边界层温度廓线遥感反演的本地化改进研究

采用MODIS资料和美国发展的MODIS大气温、湿度廓线统计反演算法,估算大气温度、湿度廓线作为初始场,应用101层快速透过率模式(PFAAST)估算了大气透过率,并采用Newton非线性迭代算法反演中国西北荒漠戈壁地区大气温度廓线。结果表明:该方法对边界层高度及以上部分的大气温度反演得比较好,误差基本都在2 K范围内,边界层范围内的温度反演误差较大,反演误差与气溶胶光学厚度增量和地表温度估算误差呈显著正相关关系,与大气水汽混合比的关系较差。文中从敏感性试验和理论分析角度阐述了地表温度和气溶胶光学厚度估算误差对大气温度反演误差的影响,发现不同光谱波段的地表温度权重均随地表温度的增加有不同程度增加,地表温度反演误差增加将增加地表温度权重,提高地表温度估算误差有助于提高地表温度权重的精度;荒漠戈壁地区大气边界层中气溶胶浓度较高,光学厚度较大,使边界层大气透过率降低,进而降低卫星红外遥感波段的地表温度权重和空气温度权重。由于该模式没有很好地考虑边界层中沙尘气溶胶的影响,使卫星反演的大气透过率偏高,以至于高估地表温度权重和大气温度权重,使得反演的表面温度和空气温度偏低。该研究结合太阳光度计获得的光学厚度资料,采用统计方法对气溶胶效应引起的大气透过率误差和表面温度估算误差进行校正,并对物理算法进行本地化改进,实现了边界层温度廓线的反演。     

半干旱草地地表土壤热通量的计算及其对能量平衡的影响

利用2008年7月兰州大学半干旱气候与环境观测(SACOL)站的观测资料,对比分析了地表土壤热通量的三种计算方法,即谐波法、温度预报校正法(TDEC法)以及结合自校正热通量板(HFP01SC)测量的温度积分法(ITHP法);进而分析了三种不同方法的计算结果对地表能量平衡的影响。比较5cm深度处谐波法和TDEC法的计算结果与HFP01SC的实测结果,三者的相位基本一致,相互之间均具有很好的线性关系;谐波法与TDEC法的计算值较为接近,但分别比HFP01SC的实测值偏大了2%和6%(主要发生在夜间)。对于地表的土壤热通量(G0),谐波法与TDEC法两者的计算结果仅偏差约1%;TDEC法与ITHP法的计算结果之间也具有很好的线性关系(R2=0.99),但偏差达到9%左右。相对于HFP01SC的实测结果,由谐波法和TDEC法计算的G0可将SACOL站的地表能量闭合率分别提高6%和7%左右;利用温度积分法将HFP01SC的实测结果校正到地表后,地表能量闭合率也提高了约6%。因此,在对涡动相关通量做了常规订正的情况下,当充分考虑了土壤热存储后,SACOL站的地表能量闭合率可提高6%～7%,达到82%～83%左右。     

Kinetics of the reactions of Cl atoms with 2-buten-1-ol, 2-methyl-2-propen-1-ol, and 3-methyl-2-buten-1-ol as a function of temperature

The reactions of three structurally similar unsaturated alcohols, 2-buten-1-ol (crotyl alcohol), 2-methyl-2-propen-1-ol (MPO221) and 3-methyl-2-buten-1-ol (MBO321) with Cl atoms, have been investigated for the first time, using a 400 l Teflon reaction chamber coupled with gas chromatograph-coupled with flame-ionization detection (GC-FID). The experiments were performed at atmospheric pressure and at temperatures between 255 and 298 K, in air or nitrogen as the bath gas. The obtained kinetic data were used to derive the Arrhenius expressions , , (in units of cm³ molecule⁻¹ s⁻¹). Finally, atmospheric lifetimes of those unsaturated alcohols with respect to OH, NO₃, O₃ and Cl have been calculated.     

