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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff
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We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
The Meseta de Somuncura forms the largest basaltic plateau (20 000 km2 ) of southern Argentina (extra-Andean domain). Most of these tholeiitic to alkaline rocks were extruded at ˜ 25 Ma (late Oligocene). The absence of rifting–thinning processes, plume activity, or slab-window phenomena leaves only one major possibility for the generation of Somuncura: asthenospheric ('OIB-like') corner flow leading to a transient thermal anomaly above the subducting plate. It is suggested herein that the intake of hot asthenosphere was forced into a favourable topography (concave-up) of the subducting plate, when a major plate reorganization event (Farallon to Nazca) was taking place in late Oligocene to early Miocene time. The fast and vigorous intake of asthenosphere would have been induced by slab roll-back, leading to decoupling of the subducting plate. The Somuncura volcanic episode can be regarded as a marker of the passage from the extremely oblique subduction of Farallon, to the birth of the Nazca plate and roughly perpendicular convergence between South America and Nazca. 相似文献
3.
Daniela Lazzaro Marcos A. Florczak Alberto Betzler Othon C. Winter Silvia M. Giuliatti-Winter Claudia A. Angeli Dietmar W. Foryta 《Planetary and Space Science》1996,44(12):1547-1550
The results of photometric observations of comet/asteroid 2060 Chiron at the Observatório do Pico dos Dias (Brazil-OPD) and the Observatoire de Haute-Provence (France-OHP) during 1994 and 1995 are presented. The analysis of the data shows a decrease of 2060 Chiron brightness from its peak values of 1988–1991. The absolute magnitude, Hv, varies from a maximum of 6.6 in February 1994 up to a minimum of 6.8 in June 1995. Therefore 2060 Chiron is back to a minimum of activity close to that of 1983–1985. The slope parameter G is found to be G = 0.71 ± 0.15. It is suggested that the H-G magnitude system, generally adopted to present 2060 Chiron brightness, is not the most appropriate due to the cometary activity of this object. 相似文献
4.
5.
E.A. Evstigneeva R.R. de Carvalho A.L. Ribeiro H.V. Capelato 《Astrophysics and Space Science》2003,284(2):487-490
We present the preliminary results of a study of how small stellar systems merge to form larger ones. As we display the families
of galaxies in the μe - Re plane (effective surface brightness versus effective radius) we realize that different morphological types occupy different
loci, evidencing the different physical mechanisms operating in each family. As proposed by Capaccioli et al. (1992) this
diagram is the logical equivalent of the HR diagram for stars. Here we take some initial steps in understanding of how we
can establish the evolutionary tracks, solely due to dynamical processes, in the μe - Re plane, ultimately making a dwarf elliptical to turn into a normal elliptical galaxy.
This revised version was published online in August 2006 with corrections to the Cover Date. 相似文献
6.
Roberto Mínguez Fernando Delgado Ignacio Escuder Manuel G. de Membrillera 《国际地质力学数值与分析法杂志》2006,30(10):1019-1037
Empirical criteria have been used successfully to design filters of most embankment large dam projects throughout the world. However, these empirical rules are only applicable to a particular range of soils tested in laboratory and do not take into account the variability of the base material and filter particle sizes. In addition, it is widely accepted that the safety of fill dams is mainly dependent on the reliability of their filter performance. The work herein presented consists in a new general method for assessing the probability of fulfilling any empirical filter design criteria accounting for base and filter heterogeneity by means of first‐order reliability methods (FORM), so that reliability indexes and probabilities of fulfilling any particular criteria are obtained. This method will allow engineers to estimate the safety of existing filters in terms of probability of fulfilling their design criteria and might also be used as a decision tool on sampling needs and material size tolerances during construction. In addition, sensitivity analysis makes possible to analyse how reliabilities are influenced by different sources of input data. Finally, in case of a portfolio risk assessment, this method will allow engineers to compare the safety of several existing dams in order to prioritize safety investments and it is expected to be a very useful tool to evaluate probabilities of failure due to internal erosion. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
7.
