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1.
2.
Summary In-situ microprobe LREE analyses of perovskite and titanite (La, Ce, Nd), and apatite (La, Ce), from SW Ugandan clinopyroxenite xenoliths and kamafugite lavas indicate that LREE distribution in these minerals is determined by a number of factors related to their different parageneses: In particular LREE content is affected by whether the LREE-bearing minerals have crystallised from metasomatic carbonate or from silicate (i.e. metasomatic or magmatic) melts in the mantle. In this situation LREE partition favours carbonate over silicate melts. Distribution of LREE in perovskite and apatite crystallised from magmatic mantle melts or mantle-derived lavas is chiefly determined by preference of LREE for perovskite > apatite > titanite. LREE zoning in perovskite is influenced by changes in melt structure: increasing melt polymerisation enhancing mineralLREE/meltLREE partition into perovskite rims in magmatic xenoliths; decreasing melt polymerisation depleting LREE in lava perovskite rims. This zoning is reinforced by perovskite competition with apatite for LREE: perovskite (cores/rims) co-crystallising with apatite is reduced in LREE. There are 37 instances of perovskitewith Ce below detection while La and Nd levels are normal. These occur in both xenoliths and lavas; in grain zones or whole grains. Likewise Ce alone of the LREE is below detection in six out of ten titanite analyses. These observations are interpreted as evidence for increased fO
2, Ce4 + being excluded from these mineral structures. Recognition of these various processes can elucidate the interpretation of bulk rock and bulk mineral LREE signatures in kamafugite volcanism.
With 3 Figures 相似文献
LREE Verteilung in Perovskit, Apatit und Titanit aus Xenolithen und kamafugitischen Laven Südwest-Ugandas
Zusammenfassung In-situ LREE Analysen von Perovskit und Titanit (La, Ce, Nd) und Apatit (La, Ce) aus Klinopyroxenit-Xenolithen und kamafugitischen Laven Südwest-Ugandas zeigen, daß die LREE Verteilung in diesen Mineralen durch eine Vielzahl von Faktoren, die mit Unterschieden in den Paragenesen zusammenhängen, bestimmt wird: Der LREE-Gehalt wird im besonderen davon bestimmt, ob die LREE-führenden Minerale aus metasomatischen Karbonat- oder aus (metasomatischen oder magmatischen) Silikatschmelzen im Mantel auskristallisierten. Dabei erfolgt die LREE Fraktionierung zu Gunsten der Karbonatschmelzen. Die LREE-Verteilung von Perovskit und Apatit, die aus magmatischen Mantelschmelzen oder -laven kristallisierten, wird vorrangig durch den bevorzugten Einbau der LREE in Perovskit > Apatit > Titanit kontrolliert. Der LREE Zonarbau von Perovskit wird durch die Änderungen der Schmelzstruktur beinflußt: Verstärkte Schmelzpolymerisation führt zu verstärkter MineralLFEE/SchmelzeLREE Fraktionierung in den Perovskiträndern magmatischer Xenolithe, eine Abnahme der Schmelzpolymerisation hingegen resultiert in einer Abreicherung der LREE in den Perovskiträndern. Diese Art der Zonierung wird durch den Wettbewerb von Perovskit mit Apatit um die LREE verstärkt. Perovskit (Kerne/Ränder), der mit Apatit gemeinsam auskristallisierte, ist ärmer an LREE. 37 Fälle, in denenCe nicht nachweisbar war, La und Nd aber in normaler Konzentration auftreten, wurden sowohl in den Xenolithen als auch in den Laven gefunden; und zwar entweder in Kornbereichen oder in ganzen Körnern. Vergleichsweise liegt Ce nur in sechs von zehn Titanitproben unterhalb der Nachweisgrenze. Diese Beobachtungen werden als Hinweise auf erhöhte SauerstoffFugazitäten, bei denen Ce4– aus der Mineralstruktur ausgeschlossen wird, angesehen.Ein Verständnis dieser verschiedenen Prozesse kann zur besseren Interpretation von LREE Gesamtgesteins- und Gesamtmineral-Signaturen in Kamafugiten beitragen.
With 3 Figures 相似文献
3.
Maowen Li Yongqiang Xiong Lloyd R. Snowdon Dale Issler 《Journal of Geochemical Exploration》2006,89(1-3):214
Molecular and isotopic compositions of crude oils in the Beaufort–Mackenzie Basin confirm three genetic end-member oil groups and suggest extensive cross-formational hydrocarbon fluid flows in the Tertiary deltaic system. Inter- and intra-fractional variations in the geochemistry of the Tertiary-reservoired oils indicate that the oil source/maturity signatures were substantially masked by biomarkers that were picked up along migration pathways. Thus, many of the previously recognized “immature non-marine oils” are in fact thermally mature, probably derived from unpenetrated deeper marine source rocks. Although the effective source rock volumes have not been evaluated and their exact stratigraphic levels remain unknown, the relative timing of oil generation versus trap formation, rather than poor source quality, may be the cause of under-filled traps in the offshore area. 相似文献
4.
