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1.
Philippe E. Raison Regis Jardin Daniel Bouëxière Rudy J. M. Konings Thorsten Geisler Claudiu C. Pavel Jean Rebizant Karin Popa 《Physics and Chemistry of Minerals》2008,35(10):603-609
The crystallographic structures of the synthetic cheralite, CaTh(PO4)2, and its homolog CaNp(PO4)2 have been investigated by X-ray diffraction at room temperature. Rietveld analyses showed that both compounds crystallize in the monoclinic system and are isostructural to monazite LnPO4 (Ln = La to Gd). The space group is P21/n (I.T. = 14) with Z = 2. The refined lattice parameters of CaTh(PO4)2 are a = 6.7085(8) Å, b = 6.9160(6) Å, c = 6.4152(6) Å, and β = 103.71(1)° with best fit parameters R wp = 4.87%, R p = 3.69% and R B = 3.99%. For CaNp(PO4)2, we obtained a = 6.6509(5) Å, b = 6.8390(3) Å, c = 6.3537(8) Å, and β = 104.12(6)° and R wp = 6.74%, R p = 5.23%, and R B = 6.05%. The results indicate significant distortions of bond length and angles of the PO4 tetrahedra in CaTh(PO4)2 and to a lesser extent in CaNp(PO4)2. The structural distortions were confirmed by Raman spectroscopy of CaTh(PO4)2. A comparison with the isostructural compounds LnPO4 (Ln = Ce and Sm) confirmed that the substitution of the large rare earth trivalent cations with Ca2+ and Th4+ introduces a distortion of the PO4 tetrahedra. 相似文献
2.
Yves Moëlo Pierre Palvadeau Nicolas Meisser Alain Meerschaut 《Comptes Rendus Geoscience》2002,334(8):529-536
Cu-poor meneghinite from La Lauzière Massif (Savoy, France) has the composition (electron microprobe) (in wt%): Pb 59.50, Sb 20.33, Bi 1.19, Cu 0.87, Ag 0.05, Fe 0.03, S 17.62, Se 0.05, Total 99.64. Its crystal structure (X-ray on a single crystal) was solved with R1=0.0506, wR2=0.1026, with an orthorhombic symmetry, space group Pnma, and a=24.080(5) Å, b=4.1276(8) Å, c=11.369(2) Å, V=1130.0(4) Å3, Z=4. Relatively to the model of Euler and Hellner (1960), this structure shows a significantly lower site occupancy factor for the tetrahedral Cu site (0.146 against 0.25). Among the five other metallic sites, Bi appears in the one with predominant Sb. Developed structural formula: Cu0.15Pb2(Pb0.53Sb0.47)(Pb0.46Sb0.54)(Sb0.75Pb0.19Bi0.06)S6; the reduced one: Cu0.58Pb12.72(Sb7.04Bi0.24)S24. The formation of such a Cu-poor variety seems to be related to specific paragenetic conditions (absence of coexisting galena), or to crystallochemical constraints (minor Bi). To cite this article: Y. Moëlo et al., C. R. Geoscience 334 (2002) 529–536. 相似文献
3.
Delphine Yeghicheyan Cécile Bossy Martine Bouhnik Le Coz Chantal Douchet Guy Granier Alexie Heimburger Francois Lacan Aurélie Lanzanova Tristan C. C. Rousseau Jean‐Luc Seidel Mickaël Tharaud Frédéric Candaudap Jérôme Chmeleff Christophe Cloquet Sophie Delpoux Marie Labatut Rémi Losno Catherine Pradoux Yann Sivry Jeroen E. Sonke 《Geostandards and Geoanalytical Research》2013,37(4):449-467
The natural river water certified reference material SLRS‐5 (NRC‐CNRC) was routinely analysed in this study for major and trace elements by ten French laboratories. Most of the measurements were made using ICP‐MS. Because no certified values are assigned by NRC‐CNRC for silicon and 35 trace element concentrations (rare earth elements, Ag, B, Bi, Cs, Ga, Ge, Li, Nb, P, Rb, Rh, Re, S, Sc, Sn, Th, Ti, Tl, W, Y and Zr), or for isotopic ratios, we provide a compilation of the concentrations and related uncertainties obtained by the participating laboratories. Strontium isotopic ratios are also given. 相似文献
4.
5.
