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1.
Mineralogical sources of the buffer capacity in a granite catchment determined by strontium isotopes
Christina Weyer Gunnar Lischeid Luc Aquilina Anne-Catherine Pierson-Wickmann Charlotte Martin 《Applied Geochemistry》2008
The role of different minerals in base cation release and thus the increase of buffering capacity of groundwater against acid deposition is controversially discussed in the literature. The 87Sr/86Sr ratios and base cation concentration were investigated in whole rock leachates, mineral separates, precipitation, soil solution, groundwater and stream water samples in the Lehstenbach catchment (Germany) to identify the weathering sequence of the granite bedrock. Three different approaches were followed in parallel. It was assumed that the contribution of different minerals to base cation supply of the groundwater with increasing weathering intensity would be observed by investigating (1) unweathered rock leachates, deep groundwater and shallow groundwater, (2) groundwater samples from new groundwater wells, reflecting the initial weathering of the drilled bedrock, and groundwater from wells that were drilled in 1988, (3) stream water during baseflow, dominated by deep groundwater, and stream water during high flow, being predominantly shallow groundwater. Whereas the first approach yielded consistent patterns, there was some evidence that groundwater from the new wells initially reflected contamination by the filter gravel rather than cation release in an initial stage of weathering. Time series samples of stream water and groundwater solute concentrations and isotope ratios turned out to reflect varying fractions of soil water and precipitation water at baseflow and high flow conditions rather than varying contributions of different minerals that prevail at different stages of granite weathering. 相似文献
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A two-layered model is considered in which the upper layer is continuously stratified and the lower layer is homogeneous. The system is driven by atmospheric forces. Bottom stress and topography are included in the model. The linear three-dimensional hydrodynamical equations are used to describe the system. Taking the eddy viscosity in the upper layer as inversely proportional to the static stability, the dependent variables are expanded in terms of continuous functions in the vertical (eigenfunctions). Using this method it is possible to compute currents and internal displacements at any depth in the upper layer. The three-dimensional structure of the lower layer is not considered in this model. The equations describing the lower layer are integrated over depth to give depth mean currents. Using a staggered finite-difference grid in the horizontal and a forward time-stepping procedure, numerical test experiments are carried out for a cross section and for a closed rectangular basin. 相似文献
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Geochemistry and mineralogy of shallow alluvial aquifers in Daudkandi upazila in the Meghna flood plain, Bangladesh 总被引:1,自引:0,他引:1
M. Aziz Hasan Mattias von Br?mssen Prosun Bhattacharya Kazi Matin Ahmed Arif Mohiuddin Sikder Gunnar Jacks Ondra Sracek 《Environmental Geology》2009,57(3):499-511
The shallow alluvial aquifers of the delta plains and flood plains of Bangladesh, comprises about 70% of total land area are
mostly affected by elevated concentrations of arsenic (As) in groundwater exposing a population of more than 35 million to
As toxicity. Geochemical studies of shallow alluvial aquifer in the Meghna flood plain show that the uppermost yellowish grey
sediment is low in As (1.03 mg/kg) compared to the lower dark grey to black sediment (5.24 mg/kg) rich in mica and organic
matter. Sequential extraction data show that solid phase As bound to poorly crystalline and amorphous metal (Fe, Mn, Al)-oxyhydroxides
is dominant in the grey to dark grey sediment and reaches its maximum level (3.05 mg/kg) in the mica rich layers. Amount of
As bound to sulphides and organic matter also peaks in the dark grey to black sediment. Vertical distributions of major elements
determined by X-ray fluorescence (XRF) show that iron (Fe2O3), aluminum (Al2O3) and manganese (MnO) follow the general trend of distribution of As in the sediments. Concentrations of As, Mn, Fe, HCO3
−, SO4
2− and NO3
− in groundwater reflect the redox status of the aquifer and are consistent with solid phase geochemistry. Mineralogical analysis
by X-ray diffraction (XRD) and scanning electron microscopy (SEM) fitted with energy dispersive X-ray spectrometer (EDS) revealed
dominance of crystalline iron oxides and hydroxides like magnetite, hematite and goethite in the oxidised yellowish grey sediment.
