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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff
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We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
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Photometric observations of Pluto in the BVR filter system were obtained in 1999 and in 1990-1993, and observations in the 0.89-μm methane absorption band were obtained in 2000. Our 1999 observations yield lightcurve amplitudes of 0.30 ± 0.01, 0.26 ± 0.01, and 0.21 ± 0.02 and geometric albedos of 0.44 ± 0.04, 0.52 ± 0.03, and 0.58 ± 0.02 in the B, V, and R filters, respectively. The low-albedo hemisphere of Pluto is slightly redder than the higher albedo hemisphere. A comparison of our results and those from previous epochs shows that the lightcurve of Pluto changes substantially through time. We developed a model that fully accounts for changes in the lightcurve caused by changes in the viewing geometry between the Earth, Pluto, and the Sun. We find that the observed changes in the amplitude of Pluto’s lightcurve can be explained by viewing geometry rather than by volatile transport. We also discovered a measurable decrease since 1992 of ∼0.03 magnitudes in the amplitude of Pluto’s lightcurve, as the model predicts. Pluto’s geometric albedo does not appear to be currently increasing, as our model predicts, although given the uncertainties in both the model and the measurements of geometric albedo, this result is not firm evidence for volatile transport. The maximum of methane-absorption lightcurve occurs near the minimum of the BVR lightcurves. This result suggests that methane is more abundant in the brightest regions of Pluto. Pluto’s phase coefficient exhibits a color dependence, ranging from 0.037 ± 0.01 in the B filter to 0.032 ± 0.01 in the R filter. Pluto’s phase curve is most like those of the bright, recently resurfaced satellites Triton and Europa. Although Pluto shows no strong evidence for volatile transport now (unlike Triton), it is important to continue to observe Pluto as it moves away from perihelion. 相似文献
4.
采用表征岩体渗透性的单位吸水量ω为参数,有效地分析了砂泥岩裂隙岩体中相对埋深和岩性对渗透性空间分布规律的影响.研究区内,在不同深度单位吸水量的最大值和最小值相差3-4个数量级,渗透性表现出显著的随机特征.通过将压水试验数据离散化并在不同深度上取logω的平均值,凸现了渗透性的结构特征.ω均值在一定范围内随相对深度表现出负指数分布规律;剔除logω的线性趋势项后,logω残差表现出与地层内部岩性相对应的规律.此外,研究还发现,渗透性参数随相对深度呈负指数分布规律是由含裂隙的砂岩介质引起的.这些规律为裂隙岩体的渗流计算和模拟奠定了基础.文章所提出的对压水试验数据离散化并在不同深度取均值以找出渗透性和深度关系,以及去除线性趋势项研究渗透性和岩性之间关系等方法具有广泛的应用价值. 相似文献
5.
An iterative inverse method, the sequential self-calibration method, is developed for mapping spatial distribution of a hydraulic
conductivity field by conditioning on nonreactive tracer breakthrough curves. A streamline-based, semi-analytical simulator
is adopted to simulate solute transport in a heterogeneous aquifer. The simulation is used as the forward modeling step. In
this study, the hydraulic conductivity is assumed to be a deterministic or random variable. Within the framework of the streamline-based
simulator, the efficient semi-analytical method is used to calculate sensitivity coefficients of the solute concentration
with respect to the hydraulic conductivity variation. The calculated sensitivities account for spatial correlations between
the solute concentration and parameters. The performance of the inverse method is assessed by two synthetic tracer tests conducted
in an aquifer with a distinct spatial pattern of heterogeneity. The study results indicate that the developed iterative inverse
method is able to identify and reproduce the large-scale heterogeneity pattern of the aquifer given appropriate observation
wells in these synthetic cases. 相似文献
6.
D. F. Falla L. M. Bartlett M. H. L. Smith R. R. Hillier 《Astrophysics and Space Science》1994,211(1):115-126
The RS CVn binary stellar system HR 1099 is a source of both X-ray and radio flares. We present here a model of the system in which the two types of flare are produced by the same population of mildly-relativistic ( 10) electrons, injected into a coronal loop. After reviewing possible radiation mechanisms we conclude that, given the probable conditions in the flaring region, the radio emission is gyrosynchrotron radiation and the X-ray emission is thermal bremsstrahlung. The thermal X-ray source must lie in the stellar chromosphere, but the apparent absence of plasma absorption at radio frequencies indicates that the radio source is located high in the coronal loop. Using the relationships given by Dulk and Marsh (1982) for the radio emission from a power-law electron energy spectrum,N() ( - 1)–, we conclude that 3 7, with 30% of the electron population trapped in the radio source. Some implications of these results for one particular version of the model are discussed. 相似文献
7.
Tony T. Gregg Amanda Dewees Drema Gross Bill Hoffman Dan Strub Matt Watson 《中国海洋大学学报(英文版)》2006,5(4):375-380
1Water LossInitiativesUnaccounted-for water(or unbilled water)has beenreceiving newscrutiny at both the state and nationallevels.For years,water conservationeffortsin Europehave emphasized reduction in water loss to a muchgreater extent thaninthe United S… 相似文献
8.
R. G. Bill Jr. R. A. Sutherland J. F. Bartholic E. Chen 《Boundary-Layer Meteorology》1978,14(4):543-556
Moderating effects of Lake Apopka, Florida on downwind surface temperatures were evaluated under cold-air advective conditions. Point temperature measurements north and south of the lake and data obtained from a thermal scanner flown at 1.6 km indicate that surface temperatures directly downwind may be higher than surrounding surface temperatures by as much as 5 °C under conditions of moderate winds (~4 m s–1). No substantial temperature effects were observed with surface wind speed less than 1 m s–1. Fluxes of sensible and latent heat from Lake Apopka were calculated from measurements of lake temperature, net radiation, relative humidity and air temperature above the lake. Bulk transfer coefficients and the Bowen ratio were calculated and found to be in agreement with reported data for non-advective conditions.IFAS Journal Series No. 1006. 相似文献
9.
Evaluation and Monitoring of Service Quality: Discussing Ways to Meet INSPIRE Requirements
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Service oriented architectures (SOA) are widely used nowadays. As the name implies such architectures rely on services. Germany developed a marine‐specific service oriented data infrastructure (MDI‐DE – Marine Dateninfrastruktur Deutschland) from 2010 to 2013. The services in MDI‐DE can contribute to fulfilling reporting commitments for various European and national legislation. The services of MDI‐DE (just like other services affected, for instance, by INSPIRE) have to meet specific requirements regarding performance, availability and conformity (quality of service, QoS). Although SOA is an important field in scientific research there are very few publications and studies available on QoS, especially regarding INSPIRE requirements. The services of MDI‐DE were analyzed using various existing tools. Their usefulness to reflect where either the aspect's performance, availability or conformity needs improvement was partly verified. Due to varying results and the neglect of some services for various reasons it can be stated that the more tools are used, the more conclusive the outcome. Furthermore, service quality was not coherent when measured with different tools. This means that measuring QoS in terms of INSPIRE will be very difficult to do in the future and there is the danger that people will choose the tools with which their services perform best. 相似文献
10.