Alberto Etchegoyen 《Astrophysics and Space Science》2004,290(3-4):379-387
The Auger Project studies the highest energies known in nature with an emphasis on energies ≥5 × 1019 eV, which are cosmic rays coming from the outer space reaching the Earth's surface with a very low flux. The questions to be elucidated are what are the origin, energy, production mechanism, and chemical composition of these cosmic rays. Auger aims at building two observatories in both the hemispheres and in 2000 the construction of the austral observatory started. Auger's two distinctive features are its exceptional size and its hybrid nature. It spans over an area of 3000 km2 and is constituted by 24 fluorescence detector telescopes and 1600 surface detectors. As such, it will provide a large number of events with less systematic detection uncertainties. The construction of the Southern Observatory in Argentina is quite advanced and the buildings at the Central Station in Malargüe city are already operational. So are the telescope buildings at Cerros Los Leones and Coihueco (two prototype telescopes were operational at Los Leones, which have now been dismantled), 32 surface detectors, and the telecommunication and data acquisition systems. About 20-hybrid events/months were detected and currently two events/hours are registered with the surface detector array. The detection of hybrid events is the most important issue since it shows that the equipment operates within the design parameters. 相似文献
8.
Irina N Belskaya Vasilij G Shevchenko Yurij N Krugly Yurij S Efimov Alberto Cellino 《Icarus》2003,166(2):276-284
The first results of the observational program devoted to simultaneous investigation of asteroid polarimetric and photometric opposition phenomena are presented. UBVRI polarimetric and V-band photometric observations of the S-type Asteroid 20 Massalia and the E-type Asteroids 214 Aschera and 620 Drakonia were carried out in 1996-1999 down to phase angles of 0.08°, 0.7°, and 1.2°, correspondingly. The S-type Asteroid 20 Massalia is characterized by the pronounced brightness opposition surge with an amplitude larger than that observed for the E-type asteroids. A sharp peak of negative polarization at small phase angles was not observed for this asteroid. The value of polarization degree at phase angle α<1° is less than 0.5% for both S and E types. The negative polarization branches of S and especially E-asteroids have an asymmetrical shape. The phase angle at which the polarization minimum occurs is close to the angle at which non-linear increase begins in the asteroid magnitude phase curves. A relation of the observed effects to the mechanism of coherent backscattering is discussed. 相似文献
9.
C.S. Botzler J. Snigula R. Bender N. Drory G. Feulner G.J. Hill U. Hopp C. Maraston C. Mendes de Oliveira 《Astrophysics and Space Science》2003,284(2):393-396
The Munich Near-IR Cluster Survey (MUNICS) is a wide-area, medium-deep, photometric survey selected in the K' band. The project's
main scientific aims are the identification of galaxy clusters up to redshifts of unity and the selection of a large sample
of field early-type galaxies up to z < 1.5 for evolutionary studies. We created a Large Scale Structure catalog, using a new structure finding technique specialized
for photometric datasets, that we developed on the basis of a friends-of-friends algorithm. We tested the plausibility of
the resulting galaxy group and cluster catalog with the help of Color-Magnitude Diagrams (CMD), as well as a likelihood- and
Voronoi-approach.
This revised version was published online in August 2006 with corrections to the Cover Date. 相似文献
10.
Andrew Mennim Richard A. Battye Carsten van de Bruck 《Astrophysics and Space Science》2003,283(4):633-638
We discuss the problems faced in trying to deduce the evolution of cosmological perturbations in brane-world models. There
are two natural ways to formulate the problem: one which makes the equations of motion simple and the other which makes the
boundary condition simple. Unfortunately the problem is difficult to solve, even numerically, in either formalism. We present
a more phenomenological approach which, while it does not solve the problem for any given model, illustrates some generic
features one might expect to see in the tensor part of the cosmic microwave background power spectrum. We find that the observed
scale invariance of the cosmic microwave background provides bounds on brane world models.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献