Amorphous Fe-oxyhydroxides identified as grain coating in the mica and organic matter rich sediment suggests weathering of
biotite is playing a critical role as the source of Fe(III)-oxyhydroxides which in turn act as sink for As. Presence of authigenic
pyrite in the dark grey sediment indicates active reduction in the aquifer. 相似文献
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The authors examined the variability in wintertime cyclone activity and storm tracks and their relation to precipitation over China for the period 1951–2006 using the observational data.Two apparent modes of variability were assumed for the cyclone activity and storm tracks.The first mode describes the oscillation in the strength of the storm tracks in East Asia,which significantly increased since the mid-1980s,whereas the second mode describes a seesaw oscillation in the storm track strength between the Central-Southeast China and northern East Asia.The storm tracks over the Central-Southeast China have increased since the late 1960s.The possible causes for the variation of the cyclone activity and storm tracks are also explored.It is shown that wintertime precipitation,which has increased since the mid-1980s,concentrates in Central-Southeast China.The enhancement may be caused by the first mode of variability of storm tracks,whereas the interannual variability of precipitation may be linked to the second mode of the storm track variability. 相似文献
7.
Groundwater – the disregarded component in lake water and nutrient budgets. Part 2: effects of groundwater on nutrients
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Lacustrine groundwater discharge (LGD) transports nutrients from a catchment to a lake, which may fuel eutrophication, one of the major threats to our fresh waters. Unfortunately, LGD has often been disregarded in lake nutrient studies. Most measurement techniques are based on separate determinations of volume and nutrient concentration of LGD: Loads are calculated by multiplying seepage volumes by concentrations of exfiltrating water. Typically low phosphorus (P) concentrations of pristine groundwater often are increased due to anthropogenic sources such as fertilizer, manure or sewage. Mineralization of naturally present organic matter might also increase groundwater P. Reducing redox conditions favour P transport through the aquifer to the reactive aquifer‐lake interface. In some cases, large decreases of P concentrations may occur at the interface, for example, due to increased oxygen availability, while in other cases, there is nearly no decrease in P. The high reactivity of the interface complicates quantification of groundwater‐borne P loads to the lake, making difficult clear differentiation of internal and external P loads to surface water. Anthropogenic sources of nitrogen (N) in groundwater are similar to those of phosphate. However, the environmental fate of N differs fundamentally from P because N occurs in several different redox states, each with different mobility. While nitrate behaves essentially conservatively in most oxic aquifers, ammonium's mobility is similar to that of phosphate. Nitrate may be transformed to gaseous N2 in reducing conditions and permanently removed from the system. Biogeochemical turnover of N is common at the reactive aquifer‐lake interface. Nutrient loads from LGD were compiled from the literature. Groundwater‐borne P loads vary from 0.74 to 2900 mg PO4‐P m?2 year?1; for N, these loads vary from 0.001 to 640 g m?2 year?1. Even small amounts of seepage can carry large nutrient loads due to often high nutrient concentrations in groundwater. Large spatial heterogeneity, uncertain areal extent of the interface and difficult accessibility make every determination of LGD a challenge. However, determinations of LGD are essential to effective lake management. Copyright © 2014 John Wiley & Sons, Ltd. 相似文献
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Yongbo Gao Christoph Merz Gunnar Lischeid Michael Schneider 《Environmental Earth Sciences》2018,77(2):47
Like almost all fields of science, hydrology has benefited to a large extent from the tremendous improvements in scientific instruments that are able to collect long-time data series and an increase in available computational power and storage capabilities over the last decades. Many model applications and statistical analyses (e.g., extreme value analysis) are based on these time series. Consequently, the quality and the completeness of these time series are essential. Preprocessing of raw data sets by filling data gaps is thus a necessary procedure. Several interpolation techniques with different complexity are available ranging from rather simple to extremely challenging approaches. In this paper, various imputation methods available to the hydrological researchers are reviewed with regard to their suitability for filling gaps in the context of solving hydrological questions. The methodological approaches include arithmetic mean imputation, principal component analysis, regression-based methods and multiple imputation methods. In particular, autoregressive conditional heteroscedasticity (ARCH) models which originate from finance and econometrics will be discussed regarding their applicability to data series characterized by non-constant volatility and heteroscedasticity in hydrological contexts. The review shows that methodological advances driven by other fields of research bear relevance for a more intensive use of these methods in hydrology. Up to now, the hydrological community has paid little attention to the imputation ability of time series models in general and ARCH models in particular. 相似文献