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31.
本文首次报道用沉积物捕捉器(ST)研究南沙群岛珊瑚礁湖沉降颗粒物中主要元素垂直通量、垂直转移形态、再循环过程及垂直通量与表层海水温度的关系。结果显示,作为生物化学沉积标志的Ca、Mg具有最高的垂直通量,达1.4和0.1g/(m2·d)以上,作为生物富集标志的Br、Ⅰ也有较高的垂直转移量;垂直转移形态的研究表明Na、K、Ca、Mg、Sr主要以碳酸盐结合态向海底转移,其中Ca、Mg、Sr占99%以上,Fe、I、Ba主要以铁锰氧化物结合态向海底输送,在垂直沉降颗粒物到达海底后,有相当部分的主要元素可再循环进入水体中,Br、I、K、Al的绝大部分进入再循环,Mg、Na、Cl有一半左右进入再循环,Ca、Sr、Ba、Fe大部分被埋葬;Na等9种元素的垂直转移量随SST呈指数降低响应,对SST的敏感性Fe>Br>Sr>Ca>Na>Cl>Mg>I>Al,这再一次验证了CaCO3随温度升高,其溶解度降低、化学沉积量增加这一自然界的普遍规律,表明在珊瑚礁海水的垂直沉降颗粒物中主要元素是作为珊瑚的重要成分与CaCO3一同被沉积下来的,CaCO3起到稀释剂的作用。 相似文献
32.
33.
The behavior of the Mediterranean ecosystem in response to realistic riverine inputs and dissolved matter exchange is investigated. The strategy is to evaluate the stability of the ecosystem subjected to various atmospheric inputs. 相似文献
34.
A VERTICAL DISTRIBUTION MODEL OF NUTRIENTS AND DISSOLVED OXYGEN IN THE SOUTHERN TAIWAN STRAIT 总被引:3,自引:0,他引:3
Sinoe vertical transport of nutrients and dissolved oxygen are quite important in the water col-umn and have drawn serious attention these recent years, a one-dmension numerical model is tried to simulate the vertical distribution of nutrients and dissolved oxygen in June at two research sites in the southemTaiwan Strait. Physical transport parameters are calibrated by temperature simulation, and thenare used to simulate the profiles of NO_3, PO_4 and dissolved oxygen. The simulation was generally success-ful for both stations. The importance of various factors, such as upwelling tidal current andbiogeochemical activities, which influence the vertical distribution of nutrients and dissolved oxygen, is revealed by analysis of the modeling results. Some important rates, fluxes and ratios are also estimated anddiscussed on the basis of simulation. 相似文献
35.
收集了以WolfgangFRogge博士研究工作为主的文献,对几种常见大气有机污染源进行了讨论,列出了由不同污染源所排放的可辨别有机合物的类别、含量以及用于定量分析和评价的示踪化合物。 相似文献
36.
Nitrogen and sulfur species in Antarctic aerosols at Mawson,Palmer Station,and Marsh (King George Island) 总被引:4,自引:0,他引:4
D. L. Savoie J. M. Prospero R. J. Larsen F. Huang M. A. Izaguirre T. Huang T. H. Snowdon L. Custals C. G. Sanderson 《Journal of Atmospheric Chemistry》1993,17(2):95-122
High volume bulk aerosol samples were collected continuously at three Antarctic sites: Mawson (67.60° S, 62.50° E) from 20 February 1987 to 6 January 1992; Palmer Station (64.77° S, 64.06° W) from 3 April 1990 to 15 June 1991; and Marsh (62.18° S, 58.30° W) from 28 March 1990, to 1 May 1991. All samples were analyzed for Na+, SO
4
2–
, NO
3
–
, methanesulfonate (MSA), NH
4
+
,210Pb, and7Be. At Mawson for which we have a multiple year data set, the annual mean concentration of each species sometimes vary significantly from one year to the next: Na+, 68–151 ng m–3; NO
3
–
, 25–30 ng m–3; nss SO
4
2–
, 81–97 ng m–3; MSA, 19–28 ng m–3; NH
4
+
, 16–21 ng m–3;210Pb, 0.75–0.86 fCi m–3. Results from multiple variable regression of non-sea-salt (nss) SO
4
2–
with MSA and NO
3
–
as the independent variables indicates that, at Mawson, the nss SO
4
2–
/MSA ratio resulting from the oxidation of dimethylsulfide (DMS) is 2.80±0.13, about 13% lower than our earlier estimate (3.22) that was based on 2.5 years of data. A similar analysis indicates that the ratio at Palmer is about 40% lower, 1.71±0.10, and more comparable to previous results over the southern oceans. These results when combined with previously published data suggest that the differences in the ratio may reflect a more rapid loss of MSA relative to nss SO
4
2–
during transport over Antarctica from the oceanic source region. The mean210Pb concentrations at Palmer and Marsh and the mean NO
3
–
concentration at Palmer are about a factor of two lower than those at Mawson. The210Pb distributions are consistent with a210Pb minimum in the marine boundary layer in the region of 40°–60° S. These features and the similar seasonalities of NO
