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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
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Daniela Lazzaro Marcos A. Florczak Alberto Betzler Othon C. Winter Silvia M. Giuliatti-Winter Claudia A. Angeli Dietmar W. Foryta 《Planetary and Space Science》1996,44(12):1547-1550
The results of photometric observations of comet/asteroid 2060 Chiron at the Observatório do Pico dos Dias (Brazil-OPD) and the Observatoire de Haute-Provence (France-OHP) during 1994 and 1995 are presented. The analysis of the data shows a decrease of 2060 Chiron brightness from its peak values of 1988–1991. The absolute magnitude, Hv, varies from a maximum of 6.6 in February 1994 up to a minimum of 6.8 in June 1995. Therefore 2060 Chiron is back to a minimum of activity close to that of 1983–1985. The slope parameter G is found to be G = 0.71 ± 0.15. It is suggested that the H-G magnitude system, generally adopted to present 2060 Chiron brightness, is not the most appropriate due to the cometary activity of this object. 相似文献
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Alberto Etchegoyen 《Astrophysics and Space Science》2004,290(3-4):379-387
The Auger Project studies the highest energies known in nature with an emphasis on energies ≥5 × 1019 eV, which are cosmic rays coming from the outer space reaching the Earth's surface with a very low flux. The questions to be elucidated are what are the origin, energy, production mechanism, and chemical composition of these cosmic rays. Auger aims at building two observatories in both the hemispheres and in 2000 the construction of the austral observatory started. Auger's two distinctive features are its exceptional size and its hybrid nature. It spans over an area of 3000 km2 and is constituted by 24 fluorescence detector telescopes and 1600 surface detectors. As such, it will provide a large number of events with less systematic detection uncertainties. The construction of the Southern Observatory in Argentina is quite advanced and the buildings at the Central Station in Malargüe city are already operational. So are the telescope buildings at Cerros Los Leones and Coihueco (two prototype telescopes were operational at Los Leones, which have now been dismantled), 32 surface detectors, and the telecommunication and data acquisition systems. About 20-hybrid events/months were detected and currently two events/hours are registered with the surface detector array. The detection of hybrid events is the most important issue since it shows that the equipment operates within the design parameters. 相似文献
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Irina N Belskaya Vasilij G Shevchenko Yurij N Krugly Yurij S Efimov Alberto Cellino 《Icarus》2003,166(2):276-284
The first results of the observational program devoted to simultaneous investigation of asteroid polarimetric and photometric opposition phenomena are presented. UBVRI polarimetric and V-band photometric observations of the S-type Asteroid 20 Massalia and the E-type Asteroids 214 Aschera and 620 Drakonia were carried out in 1996-1999 down to phase angles of 0.08°, 0.7°, and 1.2°, correspondingly. The S-type Asteroid 20 Massalia is characterized by the pronounced brightness opposition surge with an amplitude larger than that observed for the E-type asteroids. A sharp peak of negative polarization at small phase angles was not observed for this asteroid. The value of polarization degree at phase angle α<1° is less than 0.5% for both S and E types. The negative polarization branches of S and especially E-asteroids have an asymmetrical shape. The phase angle at which the polarization minimum occurs is close to the angle at which non-linear increase begins in the asteroid magnitude phase curves. A relation of the observed effects to the mechanism of coherent backscattering is discussed. 相似文献
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Sarah Church Peter Ade James Bock Melanie Bowden John Carlstrom Ken Ganga Walter Gear James Hinderks Wayne Hu Brian Keating John Kovac Andrew Lange Eric Leitch Olivier Mallie Simon Melhuish Anthony Murphy Ben Rusholme Creidhe OSullivan Lucio Piccirillo Clem Pryke Andy Taylor Keith Thompson 《New Astronomy Reviews》2003,47(11-12):1083
QUEST on DASI is a ground-based, high-sensitivity, high-resolution (ℓmax2500) experiment designed to map CMB polarization at 100 and 150 GHz and to measure the power spectra from E-modes, B-modes from lensing of the CMB, and B-modes from primordial gravitational waves. The experiment comprises a 2.6 m Cassegrain optical system, equipped with an array of 62 polarization-sensitive bolometers (PSBs), located at the South Pole. The instrument is designed to minimize systematic effects; features include differencing of pairs of orthogonal PSBs within a single feed, a rotatable achromatic waveplate, and axisymmetric rotatable optics. In addition the South Pole location allows both repeatable and highly controlled observations. QUEST on DASI will commence operation in early 2005. 相似文献
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We present a photometric analysis of the eclipsing binary systemGSC4832.400 based on 732 photometric observations obtained on sixteen clear nights during 1999–2000 in the V-Johnson and yb-Strömgren filters. The observed times of the minima yielded a linear ephemeris showing that the system has a constant period of 0.313150 ± 0.000002days. The light curve corresponds to a circular orbit for the system and clearly shows that GSC4832.400 has the defining characteristics of a W UMa-type eclipsing binary. It also shows a small O'Connell effect, which could be due to the presence of a hot spot in the primary star. A preliminary photometric solution based on the assumption of an over contact systemsatis factorily reproduced the observed light curve. 相似文献
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The ordinary kriging method, a geostatistical interpolation technique, was applied for developing contour maps of design storm depth in northern Taiwan using intensity–duration–frequency (IDF) data. Results of variogram modelling on design storm depths indicate that the design storms can be categorized into two distinct storm types: (i) storms of short duration and high spatial variation and (ii) storms of long duration and less spatial variation. For storms of the first category, the influence range of rainfall depth decreases when the recurrence interval increases, owing to the increasing degree of their spatial independence. However, for storms of the second category, the influence range of rainfall depth does not change significantly and has an average of approximately 72 km. For very extreme events, such as events of short duration and long recurrence interval, we do not recommend usage of the established design storm contours, because most of the interstation distances exceed the influence ranges. Our study concludes that the influence range of the design storm depth is dependent on the design duration and recurrence interval and is a key factor in developing design storm contours. Copyright © 2003 John Wiley & Sons, Ltd. 相似文献