2017年6月大气环流和天气分析

2017年6月大气环流的主要特征是极涡偏强且呈单极型分布,中高纬环流呈多波型,西太平洋副热带高压强度较常年偏弱。6月全国平均气温20.3℃,较常年同期偏高0.3℃;全国平均降水量112.3 mm,比常年同期(99.3 mm)偏多13%,长江流域入梅时间较常年偏早。我国南方地区有6次区域性暴雨过程,部分地区暴雨洪涝重;与此同时,东北、华北等地少雨高温,干旱持续时间较长;月内今年第2号台风苗柏在广东深圳登陆;全国19个省（区、市）遭受风雹灾害。     

2017年7月大气环流和天气分析

2017年7月大气环流特征为,极涡呈偶极型分布,主体强度较常年偏强;中高纬环流呈5波型分布,北半球副热带高压强度偏强,西太平洋副热带高压整体位置偏北,脊线持续北抬。7月我国平均气温为23.2℃,较常年同期（21.9℃）偏高1.3℃。全国平均降水量112.5 mm,较常年同期（120.6 mm）偏少6.7%,东北地区西部、江南地区东北部、江淮地区西南部和新疆北部等地降水偏少显著。强降水天气主要出现在东北地区和南方,7月我国出现9次区域性暴雨天气过程,7月13—14日降水过程多方面突破历史极值。7月西北太平洋地区有8个台风生成,其中7个台风活跃,3个台风登陆我国,数量较历史同期明显偏多;台风生成个数与1994、1967和1971年并列为历史同期最多。内蒙古东部出现气象干旱,江淮江汉伏旱发展。中东部地区和新疆持续高温天气,最长持续天数为20 d,1884站出现35℃以上高温天气;高温极值为49℃,发生在吐鲁番站。     

巴丹吉林沙漠北缘拐子湖近地层湍流能谱特征分析

利用2013年6月巴丹吉林沙漠拐子湖地区流沙下垫面的陆气通量观测资料,计算并分析了该研究区不同大气稳定层结条件下的湍流速度各分量谱和温度谱及湍流的局地各向同性特征。结果表明:该研究区风速各分量的湍流强度随平均风速的增加而逐渐减小,当平均风速2 m/s时,风速各分量的湍流强度逐渐稳定且基本限定在0.5以内。在不同大气稳定度下,湍流速度和温度能谱曲线在惯性副区内逐渐有合并趋势且遵循Kolmogorov提出的-2/3定律,速度各分量谱在高频段均满足各向同性且符合低频限制理论。随着稳定度的增加,风速分量的能谱曲线逐渐降低且向高频端移动,风速分量和温度能谱对应的谱峰长度则逐渐减小。该研究区水平湍流尺度范围为9.0~600 m,垂直湍流谱峰波长为10.79~75 m。该结果介于草地和森林下垫面之间,与塔克拉玛干沙漠腹地的试验结果较为接近。     

地球化学组成揭示的杜蒙沙地化学风化和沉积再循环特征及其对风尘物质贡献的指示

对杜蒙沙地的河流冲积砂、河漫滩泥质粉砂、沙质古土壤和风成沙等不同类型沉积物进行了采样（27组）,对这些样品的细颗粒组分（<63 μm）进行了常量元素、微量元素、稀土元素（REE）和Sr-Nd同位素比值等地球化学分析,就杜蒙沙地的化学风化、沉积再循环特征及其对风尘物质的贡献等展开了讨论。结果显示,杜蒙沙地的地球化学组成表现出空间的均一性,低的化学蚀变指数CIA（48~56,平均52）及A-CN-K和A-CNK-FM图解均表明了杜蒙沙地仅遭受了低级的化学风化程度。沙地的成分成熟度较低,大部分河流沉积物表现出初次循环沉积特征,系大兴安岭东侧中酸性岩浆母岩风化剥蚀的产物经嫩江搬运堆积形成;古土壤表现出与河流沉积物相同的初次循环特征,表明古土壤的成土母质是河流沉积物,这与野外地层出露情况一致;风成沙表现出再循环沉积特征,系河流沉积物就地起沙搬运堆积形成。不活动元素比值、REE和Sr-Nd同位素比值等物源判别图解,结合植被和地貌状况,一致表明杜蒙沙地与东北平原中东部的风尘物质没有地球化学亲缘关系,其对该地区（甚至下风向更远地区）的大气风尘的贡献很小。     

大气负荷响应计算误差估计模型

用数理统计技术，建立格林函方法计算大气变化引起重力和形焦等效应的精度评定模型，并利用中国及其邻区的大气观,蛭大气误差常数和一个计算方案的精度估计，其结果与固体潮汐检测在不同气候条件下的响应情况相一致，该系统也可应用于格林函数积分形式的其它物理模型的误差估计。     

