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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff
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We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
New determination of the Earth orientation parameters (EOP), based on optical astrometry observations since the beginning of the century, is now under preparation by the Working group established by Commission 19 of the IAU. The Hipparcos catalog is to define the celestial reference frame in which the new series of EOP are to be described, The novelties of the prepared solution are the higher resolution (5 days) and more parameters estimated from the solution (celestial pole offsets, rheological parameters of the Earth, certain instrumental constants). The mathematical model of the solution is described, and the results based on the observations made with 46 instruments at 29 observatories and a preliminary Hipparcos catalog are presented. 相似文献
3.
G. Djurašević P. Rovithis H. Rovithis-Livaniou E. Fragoulopoulou 《Astrophysics and Space Science》2005,296(1-4):311-314
BV light curves of the eclipsing binary UV Leo obtained at the Kryonerion Astronomical Station of the National Observatory of
Athens, Greece, are analyzed. The analysis is based on a Roche configuration with two spots on the secondary surface. The
elements of the two components of the system are calculated and the spot characteristics are given. 相似文献
4.
5.
Milan Burša 《Earth, Moon, and Planets》1992,56(1):57-60
The tidal long-term decrease in the angular velocity of the Earth's rotation has been estimated on the basis of the angular momentum tidal balance in the Earth-Moon-Sun system. The observed (LLR) tidal long-term decrease in the Moon's mean motion, the apparent secular acceleration in the mean longitude of the Sun and the long-term decrease in the 2nd degree zonal geopotential parameter were used.Presented at the XXth General Assembly of the I.A.G., Vienna, August 15, 1991. 相似文献
6.
7.
F.Z. Feygin YU.P. Kurchashov V.A. Troitskaya K. Dobeš 《Planetary and Space Science》1985,33(3):271-273
A high resolution numerical sonagram of Pc-1 magnetic record has shown that single narrow lines of Pc-1 spectra produce lower frequency (“red-shifted”) satellite lines more than twice as often as their higher frequency (“violet”) counterparts. The violet satellites usually emerge only when at least two ancestor lines are present simultaneously. 相似文献
8.
The behaviour of the flare in the period of enhancement and maximum of hard X-ray, microwave and decimetric type IV continuum is analysed. The elongation of the H ribbons and microwave source disclose that the energy release site was shifting through a system of loops with a velocity less than 200 km s-1, and that the energy was carried down the field lines with a velocity of about 1000 km s-1, implying the thermal conduction front mechanism of energy transport. Several processes of energy release are considered and it is concluded that an explanation in terms of succeeding interactions of neighbouring loops, involving fast reconnection of their poloidal components is in best agreement with the observations.Proceedings of the Second CESRA Workshop on Particle Acceleration and Trapping in Solar Flares, held at Aubigny-sur-Nère (France), 23–26 June, 1986. 相似文献
9.
Milan Burša 《Studia Geophysica et Geodaetica》1991,35(3):145-150
Summary The estimate of the tidal long-term decrease in the angular velocity of the Earth's rotation due to the Sun is given as –(0.8±0.3)×10
–22
rad s
–2. It was computed on the basis of the observed total long-term decrease in , of the observed tidal deceleration of the Moon and the observed decrease in the second-degree zonal Stokes geopotential harmonic term. Adopting the estimate given, the product of the Love number and the tidal phase lag angle due to the Sun (in degrees) comes out as 0.53±0.20.
am a z nuuu u z mu au u, az : –(0,8±0,3) 10 –22 a¶rt; –2 . ¶rt; ua n a¶rt;a u , n a¶rt;a nuu u ¶rt;z ¶rt;uu u n a¶rt;a u mz az znmuaz naama ma. u num n au, m nu¶rt;u ua a a z u ( za¶rt;a) a z nuua a (0,53±0,20).相似文献
10.
M. Burša 《Studia Geophysica et Geodaetica》1991,35(2):61-74
Summary It has been shown that dynamically, on the basis of the distribution of angular momenta, the Jovian system cannot be considered an analogue within the Solar system. The total tidal decrease in the angular momentum of Jupiter and in its angular velocity of rotation have been estimated, as well as the loss of mechanical energy due to tidal dissipation. It has been concluded that there are no dynamical contradictions with the hypothesis of the common cosmogonic origin of Jupiter and of its eight close satellites.
aam, m ¶rt;uauu, n an¶rt;u m uma ¶rt;uu, um numa umam aayu um. a a y au ma uma ¶rt;uu numa u z mu z au u—a nuuz mu, ma a nmu au yuu um u—a ¶rt;uunauu. a au, m m ¶rt;uauu azau zunm m zuu aaa numa u z uau u nmu.相似文献