Jianhui Wei Ningpeng Dong Benjamin Fersch Joël Arnault Sven Wagner Patrick Laux Zhenyu Zhang Qianya Yang Chuanguo Yang Shasha Shang Lu Gao Zhongbo Yu Harald Kunstmann 《水文研究》2021,35(8):e14341
The regional terrestrial water cycle is strongly altered by human activities. Among them, reservoir regulation is a way to spatially and temporally allocate water resources in a basin for multi-purposes. However, it is still not sufficiently understood how reservoir regulation modifies the regional terrestrial- and subsequently, the atmospheric water cycle. To address this question, the representation of reservoir regulation into the terrestrial component of fully coupled regional Earth system models is required. In this study, an existing process-based reservoir network module is implemented into NOAH-HMS, that is, the terrestrial component of an atmospheric–hydrologic modelling system, namely, the WRF-HMS. It allows to quantitatively differentiate role of reservoir regulation and of groundwater feedback in a simulated ground-soil-vegetation continuum. Our study focuses on the Poyang Lake basin, where the largest freshwater lake of China and reservoirs of different sizes are located. As compared to streamflow observations, the newly extended NOAH-HMS slightly improves the streamflow and streamflow duration curves simulation for the Poyang Lake basin for the period 1979–1986. The inclusion of reservoir regulation leads to major changes in the simulated groundwater recharges and evaporation from reservoirs at local scale, but has minor effects on the simulated soil moisture and surface runoff at basin scale. The performed groundwater feedback sensitivity analysis shows that the strength of the groundwater feedback is not altered by the consideration of reservoir regulation. Furthermore, both reservoir regulation and groundwater feedback modify the partitioning of the simulated evapotranspiration, thus affecting the atmospheric water cycle in the Poyang Lake region. This finding motivates future research with our extended fully coupled atmospheric–hydrologic modelling system by the community. 相似文献
6.
Water Resources - Annaba gulf is a coastal area (southwestern Mediterranean Sea) that receives large diffuse inputs from Fertial plant, Seybouse wadi and Boujemaâ wadi, which are influenced by... 相似文献
7.
Pietro Salizzoni Raphaël Van Liefferinge Patrick Mejean Lionel Soulhac Richard J. Perkins 《Boundary-Layer Meteorology》2010,135(3):455-467
The influence of surface roughness on the dispersion of a passive scalar in a rough wall turbulent boundary layer has been
studied using wind-tunnel experiments. The surface roughness was varied using different sizes of roughness elements, and different
spacings between the elements. Vertical profiles of average concentration were measured at different distances downwind of
the source, and the vertical spread of the plume was computed by fitting a double Gaussian profile to the data. An estimate
of the integral length scale is derived from the turbulence characteristics of the boundary layer and is then used to scale
the measured values of plume spread. This scaling reduces the variability in the data, confirming the validity of the model
for the Lagrangian integral time scale, but does not remove it entirely. The scaled plume spreading shows significant differences
from predictions of theoretical models both in the near and in the far field. In the region immediately downwind of the source
this is due to the influence of the wake of the injector for which we have developed a simple model. In the far field we explain
that the differences are mainly due to the absence of large-scale motions. Finally, further downwind of the source the scaled
values of plume spread fall into two distinct groups. It is suggested that the difference between the two groups may be related
to the lack of dynamical similarity between the boundary-layer flows for varying surface roughness or to biased estimates
of the plume spread. 相似文献
8.
9.
This paper applies a Kuramoto model of coupled oscillators to investigate the north–south (N–S) solar asymmetry and properties of meridional circulation. We focus our study on the asymmetry of the 11-year phase, which is slight but persistent: only two changes of sign (around 1928 and 1968) are observed in the past century. We present a model of two non-linear coupled oscillators that links the hemispheric phase asymmetry of sunspots with the asymmetry of the meridional flow. We use a Kuramoto model with evolving frequencies and constant symmetric coupling to show how asymmetry in meridional circulation could produce a persistent phase lead of one solar hemisphere over the other. We associate the natural frequencies of the two oscillators with the velocities of the meridional flow cells in the northern and southern hemispheres. We assume the respective circulations to be independent and estimate the value of the relevant cross-equatorial coupling by the coupling coefficient in the Kuramoto model. We find that a persistent N–S asymmetry of sunspots and the change of the leading hemisphere could indeed both be the result of the evolving frequencies of meridional circulation; the necessary asymmetry of the meridional flow may be small; and the cross-equatorial coupling has an intermediate range value. Possible applications of these results in solar dynamo models are discussed. 相似文献
10.
Jean‐Charles Leclerc Pascal Riera Laure M.‐L. J. Noël Cédric Leroux Ann C. Andersen 《Marine Ecology》2014,35(2):261-270
The diet of Pomatoschistus microps has been studied using both gut content and stable isotope analyses. In the Roscoff Aber Bay (Brittany, France), this fish is commonly found on sandy muddy intertidal flats. Gut content analyses were also interpreted using trophic indices. Owing to the large diversity of prey consumed, these indices emphasised the opportunistic feeding behaviour of P. microps. Here, this species fed mainly on endofauna with meiofauna being of high relative importance. The main biotic components of its trophic habitat, characterized by δ13C and δ15N, provided evidence of a major trophic pathway based on drift Enteromorpha sp. Trophic positions estimated by both diet analyses and isotopic analyses led to similar results. In this bay, P. microps is a first‐order predator with a low degree of omnivory. Despite a preferential consumption of the amphipod Corophium arenarium, we assumed that this goby behaves as a generalist feeding on a uniform variety of endofauna taxa. 相似文献