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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
A formula for the thickness of a shear band formed in saturated soils under a simple shear or a combined stress state has been proposed. It is shown that the shear band thickness is dependent on the pore pressure properties of the material and the dilatancy rate, but is independent of the details of the combined stress state. This is in accordance with some separate experimental observations. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
3.
Stress wave attenuation across fractured rock masses is a great concern of underground structure safety. When the wave amplitude is large, fractures experience nonlinear deformation during the wave propagation. This paper presents a study on normal transmission of P‐wave across parallel fractures with nonlinear deformational behaviour (static Barton–Bandis model). The results show that the magnitude of transmission coefficient is a function of incident wave amplitude, nondimensional fracture spacing and number of fractures. Two important indices of nondimensional fracture spacing are identified, and they divide the area of nondimensional fracture spacing into three parts (individual fracture area, transition area and small spacing area). In the different areas, the magnitude of transmission coefficient has different trends with nondimensional fracture spacing and number of fractures. In addition, the study reveals that under some circumstances, the magnitude of transmission coefficient increases with increasing number of fractures, and is larger than 1. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
4.
The range-averaged intensity model (RAIM) long known as a powerful method for transmission loss estimation in waveguides, is extended to other aspects of the acoustic field: impulse response and angular pattern estimations at a receiver, general time spreading in a waveguide, signal fluctuations, reverberation levels, and ambient noise structure. An example of its application to a SOFAR propagation and detection case is presented. This method appears to be a very efficient and reliable analysis tool for many underwater acoustics configurations: particularly long-range horizontal telemetry and shallow-water sonar 相似文献
5.
In the coastal and estuarine waters of Goa, particulate organic carbon (POC) varied from 0.52 to 2.51 mg l?1 and from 0.28 to 5.24 mg l?1 and particulate phosphorus (PP) varied from 0.71 to 5.18 μg l?1 and from 0.78 to 20.34 μg l?1, respectively. The mean values of chlorophyll and primary productivity were 1.94 mg m?3 and 938.1 mg C m?2 day?1 in the coastal waters and 4.3 mg m?3 and 636.5 mg C m?1 day?1 in the estuarine waters, respectively. ratios were low in June and October even when POC values were quite high. The POC in surface waters was linearly correlated with the chlorophyll content. Also PP increased when chlorophyll and primary productivity remained high. The results suggest that the phytoplankton was sharply increasing and contributed to POC and PP content. The percentage of detritus calculated from the intercept values of chlorophyll on POC varied from 46 to 76% depending on season. Results indicate that the major portion of POC and PP during postmonsoon (October–January) is derived from phytoplankton production while the allochthonous matter predominate during monsoon (June–September). 相似文献
6.
7.
Natural and agricultural wetlands are considered to be the major sources of global atmospheric methane (CH4). A one‐dimensional model was developed to simulate methane emission and used to examine the influence of various physical processes on the rate of methane emission. Three processes involved in the methane emission are implemented in the model: production, reoxidation and transport. Three transport pathways were considered: diffusion across water–air or soil–air interfaces, ebullition and diffusion through plants. These pathways are influenced by soil properties, plant growth, water‐table conditions, temperature and external inputs (e.g. fertilizer). The model was used to examine the seasonal variation of the methane emission at a rice field in Hunan, China, which was observed during a field experiment for consecutive (early and late) rice seasons in 1992. The observed seasonal variations of methane emission, and role of plants in transporting methane to the atmosphere, are captured by the model simulation. Further model applications were conducted to simulate effects of fertilizer and water‐level condition on the methane emission. The results indicate that unfermented organic fertilizer produces a higher methane emission rate than mineral fertilizer. The simulations with treatments of a deep‐water covering and constant moisture reduced the methane emission. The rice field study provides a framework for further development of the model towards simulations based on spatially distributed variables (e.g. water table, soil temperature and vegetation) at a regional scale. Copyright © 2003 John Wiley & Sons, Ltd. 相似文献
8.