庐山2008和2009年两次冰冻天气对比分析

利用高空与地面观测资料,主要从形势场、温度层结、地理形势及地面气象要素等方面,对庐山2008年和2009年两次冰冻天气过程进行对比分析。结果表明,庐山2009年冰冻灾害与2008年初中国南方出现的大范围冰冻灾害有些不同特点,2009年冰冻灾害更具有明显的庐山局部性特征。认为庐山冰冻灾害的出现主要决定于925—850hPa层次的温度层结,当层结温度降为0℃以下并伴有较明显降水时,并不一定需要太长时间和明显逆温层的存在庐山就可以出现冰冻灾害。     

东海黑潮暖舌的演变及其对我国气温的影响

利用高分辨率的海温分析资料模式资料,分析了黑潮暖舌与我国气温的关系,初步探讨了太平洋年代际振荡(PDO)等造成黑潮暖舌变化的可能原因。结果表明,冬季和春季东海黑潮暖舌存在明显的年际和年代际变化。暖舌在1996/1997年发生了一次突变,此前暖舌处在偏冷的状态,之后转为偏暖的状态。我国冬季和春季气温存在一定的年代际变化,1997年之后,冬季除东北和新疆外,气温有所偏高,而春季气温全国表现为一致的显著偏高。冬季和春季气温对黑潮暖舌存在邻(域)响应。冬季东海黑潮暖舌指数与冬季我国东部气温存在正相关,并且这一相关性能够延续到次年春季。冬季黑潮暖舌指数与我国4月海陆热力差异指数也存在显著的正相关。当冬季暖舌偏强(弱)时,4月海陆热力差异指数偏高(低),即东亚地区海陆热力差异偏大(小)。春季黑潮暖舌指数与春季我国中部及南方地区气温也存在正相关,当春季黑潮暖舌偏强(弱)时,上述地区气温将偏高(低)。PDO和黑潮暖舌之间的相互作用存在一个反馈机制。西风的增强,可通过使海洋向大气释放热量增加和向南的埃克曼(Ekman)输送,降低北太平洋中部的SST,而这一地区SST的降低对应着PDO的暖位相。增强的负风应力旋度在北太平洋副热带流涡中强迫出的向南斯维尔德鲁普(Sverdrup)流也偏强,而向北流动的东海黑潮的增强正是补偿了这一向南的海流。黑潮增强后经过两个月将大量热量输送至北太平洋中部,增强了这一地区的SST,而这对应着PDO的冷位相。     

百叶箱和通风防辐射罩气温观测系统的数据对比与订正

气温是常规地面气象观测的基本要素,其观测方法和误差直接关系到对大气过程的理解和预报精度。开展不同气温观测系统间的对比和分析,保证观测数据的准确性和可比较性,对大气科学以及天气气候的预测、预报研究具有重要意义。本文利用2009年9月至2010年8月的对比实验数据,分析了百叶箱气温观测系统和通风防辐射罩气温观测系统的数据差异,讨论了系统误差与环境温度以及辐射误差与太阳辐射和环境风速之间的关系,给出了相应的订正方法,最后对订正效果进行了检验。结果表明:与通风防辐射罩的气温数据相比,百叶箱的气温数据偏高,其中夜间平均偏高0.19°C,白天平均偏高0.29°C;系统误差是环境温度的一元线性函数,气温每升高1°C,系统误差就会增加0.006°C左右;辐射误差是太阳辐射与环境风速互相耦合作用的结果:太阳辐射有较强的增温效应,与辐射误差呈现近似的抛物线函数关系;环境风速有较好的冷却效应,与辐射误差呈现出近似的负指数函数关系;经误差订正后,夜间和白天的数据误差均减小到了0.0°C,-0.2~0.2°C的样本比例分别从订正前的64.5%和45.3%提高到了83.7%和80.6%,一致率提高到了92.3%和96.0%。     

CHARACTERISTICS OF MEI-YU PRECIPITATION AND SVD ANALYSIS OF PRECIPITATION OVER THE YANGTZE-HUAIHE RIVERS VALLEYS AND THE SEA SURFACE TEMPERATURE IN THE NORTHERN PACIFIC OCEAN

