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排序方式: 共有91条查询结果,搜索用时 15 毫秒
1.
Wenyi Zhu Nathan Yee E. Danielle Rhine John R. Reinfelder 《Geochimica et cosmochimica acta》2008,72(21):5243-5250
We examined the hypothesis that sulfide drives arsenic mobilization from pyritic black shale by a sulfide-arsenide exchange and oxidation reaction in which sulfide replaces arsenic in arsenopyrite forming pyrite, and arsenide (As−1) is concurrently oxidized to soluble arsenite (As+3). This hypothesis was tested in a series of sulfide-arsenide exchange experiments with arsenopyrite (FeAsS), homogenized black shale from the Newark Basin (Lockatong formation), and pyrite isolated from Newark Basin black shale incubated under oxic (21% O2), hypoxic (2% O2, 98% N2), and anoxic (5% H2, 95% N2) conditions. The oxidation state of arsenic in Newark Basin black shale pyrite was determined using X-ray absorption-near edge structure spectroscopy (XANES). Incubation results show that sulfide (1 mM initial concentration) increases arsenic mobilization to the dissolved phase from all three solids under oxic and hypoxic, but not anoxic conditions. Indeed under oxic and hypoxic conditions, the presence of sulfide resulted in the mobilization in 48 h of 13-16 times more arsenic from arsenopyrite and 6-11 times more arsenic from isolated black shale pyrite than in sulfide-free controls. XANES results show that arsenic in Newark Basin black shale pyrite has the same oxidation state as that in FeAsS (−1) and thus extend the sulfide-arsenide exchange mechanism of arsenic mobilization to sedimentary rock, black shale pyrite. Biologically active incubations of whole black shale and its resident microorganisms under sulfate reducing conditions resulted in sevenfold higher mobilization of soluble arsenic than sterile controls. Taken together, our results indicate that sulfide-driven arsenic mobilization would be most important under conditions of redox disequilibrium, such as when sulfate-reducing bacteria release sulfide into oxic groundwater, and that microbial sulfide production is expected to enhance arsenic mobilization in sedimentary rock aquifers with major pyrite-bearing, black shale formations. 相似文献
2.
A comparison of three image-object methods for the multiscale analysis of landscape structure 总被引:4,自引:0,他引:4
Geoffrey J. Hay Thomas Blaschke Danielle J. Marceau Andr Bouchard 《ISPRS Journal of Photogrammetry and Remote Sensing》2003,57(5-6):327
Within the conceptual framework of Complex Systems, we discuss the importance and challenges in extracting and linking multiscale objects from high-resolution remote sensing imagery to improve the monitoring, modeling and management of complex landscapes. In particular, we emphasize that remote sensing data are a particular case of the modifiable areal unit problem (MAUP) and describe how image-objects provide a way to reduce this problem. We then hypothesize that multiscale analysis should be guided by the intrinsic scale of the dominant landscape objects composing a scene and describe three different multiscale image-processing techniques with the potential to achieve this. Each of these techniques, i.e., Fractal Net Evolution Approach (FNEA), Linear Scale-Space and Blob-Feature Detection (SS), and Multiscale Object-Specific Analysis (MOSA), facilitates the multiscale pattern analysis, exploration and hierarchical linking of image-objects based on methods that derive spatially explicit multiscale contextual information from a single resolution of remote sensing imagery. We then outline the weaknesses and strengths of each technique and provide strategies for their improvement. 相似文献
3.
4.