C. Caroubalos D. Maroulis N. Patavalis J.-L. Bougeret G. Dumas C. Perche C. Alissandrakis A. Hillaris X. Moussas P. Preka-Papadema A. Kontogeorgos P. Tsitsipis G. Kanelakis 《Experimental Astronomy》2001,11(1):23-32
We present the new solar radiospectrograph of the University of Athensoperating at the Thermopylae Station since 1996. Observations cover thefrequency range from 110 to 688 MHz. The radiospectrograph has a 7-meterparabolic antenna and two receivers operating in parallel. One is a sweepfrequency receiver and the other a multichannel acousto-optical receiver.The data acquisition system consists of a front-end VME based subsystem anda Sun Sparc-5 workstation connected through Ethernet. The two subsystems areoperated using the VxWorks real-time package. The daily operation is fullyautomated: pointing of the antenna to the sun, starting and stopping theobservations at pre-set times, data acquisition, data compression by`silence suppression', and archiving on DAT tapes. The instrument can beused either by itself to study the onset and evolution of solar radio bursts or in conjunction with other instruments including theNançay Decametric Array and the WIND/WAVES RAD1 and RAD2 low frequencyreceivers to study associated interplanetary phenomena. 相似文献
9.
Himalayan magmatism and porphyry copper–molybdenum mineralization in the Yulong ore belt, East Tibet
Summary ?The NW–SE-trending Yulong porphyry Cu–Mo ore belt, situated in the Sanjiang0 area of eastern Tibet, is approximately 400 km
long and 35 to 70 km wide. Complex tectonic and magmatic processes during the Himalayan epoch have given rise to favorable
conditions for porphyry-type Cu–Mo mineralization.
Porphyry masses of the Himalayan epoch in the Yulong ore belt are distributed in groups along regional NW–SE striking tectonic
lineaments. They were emplaced mainly into Triassic and Lower Permian sedimentary-volcanic rocks. K–Ar und U–Pb isotopic datings
give an intrusion age range of 57–26 Ma. The porphyries are mainly of biotite monzogranitic and biotite syenogranitic compositions.
Geological and geochemical data indicate that the various porphyritic intrusions in the belt had a common or similar magma
source, are metaluminous to peraluminous, Nb–Y–Ba-depleted, I-type granitoids, and belong to the high-K calc-alkaline series.
Within the Yulong subvolcanic belt a number of porphyry stocks bear typical porphyry type Cu–Mo alteration and mineralization.
The most prominent porphyry Co–Mo deposits include Yulong, Malasongduo, Duoxiasongduo, Mangzong and Zhanaga, of which Yulong
is one of the largest porphyry Cu (Mo) deposits in China with approximately 8 × 106 tons of contained Cu metal. Hydrothermal alteration at Yulong developed around a biotite–monzogranitic porphyry stock that
was emplaced within Upper Triassic limestone, siltstone and mudstone. The earliest alteration was due to the effects of contact
metamorphism of the country rocks and alkali metasomatism (potassic alteration) within and around the porphyry body. The alteration
of this stage was accompanied by a small amount of disseminated and veinlet Cu–Mo sulfide mineralization. Later alteration–mineralization
zones form more or less concentric shells around the potassic zone, around which are distributed a phyllic or quartz–sericite–pyrite
zone, a silicification and argillic zone, and a propylitic zone.
Fluid inclusion data indicate that three types of fluids were involved in the alteration–mineralization processes: (1) early
high temperature (660–420 °C) and high salinity (30–51 wt% NaCl equiv) fluids responsible for the potassic alteration and
the earliest disseminated and/or veinlet Cu–Mo sulfide mineralization; (2) intermediate unmixed fluids corresponding to phyllic
alteration and most Cu–Mo sulfide mineralization, with salinities of 30–50 wt% NaCl equiv and homogenization temperatures
of 460–280 °C; and (3) late low to moderate temperature (300–160 °C) and low salinity (6–13 wt% NaCl equiv) fluids responsible
for argillic and propylitic alteration. Hydrogen and oxygen isotopic studies show that the early hydrothermal fluids are of
magmatic origin and were succeeded by increasing amounts of meteoric-derived convective waters. Sulfur isotopes also indicate
a magmatic source for the sulfur in the early sulfide mineralization, with the increasing addition of sedimentary sulfur outward
from the porphyry stock.
Received August 29, 2001; revised version accepted May 1, 2002
Published online: November 29, 2002 相似文献
10.