3
–
and210Pb at Mawson support the conclusion that the primary source regions for NO
3
–
are continental. In contrast, the mean concentrations of MSA, nss SO
4
2–
, and NH
4
+
at Palmer are all higher than those at Mawson: MSA by a factor of 2; nss SO
4
2–
by 10%; and NH
4
+
by more than 50%. However, the factor differences exhibit substantial seasonal variability; the largest differences generally occur during the austral summer when the concentrations of most of the species are highest. NH
4
+
/(nss SO
4
2–
+MSA) equivalent ratios indicate that NH3 neutralizes about 60% of the sulfur acids during December at both Mawson and Palmer, but only about 30% at Mawson during February and March. 相似文献
37.
The biogeochemical sulfur cycle in the marine boundary layer over the Northeast Pacific Ocean 总被引:1,自引:0,他引:1
T. S. Bates J. E. Johnson P. K. Quinn P. D. Goldan W. C. Kuster D. C. Covert C. J. Hahn 《Journal of Atmospheric Chemistry》1990,10(1):59-81
The major components of the marine boundary layer biogeochemical sulfur cycle were measured simultaneously onshore and off the coast of Washington State, U.S.A. during May 1987. Seawater dimethylsulfide (DMS) concentrations on the continental shelf were strongly influenced by coastal upwelling. Concentration further offshore were typical of summer values (2.2 nmol/L) at this latitude. Although seawater DMS concentrations were high on the biologically productive continental shelf (2–12 nmol/L), this region had no measurable effect on atmospheric DMS concentrations. Atmospheric DMS concentrations (0.1–12 nmol/m3), however, were extremely dependent upon wind speed and boundary layer height. Although there appeared to be an appreciable input of non-sea-salt sulfate to the marine boundary layer from the free troposphere, the local flux of DMS from the ocean to the atmosphere was sufficient to balance the remainder of the sulfur budget. 相似文献
38.
39.
We have theoretically considered the problem of interpretation of nutrient profiles in the upper ocean (100–2000m). We compare
the experimental depth profiles of nonconservative tracers, both stable and radioactive, with solutions of one-dimensional
steady state transport equations of increasing complexity including situations not encountered in the real oceans. Apart from
gaining insight into the nutrient transport processes, this analysis is useful in offering a way to obtain operational estimates
of depth dependent/independent eddy diffusivity and dissolution fluxes in the ocean. These parameters are essential for estimating
new production, total production and burial of carbon in the sediments. 相似文献
40.
P. L. Smart T. C. Atkinson I. M. S. Laidlaw M. D. Newson S. T. Trudgill 《地球表面变化过程与地形》1986,11(3):249-261
The relative advantages of fluorescent dyes and Lycopodium spores as tracers are discussed. The major advantage of fluorescent dyes is that they may be detected quantitatively. Thus, in combination with discharge measurements, a dye mass balance can be prepared for tracer tests in karst conduits, which permits elucidation of the underground network. The advantages of this procedure are illustrated by comparison of the networks derived from non-quantitative (Lycopodium and dye) and quantitative (fluorescent dye) tracer methods in the Traligill Basin, Scotland. These tests also suggest that Lycopodium does not give a true indication of travel time, due to sedimentation underground. This could also cause contamination problems in later tests. For non-quantitative tracer tests, sensitive methods are necessary if incorrect inferences on conduit networks are to be avoided. In general, however, quantitative tests give much less ambiguous results, and are therefore to be preferred. 相似文献