区域酸性沉降的数值研究：Ⅱ.个例模拟和试验

利用建立的区域酸性污染物沉降模式，配合中尺度模式ＭＭ４预报的气象场，以１９９１年６月１２￣１４日淮河流域的一次降雨过程作为实例，对我国东半部及其相邻地区的酸沉降进行了数值模拟和试验研究。结果表明，模式基本上能够模拟出区域酸性沉降的特征，具有良好的综合模拟性能和广阔的应用前景。     

Simulation of Tropospheric Ozone with MOZART-2： An Evaluation Study over East Asia

Climate changes induced by human activities have attracted a great amount of attention. With this, a coupling system of an atmospheric chemistry model and a climate model is greatly needed in China for better understanding the interaction between atmospheric chemical components and the climate. As the first step to realize this coupling goal, the three-dimensional global atmospheric chemistry transport model MOZART-2 (the global Model of Ozone and Related Chemical Tracers, version 2) coupled with CAM2 (the Community Atmosphere Model, version 2) is set up and the model results are compared against observations obtained in East Asia in order to evaluate the model performance. Comparison of simulated ozone mixing ratios with ground level observations at Minamitorishima and Ryori and with ozonesonde data at Naha and Tateno in Japan shows that the observed ozone concentrations can be reproduced reasonably well at Minamitorishima but they tend to be slightly overestimated in winter and autumn while underestimated a little in summer at Ryori. The model also captures the general features of surface CO seasonal variations quite well, while it underestimates CO levels at both Minamitorishima and Ryori. The underestimation is primarily associated with the emission inventory adopted in this study. Compared with the ozonesonde data, the simulated vertical gradient and magnitude of ozone can be reasonably well simulated with a little overestimation in winter, especially in the upper troposphere. The model also generally captures the seasonal, latitudinal and altitudinal variations in ozone concentration. Analysis indicates that the underestimation of tropopause height in February contributes to the overestimation of winter ozone in the upper and middle troposphere at Tateno.     

对流层大气的负熵流和熵产生

将原始熵平衡方程应用于大气系统，详细计算了对流层大气平均状态下的负熵流和熵产生及其各项分量，得出了它们之间的一些数量关系，并应用熵理论初步解释了大气运动的某些规律，对于天气预报和气候变化的研究具有一定参考意义。     

准实时地基GPS可降水量的解算方案与可靠性研究

对准实时地基GPS可降水量的解算方案与可靠性的探讨,围绕三个方面展开:准实时GPS对流层延迟解算的最佳方案的确定;GPS可降水量与无线电探空资料的比较;GPS可降水量与水汽辐射计数据的比较。为了实时应用于气象领域,准实时对流层延迟的最佳方案为快速预报星历松弛解。在快速预报星历松弛解GPS可降水量与无线电探空数据的比较中,两者的相关性为0.88,绝对值均值为5.4 mm。GPS可降水量与水汽辐射计资料比较得到两者差值的均方根为1.68 mm。最后得到了最佳的准实时地基GPS可降水量的解算方案和在气象领域可降水量的反演的可行性的结论。     

基于OMI的亚洲地区对流层NO2高分辨率反演产品POMINO v2.1及其与其他产品的定量对比

对流层二氧化氮(NO₂)是一种重要的痕量污染气体。现有基于OMI卫星探测器、覆盖亚洲地区的NO₂公开产品QA4ECV、OMNO2和POMINO受到广泛使用,然而对于这3个产品的差异的定量认识仍然不足。我们将前期开发的POMINO产品进行了改进和优化,更新至v2.1并将反演区域扩大至覆盖东亚、东南亚和南亚大部分地区,随后定量分析了QA4ECV、OMNO2 v4和POMINO v2.1对流层NO₂垂直柱浓度在2015年—2020年在不同采样条件下的异同。结果显示,POMINO版本的更新对自身NO₂柱浓度反演结果的整体影响较小(<10%)。当3个产品均基于POMINO v2.1进行一致采样时,产品之间在整个亚洲区域的平均差异约为10%,在京津冀等污染地区的差异最高可达40%。3个产品均显示,京津冀地区NO₂柱浓度在五年间下降了约30%,而长三角地区的变化趋势较小。当3个产品进行分别采样时,POMINO v2.1的有效数据量比其他两个产品增加了11%—44%,特别是更好地保留了重...     

Stratospheric Ozone-induced Cloud Radiative Effects on Antarctic Sea Ice

Recent studies demonstrate that the Antarctic Ozone Hole has important influences on Antarctic sea ice. While most of these works have focused on effects associated with atmospheric and oceanic dynamic processes caused by stratospheric ozone changes, here we show that stratospheric ozone-induced cloud radiative effects also play important roles in causing changes in Antarctic sea ice. Our simulations demonstrate that the recovery of the Antarctic Ozone Hole causes decreases in clouds over Southe...     

南极对流层-平流层下部气候变化特征及其原因

利用南极16站30余年地面至30hPa10层月平均气温距平序列资料,采用最大熵功率谱方法,研究了南极对流层至平流层下部气候变化的长期趋势和周期性特征,并讨论了平流层(对流层)气候变化与南极臭氧总量(南半球500hPa环流)变化之间的联系。指出:南极气温具有明显的长期趋势和周期性变化;平流层下部显着变冷、对流层增暖,变化最大层高度在100、700hPa,最大降冷速率远大于增暖速率,气层稳定度趋于减弱;30、50hPa气温具有准两年周期,100hPa上下具有显着的年周期,对流层是以3.5年甚低频周期为主;对流层顶气温无显着趋势变化和周期性变化;南极最大臭氧层高度显着变冷与近15年来臭氧层损耗有关。南半球对流层中部极涡及绕极气流减弱是南极对流层气候变暖的直接原因。