAS extraction process. Our mixing models indicate that in samples with much less than 1 wt.% pyrite and relatively high δ34Spyrite values, the isotopic offset imparted by oxidation of pyrite should be much less than ? 4‰. A wealth of literature exists on the oxidation of pyrite by Fe3+ and we believe this mechanism drives the oxidation of pyrite during CAS extraction, during which the oxygen used to form sulfate is taken from H2O, not O2. Consequently, extracting CAS under anaerobic conditions would only slow, but not halt, the oxidation of pyrite. Future studies of CAS should attempt to quantify pyrite abundance and isotopic composition. 相似文献
5.
Quantitative sinkhole hazard assessments in karst areas allow calculation of the potential sinkhole risk and the performance
of cost-benefit analyses. These estimations are of practical interest for planning, engineering, and insurance purposes. The
sinkhole hazard assessments should include two components: the probability of occurrence of sinkholes (sinkholes/km2 year) and the severity of the sinkholes, which mainly refers to the subsidence mechanisms (progressive passive bending or
catastrophic collapse) and the size of the sinkholes at the time of formation; a critical engineering design parameter. This
requires the compilation of an exhaustive database on recent sinkholes, including information on the: (1) location, (2) chronology
(precise date or age range), (3) size, and (4) subsidence mechanisms and rate. This work presents a hazard assessment from
an alluvial evaporite karst area (0.81 km2) located in the periphery of the city of Zaragoza (Ebro River valley, NE Spain). Five sinkholes and four locations with features
attributable to karstic subsidence where identified in an initial investigation phase providing a preliminary probability
of occurrence of 0.14 sinkholes/km2 year (11.34% in annual probability). A trenching program conducted in a subsequent investigation phase allowed us to rule
out the four probable sinkholes, reducing the probability of occurrence to 0.079 sinkholes/km2 year (6.4% in annual probability). The information on the severity indicates that collapse sinkholes 10–15 m in diameter
may occur in the area. A detailed study of the deposits and deformational structures exposed by trenching in one of the sinkholes
allowed us to infer a modern collapse sinkhole approximately 12 m in diameter and with a vertical throw of 8 m. This collapse
structure is superimposed on a subsidence sinkhole around 80 m across that records at least 1.7 m of synsedimentary subsidence.
Trenching, in combination with dating techniques, is proposed as a useful methodology to elucidate the origin of depressions
with uncertain diagnosis and to gather practical information with predictive utility about particular sinkholes in alluvial
karst settings: precise location, subsidence mechanisms and magnitude, and timing and rate of the subsidence episodes. 相似文献
6.
Rita Borges Radhouan Ben-Hamadou M. Alexandra Chícharo Pedro R Emanuel J. Gonalves 《Estuarine, Coastal and Shelf Science》2007,71(3-4):412-428
There have been no previous studies of the composition of nearshore larval fish assemblages along the coast of Portugal. We aimed to describe the composition and horizontal distribution patterns of larval fish assemblages and their temporal dynamics near a rocky reef at depths shallower than 13 m (inshore) and at two miles (3.70 km) from shore (offshore), as well as along transects perpendicular to the shoreline, from the reef to 10 miles offshore (18.52 km). Samples were taken using 5 min sub-surface trawls at the rocky shore of the Arrábida Marine Park (W Portugal). A total of 1021 larvae were collected, belonging to 61 taxa inshore and to 29 taxa offshore. Along transects, 626 larvae of 52 taxa were collected. Most larvae belonged to coastal species associated with rocky reefs. Total larval abundance and diversity were higher from May to July, which is consistent with the spawning activity of adults. Diversity and total larval abundance decreased significantly with increasing distance from shore, both in the inshore/offshore comparison and in the transects, where this decrease was evident at a very small spatial scale (within the first mile from the reef). Species assemblages differed in the pattern of distribution, with most species clearly associated to the extreme nearshore. The distribution patterns obtained were independent of the spawning mode of species. Results are discussed in the light of the possible physical mechanisms that can potentially act at the Arrábida Marine Park to facilitate larvae retention and the role of larval behaviour. 相似文献
7.
