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Treatment with metallic copper for the removal of elemental sulfur from bitumen extracted from sedimentary rocks or petroleum is the most widely used method. Little attention has been paid, however, to its disadvantages. It was observed that copper can interact with some polar organic substances during conventional sulfur removal, which can strongly influence the quantitative and qualitative determination of bitumen, as has been confirmed by interaction of long-chain fatty acids with copper. The copper soap generated was analyzed by element analysis, inductively coupled plasma optical emission spectrometry (ICP-OES), thermal analysis (TG-DSC) and Fourier Transform Infrared spectroscopy (FFIR). Mechanism of the interaction was investigated and elucidated. Our experimental results would necessitate improvement of the present method for sulfur removal and/or a search for a new one. 相似文献
84.
GPS observations of the ionospheric F2-layer behavior during the 20th November 2003 geomagnetic storm over South Korea 总被引:4,自引:1,他引:3
The ionospheric F2-layer peak density (NmF2) and its height (hmF2) are of great influence on the shape of the ionospheric
electron density profile Ne (h) and may be indicative of other physical processes within the ionosphere, especially those
due to geomagnetic storms. Such parameters are often estimated using models such as the semiempirical international reference
ionosphere (IRI) models or are measured using moderately priced to expensive instrumentation, such as ionosondes or incoherent
scatter radars. Global positioning system (GPS) observations have become a powerful tool for mapping high-resolution ionospheric
structures, which can be used to study the ionospheric response to geomagnetic storms. In this paper, we describe how 3-D
ionospheric electron density profiles were produced from data of the dense permanent Korean GPS network using the tomography
reconstruction technique. These profiles are verified by independent ionosonde data. The responses of GPS-derived parameters
at the ionospheric F2-layer to the 20th November 2003 geomagnetic storm over South Korea are investigated. A fairly large
increase in the electron density at the F2-layer peak (the NmF2) (positive storm) has been observed during this storm, which
is accompanied by a significant uplift in the height of the F2 layer peak (the hmF2). This is confirmed by independent ionosonde
observations. We suggest that the F2-layer peak height uplift and NmF2 increase are mainly associated with a strong eastward
electric field, and are not associated with the increase of the O/N2 ratio obtained from the GUVI instruments aboard the TIMED satellite. It is also inferred that the increase in NmF2 is not
caused by the changes in neutral composition, but is related to other nonchemical effects, such as dynamical changes of vertical
ion motions induced by winds and E × B drifts, tides and waves in the mesosphere/lower thermosphere region, which can be dynamically
coupled upward to generate ionospheric perturbations and oscillations. 相似文献
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在夏季分层期间对红枫湖南、北湖湖心的水样进行分层采集,同时测定了分层水样的温度、pH、HCO3-浓度、溶解氧(DO)、叶绿素a(Chl-a)及铵根离子(NH4+)、硝酸根离子(NO3-)、磷酸根离子(PO43-)的浓度,水体中CO2的分压(pCO2)由化学平衡及亨利定律求得。研究结果表明:光合作用、有机质降解及水体热分层是影响红枫湖夏季pCO2分布的主要因素。其中,温水层CO2欠饱和是光合作用吸收CO2引起的,温跃层中pCO2的急剧增加是光合产物降解产生CO2引起的。静水层沉积物附近pCO2最高并且还有持续增加的趋势,说明沉积物中有机质降解是静水层中CO2增加的主要原因,夏季湖底水温较高加快了沉积物中有机质的降解。分层现象使pCO2在水体中的分布差别明显,并且使静水层中CO2得到积累。此外,夏季红枫湖水体中pCO2的变化与NH4+、PO43-的变化密不可分,表现为温水层中光合作用消耗NH4+、PO43-,有机质降解过程伴随NH4+、PO43-的释放。 相似文献
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通过对呼伦贝尔市煤矿地质环境敏感性的综合评价,结合当地实际情况,提出了以修筑拦挡建筑物、支撑与坡面防护、锚固、排水、选择更合理的开采工艺等技术手段,对该地区地质灾害进行防治的方案。方案对海拉尔河河道治理、生物措施、井下回填工程、加固边坡、抽排水、发展煤矸石砖厂、移民避让、招商引资8个部分提出了防治方法,促进地质环境治理工作的进行。 相似文献
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Analyses of 72 samples from Upper Panjhara basin in the northern part of Deccan Plateau, India, indicate that geochemical
incongruity of groundwater is largely a function of mineral composition of the basaltic lithology. Higher proportion of alkaline
earth elements to total cations and HCO3>Cl + SO4 reflect weathering of primary silicates as chief source of ions. Inputs of Cl, SO4, and NO3 are related to rainfall and localized anthropogenic factors. Groundwater from recharge area representing Ca + Mg–HCO3 type progressively evolves to Ca + Na–HCO3 and Na–Ca–HCO3 class along flow direction replicates the role of cation exchange and precipitation processes. While the post-monsoon chemistry
is controlled by silicate mineral dissolution + cation exchange reactions, pre-monsoon variability is attributable chiefly
to precipitation reactions + anthropogenic factors. Positive correlations between Mg vs HCO3 and Ca + Mg vs HCO3 supports selective dissolution of olivine and pyroxene as dominant process in post-monsoon followed by dissolution of plagioclase
feldspar and secondary carbonates. The pre-monsoon data however, points toward the dissolution of plagioclase and precipitation
of CaCO3 supported by improved correlation coefficients between Na + Ca vs HCO3 and negative correlation of Ca vs HCO3, respectively. It is proposed that the eccentricity in the composition of groundwater from the Panjhara basin is a function
of selective dissolution of olivine > pyroxene followed by plagioclase feldspar.
The data suggest siallitization (L < R and R
k) as dominant mechanism of chemical weathering of basalts, stimulating monosiallitic (kaolinite) and bisiallitic (montmorillonite)
products. The chemical denudation rates for Panjhara basin worked out separately for the ground and surface water component
range from 6.98 to 36.65 tons/km2/yr, respectively. The values of the CO2 consumption rates range between 0.18 × 106 mol//km2/yr (groundwater) and 0.9 × 106 mol/km2/yr (surface water), which indicates that the groundwater forms a considerable fraction of CO2 consumption, an inference, that is, not taken into contemplation in most of the studies. 相似文献