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1.
Bruno Lanson Matthew A. Marcus Sirine Fakra Frdric Panfili Nicolas Geoffroy Alain Manceau 《Geochimica et cosmochimica acta》2008,72(10):2478-2490
It is now well established that a number of terrestrial and aquatic microorganisms have the capacity to oxidize and precipitate Mn as phyllomanganate. However, this biomineralization has never been shown to occur in plant tissues, nor has the structure of a natural Mn(IV) biooxide been characterized in detail. We show that the graminaceous plant Festuca rubra (red fescue) produces a Zn-rich phyllomanganate with constant Zn:Mn and Ca:Mn atomic ratios (0.46 and 0.38, respectively) when grown on a contaminated sediment. This new phase is so far the Zn-richest manganate known to form in nature (chalcophanite has a Zn:Mn ratio of 0.33) and has no synthetic equivalent. Visual examination of root fragments under a microscope shows black precipitates about ten to several tens of microns in size, and their imaging with backscattered and secondary electrons demonstrates that they are located in the root epidermis. In situ measurements by Mn and Zn K-edge extended X-ray absorption fine structure (EXAFS) spectroscopy and X-ray diffraction (XRD) with a micro-focused beam can be quantitatively described by a single-phase model consisting of Mn(IV) octahedral layers with 22% vacant sites capped with tetrahedral and octahedral Zn in proportions of 3:1. The layer charge deficit is also partly balanced by interlayer Mn and Ca. Diffracting crystallites have a domain radius of 33 Å in the ab plane and contain only 1.2 layers (8.6 Å) on average. Since this biogenic Mn oxide consists mostly of isolated layers, basal 00l reflections are essentially absent despite its lamellar structure. Individual Mn layers are probably held together in the Mn–Zn precipitates by stabilizing organic molecules. Zinc biomineralization by plants likely is a defense mechanism against toxicity induced by excess concentrations of this metal in the rhizosphere. 相似文献
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The dynamics and thermodynamics of large ash flows 总被引:6,自引:6,他引:0
Ash flow deposits, containing up to 1000 km3 of material, have been produced by some of the largest volcanic eruptions known. Ash flows propagate several tens of kilometres
from their source vents, produce extensive blankets of ash and are able to surmount topographic barriers hundreds of metres
high. We present and test a new model of the motion of such flows as they propagate over a near horizontal surface from a
collapsing fountain above a volcanic vent. The model predicts that for a given eruption rate, either a slow (10–100 m/s) and
deep (1000–3000 m) subcritical flow or a fast (100–200 m/s) and shallow (500–1000 m) supercritical flow may develop. Subcritical
ash flows propagate with a nearly constant volume flux, whereas supercritical flows entrain air and become progressively more
voluminous. The run-out distance of such ash flows is controlled largely by the mass of air mixed into the collapsing fountain,
the degree of fragmentation and the associated rate of loss of material into an underlying concentrated depositional system,
and the mass eruption rate. However, in supercritical flows, the continued entrainment of air exerts a further important control
on the flow evolution. Model predictions show that the run-out distance decreases with the mass of air entrained into the
flow. Also, the mass of ash which may ascend from the flow into a buoyant coignimbrite cloud increases as more air is entrained
into the flow. As a result, supercritical ash flows typically have shorter runout distances and more ash is elutriated into
the associated coignimbrite eruption columns. We also show that one-dimensional, channellized ash flows typically propagate
further than their radially spreading counterparts.
As a Plinian eruption proceeds, the erupted mass flux often increases, leading to column collapse and the formation of pumiceous
ash flows. Near the critical conditions for eruption column collapse, the flows are shed from high fountains which entrain
large quantities of air per unit mass. Our model suggests that this will lead to relatively short ash flows with much of the
erupted material being elutriated into the coignimbrite column. However, if the mass flux subseqently increases, then less
air per unit mass is entrained into the collapsing fountain, and progressively larger flows, which propagate further from
the vent, will develop.
Our model is consistent with observations of a number of pyroclastic flow deposits, including the 1912 eruption of Katmai
and the 1991 eruption of Pinatubo. The model suggests that many extensive flow sheets were emplaced from eruptions with mass
fluxes of 109–1010 kg/s over periods of 103–105 s, and that some indicators of flow "mobility" may need to be reinterpreted. Furthermore, in accordance with observations,
the model predicts that the coignimbrite eruption columns produced from such ash flows rose between 20 and 40 km.
Received: 25 August 1995 / Accepted: 3 April 1996 相似文献
4.
