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81.
Measurements of CO2 fluxes from open-vent volcanos are rare, yet may offer special capabilities for monitoring volcanos and forecasting activity.
The measured fluxes of CO2 and SO2 from Mount St. Helens decreased from July through November 1980, but the record includes variations of CO2/SO2 in the emitted gas and episodes of greatly increased fluxes of CO2. We propose that the CO2 flux variations reflect two gas components: (a) a component whose flux decreased in proportion to 1/ √t with a CO2/SO2 mass ratio of 1.7, and (b) a residual flux of CO2 consisting of short-lived, large peaks with a CO2/SO2 mass ratio of 15. We propose two hypotheses: (a) the 1/ √t dependence was generated by crystallization in a deep magma body at rates governed by diffusion-limited heat transfer, and
(b) the gas component with the higher CO2/SO2 was released from ascending magma, which replenished the same magma body. The separation of the total CO2 flux into contributions from known processes permits quantitative inferences about the replenishment and crystallization
rates of open-system magma bodies beneath volcanos. The flux separations obtained by using two gas sources with distinct CO2/SO2 ratios and a peak minus background approach to obtain the CO2 contributions from an intermittent source and a continuously emitting source are similar. The flux separation results support
the hypothesis that the second component was generated by episodic magma ascent and replenishment of the magma body. The diffusion-limited
crystallization hypothesis is supported by the decay of minimum CO2 and SO2 fluxes with 1/ √t after 1 July 1980. We infer that the magma body at Mount St. Helens was replenished at an average rate (2.8×106 m3 d–1) which varied by less than 5% during July, August, and September 1980. The magma body volume (2.4–3.0 km3) in early 1982 was estimated by integrating a crystallization rate function inferred from CO2 fluxes to maximum times (20±4 years) estimated from the increase of sample crystallinity with time. These new volcanic gas
flux separation methods and the existence of relations among the CO2 flux, crystallization rates, and magma body replenishment rates yield new information about the dynamics of an open-vent,
replenished magma body.
Received: 15 February 1995 / Accepted: 30 March 1996 相似文献
82.
The 1783–1784 Laki tholeiitic basalt fissure eruption in Iceland was one of the greatest atmospheric pollution events of
the past 250 years, with widespread effects in the northern hemisphere. The degassing history and volatile budget of this
event are determined by measurements of pre-eruption and residual contents of sulfur, chlorine, and fluorine in the products
of all phases of the eruption. In fissure eruptions such as Laki, degassing occurs in two stages: by explosive activity or
lava fountaining at the vents, and from the lava as it flows away from the vents. Using the measured sulfur concentrations
in glass inclusions in phenocrysts and in groundmass glasses of quenched eruption products, we calculate that the total accumulative
atmospheric mass loading of sulfur dioxide was 122 Mt over a period of 8 months. This volatile release is sufficient to have
generated ∼250 Mt of H2SO4 aerosols, an amount which agrees with an independent estimate of the Laki aerosol yield based on atmospheric turbidity measurements.
Most of this volatile mass (∼60 wt.%) was released during the first 1.5 months of activity. The measured chlorine and fluorine
concentrations in the samples indicate that the atmospheric loading of hydrochloric acid and hydrofluoric acid was ∼7.0 and
15.0 Mt, respectively. Furthermore, ∼75% of the volatile mass dissolved by the Laki magma was released at the vents and carried
by eruption columns to altitudes between 6 and 13 km. The high degree of degassing at the vents is attributed to development
of a separated two-phase flow in the upper magma conduit, and implies that high-discharge basaltic eruptions such as Laki
are able to loft huge quantities of gas to altitudes where the resulting aerosols can reside for months or even 1–2 years.
The atmospheric volatile contribution due to subsequent degassing of the Laki lava flow is only 18 wt.% of the total dissolved
in the magma, and these emissions were confined to the lowest regions of the troposphere and therefore important only over
Iceland. This study indicates that determination of the amount of sulfur degassed from the Laki magma batch by measurements
of sulfur in the volcanic products (the petrologic method) yields a result which is sufficient to account for the mass of
aerosols estimated by other methods.
Received: 30 May 1995 / Accepted: 19 April 1996 相似文献