Relationships Between Community Structure of the Intertidal Macroinfauna and Sandy Beach Characteristics Along the Chilean Coast 总被引:2,自引:0,他引:2
Eduardo Jaramillo Heraldo Contreras Cristian Duarte & Pedro Quijón 《Marine Ecology》2001,22(4):323-342
Abstract. Eight sandy beaches were seasonally sampled along the coast of Chile, from ca. 21 to 42° S (about 3000 km) to study the relationship between community structure of the intertidal macroinfauna and beach characteristics. Sediment samples (0.1 m2 , 30 cm deep) were collected (July – September 1998 and December 1998 – January 1999) with plastic cylinders at 15 equally spaced levels along three replicated transects extending from above the drift line to the swash zone. The sediment was sieved through a 1 mm mesh and the organisms collected stored in 5 % formalin. To define beach types, Dean's parameter (Ω) was calculated from wave heights and periods, and fall velocity of sand particles from the swash zone. Crustaceans (mainly peracarids) were the most diverse group with 14 species, followed by polychaetes with 5 species. The talitrid amphipod Orchestoidea tuberculata , the cirolanid isopods Excirolana braziliensis and E. hirsuticauda and the anomuran decapod Emerita analoga were the most widely distributed and common species. Regression analyses between species richness, abundance and biomass of the whole macroinfauna versus sediment characteristics, beach face slopes and morphodynamic beach states showed no significant relationships. Thus, macroinfaunal community characteristics did not increase linearly from lower intermediate to higher intermediate or dissipative beach states as had been found before in Chile or in other coasts. A comparative analysis with data from sandy beaches of other world regions showed that the number of species inhabiting Chilean sandy beaches was generally lower, whereas total population abundances were generally higher compared with values reported elsewhere. 相似文献
8.
We investigate the effect of the temperature–size rule upon zooids of the tropical American bryozoan Cupuladria exfragminis. Results show that mean zooid length, zooid width and zooid area vary significantly between clonal replicates of C. exfragminis kept under different controlled temperature conditions. Significantly larger zooids are produced during times of lowered water temperature that are comparable with the temperatures that occur during seasonal upwelling along the Pacific coast of Panama where the animal lives in abundance. Interpolation of data suggests that a drop of 1 °C causes a 5% increase in zooid size, and that almost all variation in zooid size in natural populations can be explained by temperature. Results are discussed in context of the potential use of zooid size variation in cupuladriid bryozoans to measure the strength of seasonal upwelling in ancient seas by analysing zooid size changes in fossil colonies. The technique of cloning cupuladriid colonies by fragmentation is also discussed with reference to its benefits in experimental studies where genotypes need to be controlled or replicated. 相似文献
9.
10.
A coupled model, consisting of an ocean wave model and an atmospheric general circulation model (AGCM), is integrated under permanent July conditions. The wave model is forced by the AGCM wind stress, whereas the wind waves modify the AGCM surface fluxes of momentum, sensible and latent heat. We investigate the following aspects of the coupled model: how realistic are the wave fields, how strong is the coupling, and how sensitive is the atmospheric circulation to the spatially and temporally varying wave field. The wave climatology of the coupled model compares favorably with observational data. The interaction between the two models is largest (although weak) in the storm track in the Southern Hemisphere. Young windsea, which is associated with enhanced surface fluxes is generated mostly in the equatorward frontal area of an individual cyclone. However, the enhancement of the surface fluxes is too small to significantly modify the climatological mean atmospheric circulation.This paper was presented at the Second International Conference on Modelling of Global Climate Variability, held in Hamburg 7–11 September 1992 under the auspices of the Max Planck Institute for Meteorology. Guest Editor for these papers is L. Dümenil 相似文献