Based on the precipitation data of Meiyu at 37 stations in the valleys of Yangtze and Huaihe Rivers from 1954 to 2001, the temporal-spatial characteristics of Meiyu precipitation and their relationships with the sea surface temperature in northern Pacific are investigated using such methods as harmonic analysis, empirical orthogonal function (EOF), composite analysis and singular value decomposition (SVD). The results show that the temporal evolution and spatial distribution of Meiyu precipitation are not homogeneous in the Yangtze-Huaihe Rivers basins but with prominent inter-annual and inter-decadal variabilities. The key region between the anomalies of Meiyu precipitation and the monthly sea surface temperature anomalies (SSTA) lies in the west wind drift of North Pacific, which influences the precipitation anomaly of Meiyu precipitation over a key period of time from January to March in the same year. When the SST in the North Pacific west wind drift is warmer (colder) than average during these months, Meiyu precipitation anomalously increases (decreases) in the concurrent year. Results of SVD are consistent with those of composite analysis which pass the significance test of Monte-Carlo at 0.05.     

2008年初贵州低温雨雪凝冻灾害天气成因分析

利用NECP 2.5°×2.5°的日平均再分析资料和常规观测资料,对2008年1月12日-2月13日期间贵州省历史罕见的持续低温雨雪凝冻天气过程的环流特征及物理量进行了分析,并对中东部凝冻严重的前期和西部凝冻严重的后期做了对比.揭示了此次灾害天气的几个主要天气特征:(1)地面静止锋的位置关系着我省低温雨雪凝冻灾害的区域.(2)500 hPa环流前期和后期影响系统明显不同.过程期间欧亚大陆500 hPa高度场距平呈"北高南低"分布,亚洲区极涡南掉,面积偏大.(3)过程前期850 hPa冷舌明显,等温线密集;后期700 hPa 温降低,有冷舌活动,850 hPa冷舌明显减弱,低温维持.中东部和西部地区冷暖平流垂直方向上的配制不同.强盛的700 hPa暖湿气流是此次过程的主要水汽来源.     

红外焦平面探测器信息获取与预处理电路设计

针对中国科学院上海技术物理研究所研制的1500元红外线列焦平面探测器的输出特性,提出了以低噪声运放为核心的信息获取电路和以FPGA(Field Programmable Gate Array)为核心的数据预处理的设计方案,实现了驱动电路和探测器的良好匹配,较好地发挥了探测器高灵敏度的特性.测试结果表明,该方案不仅对系统获得优于50 mK噪声等效温差的高灵敏度成像起到了重要作用,足够宽的量化设计还保证了系统的动态范围和图像的丰富层次.该设计方案已成功应用在一些其他类型的红外焦平面探测器中.     

Coupling photochemistry with haze formation in Titan's atmosphere, Part II: Results and validation with Cassini/Huygens data

The new one-dimensional radiative-convective/photochemical/microphysical model described in Part I is applied to the study of Titan's atmospheric processes that lead to haze formation. Our model generates the haze structure from the gaseous species photochemistry. Model results are presented for the species vertical concentration profiles, haze formation and its radiative properties, vertical temperature/density profiles and geometric albedo. These are validated against Cassini/Huygens observations and other ground-based and space-borne measurements. The model reproduces well most of the latest measurements from the Cassini/Huygens instruments for the chemical composition of Titan's atmosphere and the vertical profiles of the observed species. For the haze production we have included pathways that are based on pure hydrocarbons, pure nitriles and hydrocarbon/nitrile copolymers. From these, the nitrile and copolymer pathways provide the stronger contribution, in agreement with the results from the ACP instrument, which support the incorporation of nitrogen in the pyrolized haze structures. Our haze model reveals a new second major peak in the vertical profile of haze production rate between 500 and 900 km. This peak is produced by the copolymer family used and has important ramifications for the vertical atmospheric temperature profile and geometric albedo. In particular, the existence of this second peak determines the vertical profile of haze extinction. Our model results have been compared with the DISR retrieved haze extinction profiles and are found to be in very good agreement. We have also incorporated in our model heterogeneous chemistry on the haze particles that converts atomic hydrogen to molecular hydrogen. The resultant H₂ profile is closer to the INMS measurements, while the vertical profile of the diacetylene formed is found to be closer to that of the CIRS profile when this heterogenous chemistry is included.