This paper describes an extension to the Combined Hydrology And Stability Model (CHASM) to fully include the effects of vegetation and slope plan topography on slope stability. The resultant physically based numerical model is designed to be applied to site‐specific slopes in which a detailed assessment of unsaturated and saturated hydrology is required in relation to vegetation, topography and slope stability. Applications are made to the Hawke's Bay region in New Zealand where shallow‐seated instability is strongly associated with spatial and temporal trends in vegetation cover types, and the Mid‐Levels region in Hong Kong, an area subject to a variety of landslide mechanisms, some of which may be subject to strong topographic control. An improved understanding of process mechanism, afforded by the model, is critical for reliable and appropriate design of slope stabilization and remedial measures. Copyright © 2002 John Wiley & Sons, Ltd. 相似文献
5.
Dauphiné twinning and texture memory in polycrystalline quartz. Part 3: texture memory during phase transformation 总被引:1,自引:0,他引:1
Hans-Rudolf?WenkEmail author N.?Barton M.?Bortolotti S.?C.?Vogel M.?Voltolini G.?E.?Lloyd G.?B.?Gonzalez 《Physics and Chemistry of Minerals》2009,36(10):567-583
Samples of quartz-bearing rocks were heated above the α (trigonal)–β (hexagonal) phase transformation of quartz (625–950°C)
to explore changes in preferred orientation patterns. Textures were measured both in situ and ex situ with neutron, synchrotron
X-ray and electron backscatter diffraction. The trigonal–hexagonal phase transformation does not change the orientation of
c- and a-axes, but positive and negative rhombs become equal in the hexagonal β-phase. In naturally deformed quartzites measured by
neutron diffraction a perfect texture memory was observed, i.e. crystals returned to the same trigonal orientation they started
from, with no evidence of twin boundaries. Samples measured by electron back-scattered diffraction on surfaces show considerable
twinning and memory loss after the phase transformation. In experimentally deformed quartz rocks, where twinning was induced
mechanically before heating, the orientation memory is lost. A mechanical model can explain the memory loss but so far it
does not account for the persistence of the memory in quartzites. Stresses imposed by neighboring grains remain a likely cause
of texture memory in this mineral with a very high elastic anisotropy. If stresses are imposed experimentally the internal
stresses are released during the phase transformation and the material returns to its original state prior to deformation.
Similarly, on surfaces there are no tractions and thus texture memory is partially lost. 相似文献
6.
K. Perner M. Moros J.M. Lloyd A. Kuijpers R.J. Telford J. Harff 《Quaternary Science Reviews》2011,30(19-20):2815-2826
A new centennial scale benthic foraminiferal record of late Holocene climate variability and oceanographic changes off West Greenland (Disko Bugt) highlights substantial subsurface water mass changes (e.g. temperature and salinity) of the West Greenland Current (WGC) over the past 3.6 ka BP. Benthic foraminifera reveal a long-term late Holocene cooling trend, which may be attributed to increased advection of cold, low-salinity water masses derived from the East Greenland Current (EGC). Cooling becomes most pronounced from c. 1.7 ka BP onwards. At this point the calcareous Atlantic benthic foraminiferal fauna decrease significantly and is replaced by an agglutinated Arctic fauna. Superimposed on this cooling trend, centennial scale variability in the WGC reveals a marked cold phase at c. 2.5 ka BP, which may correspond to the 2.7 ka BP cooling-event recorded in marine and terrestrial archives elsewhere in the North Atlantic region. A warm phase recognized at c. 1.8 ka BP is likely to correspond to the ‘Roman Warm Period’ and represents the warmest bottom water conditions. During the time period of the ‘Medieval Climate Anomaly’ we observe only a slight warming of the WGC. A progressively more dominant cold water contribution from the EGC on the WGC is documented by the prominent rise in abundance of agglutinated Arctic water species from 0.9 ka BP onwards. This cooling event culminates at c. 0.3 ka BP and represents the coldest episode of the ‘Little Ice Age’.Gradually increased influence of cold, low-salinity water masses derived from the EGC may be linked to enhanced advection of Polar and Arctic water by the EGC. These changes are possibly associated with a reported shift in the large-scale North Atlantic Oscillation atmospheric circulation pattern towards a more frequent negative North Atlantic Oscillation mode during the late Holocene. 相似文献
7.
