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We have used observations of the rare isotopes of HCN and HNC to determine the relative abundance of these two chemical isomers along the central ridge of the Orion molecular cloud. The abundance ratio [HCN]/[HNC] decreases by more than an order of magnitude from the relatively warm plateau and hot core sources toward the KL nebula to the colder, more quiescent clouds to the north and south. Even in the cooler regions, however, the ratio is an order of magnitude larger than that found in previous investigations of cold dark clouds. We determine the kinetic temperature in the regions we have studied from new observations of methylacetylene (CH3CCH), together with other recent estimates of the gas temperature near KL. The results suggest that the warmer portions of the cloud are dominated by different chemical pathways than those in the general interstellar cloud material. 相似文献
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X射线衍射分析法适宜于分析有机显微组分的芳环层的层状结构。有机质的芳环层结构与其类型和演化程度有关。表征有机质芳环层的层状结构的主要参数:高度Lc、宽度La、网面间距dhk1和芳环层层数可作为油气勘探中判断源岩性质、类型、演化程度与生烃潜力的依据。文章还对参数的变化与意义进行了初步讨论。 相似文献
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Ice-core samples from Upper Fremont Glacier (UFG), Wyoming, were used as proxy records for the chemical composition of atmospheric
deposition. Results of analysis of the ice-core samples for stable isotopes of nitrogen (δ15N, ) and sulfur (δ34S, ), as well as and deposition rates from the late-1940s thru the early-1990s, were used to enhance and extend existing National Atmospheric
Deposition Program/National Trends Network (NADP/NTN) data in western Wyoming. The most enriched δ34S value in the UFG ice-core samples coincided with snow deposited during the 1980 eruption of Mt. St. Helens, Washington.
The remaining δ34S values were similar to the isotopic composition of coal from southern Wyoming. The δ15N values in ice-core samples representing a similar period of snow deposition were negative, ranging from -5.9 to -3.2 ‰ and
all fall within the δ15N values expected from vehicle emissions. Ice-core nitrate and sulfate deposition data reflect the sharply increasing U.S.
emissions data from 1950 to the mid-1970s. 相似文献
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杨家堡含钒石煤的物质成分和钒的赋存状态及配分的研究 总被引:1,自引:0,他引:1
杨家堡下寒武统黑色岩系中,含钒的腐泥煤和次腐泥煤(一般称为含钒石煤)是以钒为主并伴有多种金属元素的大型海相沉积矿床。层位稳定、分布广泛、规模巨大,是一种新型的矿产资源——黑色页岩型多金属矿床。杨家堡含钒石煤中V_2O_5含量达0.7—4.63%,一般品位为0.8—1.0%,完全符合作为独立钒矿床开采的要求。对杨家堡含钒石煤物质成分和钒的赋存状态的研究,是为杨家堡石煤提钒工艺流程的确定提供必要的数据和理论依据,并为黑色页岩型多金属矿床成因理论的研究提供基础资料。 相似文献
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Uncertainty regarding spatial variations of model parameters often results in the simplifying assumption that parameters are spatially uniform. However, spatial variability may be important in resource assessment and model calibration. In this paper, a methodology is presented for estimating a critical basin size, above which base flows appear to be relatively less sensitive to the spatial distribution of recharge and hydraulic conductivity, and below which base flows are relatively more sensitive to this spatial variability. Application of the method is illustrated for a watershed that exhibits distinct infiltration patterns and hydrostratigraphic layering. A ground water flow model (MODFLOW) and a parameter estimation code (UCODE) were used to evaluate the influence of recharge zonation and hydrostratigraphic layering on base flow distribution. Optimization after removing spatial recharge variability from the calibrated model altered base flow simulations up to 53% in watersheds smaller than 40 km(2). Merging six hydrostratigraphic units into one unit with average properties increased base flow residuals up to 83% in basins smaller than 50 km(2). Base flow residuals changed <5% in watersheds larger than 40 and 50 km(2) when recharge and hydrostratigraphy were simplified, respectively; thus, the critical basin size for the example area is approximately 40 to 50 km(2). Once identified for an area, a critical basin size could be used to guide the scale of future investigations. By ensuring that parameter discretization needed to capture base flow distribution is commensurate with the scope of the investigation, uncertainty caused by overextending uniform parameterization or by estimating extra parameter values is reduced. 相似文献