Anis Gasmi Cécile Gomez Hédi Zouari Antoine Masse Danielle Ducrot 《Arabian Journal of Geosciences》2016,9(20):753
The purpose of this study was to examine the efficiency of Advanced Space Borne Thermal Emission and Reflection Radiometer (ASTER) data in the discrimination of geological formations and the generation of geological map in the northern margin of the Tunisian desert. The nine ASTER bands covering the visible (VIS), near-infrared (NIR) and short-wave infrared (SWIR) spectral regions (wavelength range of 400–2500 nm) have been treated and analyzed. As a first step of data processing, crosstalk correction, resampling, orthorectification, atmospheric correction, and radiometric normalization have been applied to the ASTER radiance data. Then, to decrease the redundancy information in highly correlated bands, the principal component analysis (PCA) has been applied on the nine ASTER bands. The results of PCA allow the validation and the rectification of the lithological boundaries already published on the geologic map, and gives a new information for identifying new lithological units corresponding to superficial formations previously undiscovered. The application of a supervised classification on the principal components image using a support vector machine (SVM) algorithm shows good correlation with the reference geologic map. The overall classification accuracy is 73 % and the kappa coefficient equals to 0.71. The processing of ASTER remote sensing data set by PCA and SVM can be employed as an effective tool for geological mapping in arid regions. 相似文献
5.
Mariana Vezzone Ricardo Cesar Helena Polivanov Aline Serrano Danielle Siqueira Leticia Abreu Miriam Bianchi Maria Elizabeth Correia Zuleica Castilhos Tácio de Campos 《Environmental Earth Sciences》2018,77(21):743
The toxicity and metal bioavailability were studied in dredged sediments from Rodrigo de Freitas Lagoon (Rio de Janeiro, RJ, Brazil) using acute and avoidance tests with Eisenia andrei, and reproduction tests with Folsomia candida. The sediment was mixed with an artificial soil, and two natural soils (ferralsol and chernosol—representative Brazilian tropical soils) to obtain the following doses: 1, 3, 6, 12, 18, 24 and 30%. Total metal concentrations were determined in the sediment to support the interpretation of ecotoxicological data. Metal concentrations in the mixtures were in agreement with the threshold limits established by Brazilian law. However, significant avoidance responses were found on doses ≥?3% and were the most sensitive endpoint. Earthworm mortality found in artificial soil mixtures (LC50?=?3.9) suggests higher toxicity levels than those obtained in ferralsol (LC50?=?7.6%) and chernosol (11.0%) treatments. Earthworm mortality, avoidance responses and collembolan reproduction levels found in ferralsol mixtures (LC50?=?9.2; avoidance EC50?=?2.3%; reproduction EC50?=?2.8%) were higher compared to chernosol treatments (LC50?=?11.0%; avoidance EC50?=?4.3%; reproduction EC50?=?4.9%). The reduction of toxicity levels in chernosol mixtures is probably due to the abundance of expansive clay minerals in chernosols with capacity of adsorbing metals and other xenobiotic substances from soil pore water, decreasing metal bioavailability. Finally, threshold limits defined by Brazilian legislation for soil quality and land disposal of dredged sediments are not sufficient to prevent noxious effects on soil fauna and should be complemented with a preliminary ecotoxicological evaluation. 相似文献
6.
Trace element and isotopic characteristics of late Carboniferous to early Permian minettes and kersantites have been determined. These lamprophyres have been sampled throughout the Western European Hercynian orogen, from Brittany to the west to Schwarzwald to the east. In spite of sharp petrological differences reflected by mineralogy and major element geochemistry, minettes and kersantites exhibit close identity with respect to trace element and isotopic features. These features comprise enrichment in incompatible elements, highCs/Rb and lowCe/Pb ratios, Ta and Ti relative depletion, high abundance in transition elements and highNi/Mg ratios. Pb isotope ratios are undistinguishable from those measured on Hercynian continental crust. Initial143Nd/144Nd ratios are between0.5120 (εi −5) and0.5122 (εi −1) for minettes and kersantites whereas initial87Sr/86Sr ratios vary between 0.7055–0.710 for minettes and 0.707–0.708 for kersantites. No simple mixing relations are visible on RbSr and SmNd isochron diagrams. The exceptional homogeneity of these geochemical characteristics along a 1000 km traverse does not allow for an hypothesis of enrichment through upper level assimilation and thus leads to propose that these rocks originated through melting of a mantle enriched by recycling of crustal material. 相似文献
7.