8.
Accurate water level forecasts are essential for flood warning. This study adopts a data‐driven approach based on the adaptive network–based fuzzy inference system (ANFIS) to forecast the daily water levels of the Lower Mekong River at Pakse, Lao People's Democratic Republic. ANFIS is a hybrid system combining fuzzy inference system and artificial neural networks. Five ANFIS models were developed to provide water level forecasts from 1 to 5 days ahead, respectively. The results show that although ANFIS forecasts of water levels up to three lead days satisfied the benchmark, four‐ and five‐lead‐day forecasts were only slightly better in performance compared with the currently adopted operational model. This limitation is imposed by the auto‐ and cross‐correlations of the water level time series. Output updating procedures based on the autoregressive (AR) and recursive AR (RAR) models were used to enhance ANFIS model outputs. The RAR model performed better than the AR model. In addition, a partial recursive procedure that reduced the number of recursive steps when applying the AR or the RAR model for multi‐step‐ahead error prediction was superior to the fully recursive procedure. The RAR‐based partial recursive updating procedure significantly improved three‐, four‐ and five‐lead‐day forecasts. Our study further shows that for long lead times, ANFIS model errors are dominated by lag time errors. Although the ANFIS model with the RAR‐based partial recursive updating procedure provided the best results, this method was able to reduce the lag time errors significantly for the falling limbs only. Improvements for the rising limbs were modest. Copyright © 2011 John Wiley & Sons, Ltd. 相似文献
9.
Origin of glass in upper mantle xenoliths from the quaternary volcanics of Gees,West Eifel,Germany 总被引:6,自引:0,他引:6
A. D. Edgar F. E. Lloyd D. M. Forsyth R. L. Barnett 《Contributions to Mineralogy and Petrology》1989,103(3):277-286
Glasses have been analysed from six mantle-derived xenoliths (5 orthopyroxene and/or olivine-rich, 1 clinopyroxene-rich) from the Quaternary volcanics S.E. of Gees, West Eifel, Germany. The glasses in these xenoliths occur as pools surrounding and embaying spinels, as inclusions in spinels, as veins and stringers within phlogopiterich veins, and as jackets partially surrounding some of the xenoliths. Glasses analysed are felsic and characterised by low to intermediate SiO2 (40–62 wt.%), variable CaO (1–11 wt.%) and MgO (1–4 wt.%), high Al2O3 (14–21 wt.%), and up to 11 wt.% Na2O + K2O. The jacket glasses have the lowest SiO2, highest CaO and MgO. Variations in all of the glass compositions are similar and imply a unifying factor or process in their formation. Glass as pools and stringers within veins of phlogopite forms part of the same trends shown by all the glasses when plotted on bivariate (oxide vs SiO2) diagrams but can be distinguished from glass surrounding and enclosed by spinels. Glasses occurring as jackets are similar in composition to those in pools and veinlets associated with phlogopite but are of quite different composition to the glasses found within the xenoliths that they partially enclose. The occurrence and chemistry of the glasses do not support such glasses as representing original or differentiated magma trapped during formation of the xenolithic assemblages. The chemistry of the glasses also makes it unlikely that they were produced by dissociation of phlogopite during ascent of the xenoliths. The most likely origin for the glasses is that they represent volatile-rich melts which migrated through upper mantle material. These melts are likely to be responsible for the heterogeneous nature of the mantle underlying this part of the West Eifel region. 相似文献
10.
E. H. Lloyd D. Warren 《Stochastic Environmental Research and Risk Assessment (SERRA)》1988,2(3):175-188
It was remarked by Hurst in 1951 that the adjusted range gives the size of the smallest reservoir capable of providing a constant discharge equal to the mean inflow. Since that time this range and its rescaled modification, the Hurst range, have been widely discussed, not however primarily with a view to applying them to reservoir design problems, but rather on account of their possible relevance to the simulation of geophysical time series.Acknowledging the well-known conceptual weaknesses of adjusted ranges and the theoretical difficulties that inhibit their direct utilisation in the design and operation of real reservoirs, the authors argue that the interest displayed on ranges during the past few decades justifies the effort of eliminating one in particular of these weakness, namely their non-implementability as operating policies, a consequence of the fact that they can only be retrospectively evaluated. The paper proposes modifications in which the unknowable mean and standard deviation of future samples are replaced by the known mean and sample standard deviation of historical data, leading to the historically adjusted range and the historically rescaled and adjusted range. The latter is produced as an implementable approximation to Hurst's (1951) solution to the optimal reservoir problem.The expected values of the new ranges are evaluated and numerically tabulated. 相似文献