Remote observations of the lunar radiowave emission are reexamined in the light of physical property data accumulated through the Apollo program. It is found that thermal and electrical properties determined for a number of different landing sites yield theoretical results in good agreement with remote observations for millimeter and short centimeter wavelengths. Theoretical models incorporating reflecting layers of rock and physical property data from the Apollo program are compared to the longer wavelength (5–500 cm) observational data to estimate a disk average steady state heat flow and a mean depth of the lunar regolith. It is found that a high heat flow, comparable to the heat flows measured at the Apollo 15 and 17 sites, is required to fit the available 5–20 cm wavelength remote data, and that a lunar surface layer relatively free of large boulders within the upper 10–30 m best fits the observations of a decreasing brightness temperature with wavelength for wavelengths greater than ~ 50 cm. 相似文献
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W. Andrew Marcus Carl J. Legleiter Richard J. Aspinall Joseph W. Boardman Robert L. Crabtree 《Geomorphology》2003,55(1-4):363
This article evaluates the potential of 1-m resolution, 128-band hyperspectral imagery for mapping in-stream habitats, depths, and woody debris in third- to fifth-order streams in the northern Yellowstone region. Maximum likelihood supervised classification using principal component images provided overall classification accuracies for in-stream habitats (glides, riffles, pools, and eddy drop zones) ranging from 69% for third-order streams to 86% for fifth-order streams. This scale dependency of classification accuracy was probably driven by the greater proportion of transitional boundary areas in the smaller streams. Multiple regressions of measured depths (y) versus principal component scores (x1, x2,…, xn) generated R2 values ranging from 67% for high-gradient riffles to 99% for glides in a fifth-order reach. R2 values were lower in third-order reaches, ranging from 28% for runs and glides to 94% for pools. The less accurate depth estimates obtained for smaller streams probably resulted from the relative increase in the number of mixed pixels, where a wide range of depths and surface turbulence occurred within a single pixel. Matched filter (MF) mapping of woody debris generated overall accuracies of 83% in the fifth-order Lamar River. Accuracy figures for the in-stream habitat and wood mapping may have been misleadingly low because the fine-resolution imagery captured fine-scale variations not mapped by field teams, which in turn generated false “misclassifications” when the image and field maps were compared.The use of high spatial resolution hyperspectral (HSRH) imagery for stream mapping is limited by the need for clear water to measure depth, by any tree cover obscuring the stream, and by the limited availability of airborne hyperspectral sensors. Nonetheless, the high accuracies achieved in northern Yellowstone streams indicate that HSRH imagery can be a powerful tool for watershed-wide mapping, monitoring, and modeling of streams. 相似文献
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9.
Marcus Schulz Jan Priegnitz Jörg Klasmeier Stefan Heller Stefan Meinecke Michael Feibicke 《水文研究》2012,26(2):272-280
In several empirical and modelling studies on river hydraulics, dispersion was negatively correlated to surface roughness. In this study, it was aimed to investigate the influence of surface roughness on longitudinal dispersion under controlled conditions. In artificial flow channels with a length of 104 m, tracer experiments with variations in channel bed material were performed. By use of measured tracer breakthrough curves, average flow velocity, mean longitudinal dispersion, and mean longitudinal dispersivity were calculated. Longitudinal dispersion coefficients ranged from 0·018 m2 s?1 in channels with smooth bed surface up to 0·209 m2 s?1 in channels with coarse gravel as bed material. Longitudinal dispersion was linearly related to mean flow velocity. Accordingly, longitudinal dispersivities ranged between 0·152 ± 0·017 m in channels with smooth bed surface and 0·584 ± 0·015 m in identical channels with a coarse gravel substrate. Grain size and surface roughness of the channel bed were found to correlate positively to longitudinal dispersion. This finding contradicts several existing relations between surface roughness and dispersion. Future studies should include further variation in surface roughness to derive a better‐founded empirical equation forecasting longitudinal dispersion from surface roughness. Copyright © 2011 John Wiley & Sons, Ltd. 相似文献
10.
Venkatarathnam Kolla Lawrence Sullivan S.Stephen Streeter Marcus G. Langseth 《Marine Geology》1976,21(3):171-189
Data on bottom-water potential temperature, turbidity and current indications show that in the Southern Ocean west of the Kerguelen Plateau, Antarctic Bottom Water (AABW) of Weddell Sea origin spreads northwards from the Atlantic—Indian Basin in two directions: (1) AABW enters the Agulhas Basin through relatively deep areas in the Mid-Indian Ridge at 20–25°E and possibly at 35°E, and flows northwards into the Mozambique Basin as far as its northern limits; (2) a more easterly spreading path extends from the Atlantic—Indian Basin through the Crozet into the Madagascar, Mascarene, Somali and Arabian Basins. The passage in the western branch of the Indian Ridge for the AABW spreading from the Crozet into the Madagascar Basin appears to be at 29-26°S and 60–64°E.East of the Kerguelen Plateau in the South Indian Basin, the bottom water formed mainly along the Adélie Coast and Ross Sea travels west towards the Kerguelen Plateau and then parallel to it. This water finally flows eastwards hugging the Southeast Indian Ridge. Significant deviations from this general circulation pattern occur due to local topographic effects. Some AABW in the South Indian Basin exits through a passage at 120–125°E in the region of the Australian—Antarctic discordance in the Southeast Indian Ridge and enters the South Australian Basin and subsequently the Wharton Basin. This passage is clearly indicated by the northward extension of a cold, bottom-water tongue as shown by the temperature distribution in the region; the bottom-water effects in the passage are reflected in the high turbidity and current lineations on the sea floor.In the Southern Ocean basins, bottom-water turbidity is generally high, reflecting in part the strong bottom-water activity. The effects of AABW circulation on the sea floor—in the form of well-developed small- or large-scale current ripples and erosional/depositional features, manganese-nodule formations, and unconformities and reworking of sediments observed in cores — are also marked in these basins. Even though the AABW in the Wharton Basin is cold, its spreading effects on the sea floor are minimal in this basin in contrast to the basins west of the Mid-Indian Ridge at comparable latitudes. 相似文献