A Simple Kinetic Model for Autoxidation of S(IV) Oxides Catalyzed by Iron and/or Manganese Ions

The reaction kinetics of S(IV) autoxidation catalyzed by single metal ions of Mn(II) and Fe(II) or Fe(III) and by a mixture of Mn(II) and Fe(II) under the conditions representative for acidified atmospheric liquid water was investigated. A simple power law kinetic model based on the stability constants for metal-sulfito complexes formed during the first step of a radical chain mechanism predicts well the kinetics for the reactions catalyzed by single metal ions. The calculated stability constants for iron (5.7×10³ dm³ mol^–1) and manganese (10×10⁴ dm³ mol^–1) sulfito complexes are close to those reported in the literature. The catalytic synergism between Mn(II) and Fe(II) was confirmed. For this system the following power law rate equation was suggested:r_tot = S_Fe · r_Fe + S_Mn · r_Mn ,where r_Fe and r_Mn are the reaction rates in the presence of Fe(II) and Mn(II), respectively. S_Fe and S_Mn are proportional factors, which account for the synergistic effect. The proposed power law rate equation predicts the reaction kinetics very well. The values of S_Fe (1.35) and S_Mn (15) indicate that the influence of Fe(II)/Fe(III) on Mn(II)/Mn(III) cycling is larger than, vice versa, agreeing with the reaction mechanism proposed for the S(IV) autoxidation catalyzed by mixed metal ions.     

风成沉积物磁组构与中国黄土区第四纪风向变化

通过对黄土高原几个剖面黄土样品磁化率各向异性的初步研究，发现了风成沉积物中的磁组构特征，且它的形成受沉积作用控制并与黄土高原形成时的古风场有关，即风成沉积物磁化率椭球体主轴方向及各轴比值与磁性颗粒分布排列方式亦即与空气动力条件相关．阐明了风成沉积物磁组构形成机制及其与古风向的关系，提出一种能够定量研究黄土高原形成时古风场的方法，为研究黄土高原形成演化和第四纪以来气候变化提供了基础数据．     

CLIMATIC CHARACTERISTICS OF ATMOSPHERIC NET RADIATION OVER CHINA*

In terms of ERBE and ISCCP data.and measured/calculated surface net radiation,computation is performed of the climatic characteristics of ANR(atmospheric net radiation) across China alongside with the discussion and relations to other two kinds of radiation and contributing factors.Evidence suggests a high linear correlation of ANR with atmosphere-absorbed shortwave radiation.whereby can be established a general expression for ANR,which decreases more sharply as a function of altitude and increases slightly with latitude in summer,and changes uniformly in winter.Eventually,a comparison is made of the findings presented in this paper and literatures regarding the ANR pattern and magnitudes,indicating their great difference.     

Tunable diode laser measurements of trace gases during the 1988 Polarstern cruise and intercomparisons with other methods

Measurements of NO₂, HCHO, and H₂O₂ were made by the highly specific method of mid infra-red absorption spectroscopy using tunable diode lasers (TDLAS) during the 1988 Polarstern expedition. The TDLAS data are compared to those obtained during the cruise using less direct methods. Southern Hemisphere NO₂ levels suggest nett photochemical destruction of O₃ in the boundary layer. Northern Hemisphere HCHO averaged 0.47±0.2 ppbv; the HCHO measurements are used in a simple calculation to estimate OH noontime maxima of 3–6×10⁶ cm^-3.     

Comments on the origin of dust in East Antarctica for present and ice age conditions

We have studied the distribution of 327 clay mineral particles retrieved from four Antaretic ice smaples corresponding to present and Last Glacial Maximum (LGM) climate conditions. Illite, chlorite, smectite and kaolinite were identified in all samples. Focusing on kaolinite, because of its use as a possible tracer of low latitude soils, we find a significantly smaller amount for LGM samples while the dust concentration in snow during the LGM was about 30 times higher than for present climate conditions. This can be interpreted as change in the contribution of the Australian source with climate.A second approach was based on the modeling of the desert dust cycle using an Atmospheric General Circulation Model (AGCM) under both present-day and ice age conditions. Unlike mineralogical results, the model suggests the prevalence of the Australian dust source in the deposits over East Antarctica under both present-day and LGM climate conditions. However the model fails to reproduce the strong increase in dust deposits during the LGM. This discrepancy could be partly due to the lack of a higher latitude dust source in the model.The stronger dust input recorded in ice cores for the LGM could be related to an additional active high latitude source (possibly close to South America) overlapping the atmospheric background coming from low latitude areas.