Danielle J. Marceau Luc Guindon Mireille Bruel Claude Marois 《The Professional geographer》2001,53(4):546-558
This article addresses the issue of linking temporal and spatial information into a GIS database structure to investigate the land‐use changes in a rural‐urban region over a thirty‐five‐year period. More specifically, it describes the application of a programming package developed to build temporal topology in an historical land‐use GIS database to efficiently perform spatiotemporal queries. The program was created within the MapInfo environment using MapBasic language. Different types of information, such as the rate of change, the relationship between the change of land use and zoning regulations, and land‐use succession were extracted from the database. A user‐friendly interface was also developed to easily address spatiotemporal queries to the database. This approach represents a flexible and performing tool for scientists and planners who need to efficiently capture essential spatiotemporal information required for geographical inquiry and decision‐making. 相似文献
8.
Wildfires cause enormous damage worldwide, particularly in Victoria, Australia, with growing populations in fire-prone ecosystems. Broad-scale prescribed burning is an established, yet controversial, wildfire management policy in Victoria and Australia. But does broad-scale prescribed burning reduce fire damage? The answer depends on how damage is measured. We propose that different perceptions about the efficacy of broad-scale prescribed burning derive from different disciplinary measures of damage (e.g., biodiversity, area burned, or fatalities). Although broad-scale prescribed burning reduces subsequent wildfire size, there is little evidence that it saves human lives and homes. Evidence suggests that small-scale fuel reduction may be more effective at saving lives. The prescribed burning debate might be better focused on what damage we wish to limit, and which measures are most effective at limiting this damage. In this context, the current policy focus on broad-scale prescribed burning targets may distract efforts from more effective lifesaving strategies. 相似文献
9.
Topography and morphodynamics in the German Bight using SAR and optical remote sensing data 总被引:3,自引:0,他引:3
Morphological changes in coastal areas, especially in river estuaries, are of high interest in many parts of the world. Satellite
data from both optical and radar sensors can help to monitor and investigate these changes. Data from both kinds of sensors
being available for up to 30 years now, allow examinations over large timescales, while high resolution sensors developed
within the last decade allow increased accuracy. So the creation of digital elevation models (DEMs) of, for example, the wadden
sea from a series of satellite images is already possible. ENVISAT, successfully launched on March 1, 2002, continues the
line of higher resolution synthetic aperture radar (SAR) imaging sensors with its ASAR instrument and now also allows several
polarization modes for better separation of land and water areas. This article gives an overview of sensors and algorithms
for waterline determination as well as several applications. Both optical and SAR images are considered. Applications include
morphodynamic monitoring studies and DEM generation.
相似文献
Andreas NiedermeierEmail: |
10.
Radovan Pipík Anne-Marie Bodergat Danielle Briot Michal Ková? Ján Král’ Grzegorz Zielinski 《Journal of Paleolimnology》2012,47(2):233-249
The Turiec Basin (TB) of Slovakia formed in the Miocene when the West Carpathians escaped from the Alpine region. The 1,250-m-thick
sedimentary Neogene fill of the basin preserved fossil leaves as well as endemic bivalves, gastropods, and ostracodes. The
paleolimnologic changes recorded in the TB infill were derived from the most abundant fossils, the ostracodes. Five contemporaneous
ostracode assemblages within the Late Miocene lacustrine system were distinguished through statistical analysis. These assemblages
have low species similarity, between 2.1 and 24.1%, and are recognized by shape differences among the Candoninae. The ostracode
assemblages, mollusca fossils, and Sr-isotope ratios suggest a low-salinity environment at the beginning of the Late Miocene,
during a brief connection with the Central Paratethys. When the connection ceased, the basin became an isolated freshwater
lake, with five zones differentiated ecologically and bathymetrically using the ostracode assemblages. Taxonomic comparison
of the faunas of the TB and the freshwater to brackish Neogene basins of Europe demonstrates the endemic character of the
TB ostracode fauna. The biologic characteristics of the ostracode families, along with the geology of the lake basin, suggest
that the longevity of the Late Miocene lake probably exceeded 1 Ma. 相似文献